Corrosion Properties of Oxide Ceramic Coatings Based on Alloys of the Al–Cu–Mg and Al–Mg Systems

By the methods of electrochemical impedance spectroscopy and potentiodynamic methods, we estimate the corrosion resistance of oxide ceramic coatings obtained on Al–Cu–Mg and Al–Mg alloys in the course of ozone bubbling. The results are compared with the data on the corrosion resistance of materials...

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Vydané v:	Materials science (New York, N.Y.) Ročník 57; číslo 2; s. 256 - 263
Hlavní autori:	Bilyi, L. M., Posuvailo, V. M., Ivashkiv, V. R., Kovalchuk, I. V.
Médium:	Journal Article
Jazyk:	English
Vydavateľské údaje:	New York Springer US 01.09.2021 Springer Springer Nature B.V
Predmet:	Alloys Aluminum base alloys Analysis Aqueous solutions Ceramic coatings Ceramic glazes Ceramics Characterization and Evaluation of Materials Chemistry and Materials Science Copper Corrosion resistance Electrochemical impedance spectroscopy Magnesium Materials Materials Science Protective coatings Sodium chloride Solid Mechanics Specialty metals industry Structural Materials aluminum oxides corrosion alloy plasma-electrolyte oxidation oxide ceramic coatings X-ray diffraction analysis
ISSN:	1068-820X, 1573-885X
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Abstract	By the methods of electrochemical impedance spectroscopy and potentiodynamic methods, we estimate the corrosion resistance of oxide ceramic coatings obtained on Al–Cu–Mg and Al–Mg alloys in the course of ozone bubbling. The results are compared with the data on the corrosion resistance of materials produced by using standard methods. The capacitance of all obtained oxide-ceramic coatings after 90 days is stabilized and becomes equal to 1–4 pF/cm 2 . Their corrosion resistance of the D16 alloy is twice higher than for the AMg5 alloy. All developed coatings are characterized by the elevated protective properties and their resistance in a 3% aqueous solution of sodium chloride is 1–4 G Ω ⋅ cm 2 .
AbstractList	By the methods of electrochemical impedance spectroscopy and potentiodynamic methods, we estimate the corrosion resistance of oxide ceramic coatings obtained on Al-Cu-Mg and Al-Mg alloys in the course of ozone bubbling. The results are compared with the data on the corrosion resistance of materials produced by using standard methods. The capacitance of all obtained oxide-ceramic coatings after 90 days is stabilized and becomes equal to 1-4 pF/cm.sup.2. Their corrosion resistance of the D16 alloy is twice higher than for the AMg5 alloy. All developed coatings are characterized by the elevated protective properties and their resistance in a 3% aqueous solution of sodium chloride is 1-4 G Î© · cm.sup.2. By the methods of electrochemical impedance spectroscopy and potentiodynamic methods, we estimate the corrosion resistance of oxide ceramic coatings obtained on Al–Cu–Mg and Al–Mg alloys in the course of ozone bubbling. The results are compared with the data on the corrosion resistance of materials produced by using standard methods. The capacitance of all obtained oxide-ceramic coatings after 90 days is stabilized and becomes equal to 1–4 pF/cm2. Their corrosion resistance of the D16 alloy is twice higher than for the AMg5 alloy. All developed coatings are characterized by the elevated protective properties and their resistance in a 3% aqueous solution of sodium chloride is 1–4 G Ω ⋅ cm2. By the methods of electrochemical impedance spectroscopy and potentiodynamic methods, we estimate the corrosion resistance of oxide ceramic coatings obtained on Al–Cu–Mg and Al–Mg alloys in the course of ozone bubbling. The results are compared with the data on the corrosion resistance of materials produced by using standard methods. The capacitance of all obtained oxide-ceramic coatings after 90 days is stabilized and becomes equal to 1–4 pF/cm 2 . Their corrosion resistance of the D16 alloy is twice higher than for the AMg5 alloy. All developed coatings are characterized by the elevated protective properties and their resistance in a 3% aqueous solution of sodium chloride is 1–4 G Ω ⋅ cm 2 .
Audience	Academic
Author	Posuvailo, V. M. Kovalchuk, I. V. Ivashkiv, V. R. Bilyi, L. M.
Author_xml	– sequence: 1 givenname: L. M. surname: Bilyi fullname: Bilyi, L. M. email: billevko@gmail.com organization: Karpenko Physicomechanical Institute, National Academy of Sciences of Ukraine – sequence: 2 givenname: V. M. surname: Posuvailo fullname: Posuvailo, V. M. organization: Karpenko Physicomechanical Institute, National Academy of Sciences of Ukraine – sequence: 3 givenname: V. R. surname: Ivashkiv fullname: Ivashkiv, V. R. organization: Karpenko Physicomechanical Institute, National Academy of Sciences of Ukraine – sequence: 4 givenname: I. V. surname: Kovalchuk fullname: Kovalchuk, I. V. organization: Karpenko Physicomechanical Institute, National Academy of Sciences of Ukraine
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References	I. B. Ivasenko, V. M. Posuvailo, H. H. Veselivska, and V. Vynar, “Porosity segmentation and analysis of oxide ceramic coatings of D16T alloy,” in: Proc. of the IEEE 15th Internat. Sci. -Techn. Conf. on Computer Sciences and Information Technologies, CSIT 2020, Vol. 2 (2020), pp. 50–53. I. V. Suminov, P. M. Belkin, A. V. Èpel’fel’d, V. B. Lyudin, B. L. Krit, and A. M. Borisov, Plasma-Electrolytic Modification of the Surfaces of Metals and Alloys [in Russian], Vols. 1-2, , Vol. 2, Tekhnosfera, Moscow (2011). PokhmurskiiVKorniySKopyletsVThe theoretical study of interaction of water chloride containing environment components with CuAl2 intermetallic surfaceJ. of Cluster Sci.201021135431:CAS:528:DC%2BC3cXis1entLY%3D10.1007/s10876-010-0279-9 HusseinRONieXNorthwoodDOAn investigation of ceramic coating growth mechanisms in plasma-electrolytic oxidation (PEO) processingElectrochim. Acta20131121111191:CAS:528:DC%2BC3sXhvFSksbjK10.1016/j.electacta.2013.08.137 M. M. Student, I. B. Ivasenko, V. M. Posuvailo, Y. Y. Sirak, and V. M. Yus’kiv, “Influence of the porosity of a plasma-electrolytic coating on the corrosion resistance of D16 alloy,” Fiz.-Khim. Mekh. Mater.,54, No. 4, 130–137 (2018), English translation: Mater. Sci.,54, No. 6, 899–906 (2019). L. A. Snezhko, A. L. Erokhin, O. A. Kalinichenko, and D. O. Misnyankin, “Hydrogen release on the anode in the course of plasma electrolytic oxidation of aluminum,” Fiz.-Khim. Mekh. Mater.,52, No. 3, 111–119 (2016), English translation: Mater. Sci.,52, No. 3, 421–430 (2016). SnizhkoLOYerohinALPilkingtonAGurevinaNLMisnyankinaDOLeylandAMatthewsAAnodic processes in plasma electrolytic oxidation of aluminum in alkaline solutionsElectrochim. Acta200449208520951:CAS:528:DC%2BD2cXhs1Ckt7w%3D10.1016/j.electacta.2003.11.027 V. Hutsaylyuk, M. Student, V. Posuvailo, O. Student, Y. Sirak, V. Hvozdets’kyi, P. Maruchak, and H. Veselivska, “The properties of oxide-ceramic layers with Cu and Ni inclusions synthesizing by PEO method on top of the gas-spraying coatings on aluminum alloys,” Vacuum,179, 109–514 (2020). M. D. Klapkiv, “Simulation of synthesis of oxide-ceramic coatings in discharge channels of a metal-electrolyte system,” Fiz.-Khim. Mekh. Mater.,35, No. 2, 111–114 (1999), English translation: Mater. Sci.,35, No. 2, 279–283 (1999). BorisenkovaTAKaluzhinaSAAnodic behavior of aluminum in neutral electrolytes with different anionic compositionsKondens. Sredy Mezhph. Gran.20091121061091:CAS:528:DC%2BC3MXhtFyit7nM M. M. Student, V. M. Dovhunyk, V. M. Posuvailo, I. V. Koval’chuk, and V. M. Hvozdets’kyi, “Friction behavior of iron-carbon alloys in couples with plasma-electrolytic oxide-ceramic layers synthesized on D16T alloy,” Fiz.-Khim. Mekh. Mater.,53, No. 2, 63–70 (2017), English translation: Mater. Sci.,53, No. 2, 359–367 (2017). PosuvailoVMKulykVVDuriaginaZAStudentMMVasylivBDThe effect of electrolyte composition on the plasma electrolyte oxidation and phase composition of oxide ceramic coatings formed on 2024 aluminum alloyArch. Mat. Sci. Eng.202010524955 V. I. Chernenko, L. A. Snezhko, and I. I., Papanov, Application of Coatings by Anode-Arc Electrolysis [in Russian], Khimiya, Leningrad (1991), 127 pp. M. M. Student, H. H. Veselivska, O. S. Kalakhan, V. M. Hvozdetskyi, Kh. R. Zadorozhna, and Ya. Ya. Sirak, “Influence of the conditions of plasma-electrolytic treatment of D16T aluminum alloy on its corrosion resistance in 3% NaCl solution,” Fiz.-Khim. Mekh. Mater.,56, No. 4, 105–114 (2020), English translation: Mater. Sci.,56, No. 4, 550–559 (2021). M. M. Student, V. M. Posuvailo, H. H. Veselivs’ka, Ya. Ya. Sirak, and R. А. Yatsyuk, “Corrosion resistance of plasma-electrolytic layers on alloys and coatings of the Al–Cu–Mg system for various modes of heat treatment,” Fiz.-Khim. Mekh. Mater.,53, No. 6, 42–47 (2017), English translation: Mater. Sci.,53, No. 6, 789–795 (2017). M. D. Klapkiv, O. S. Chuchmarev, P. Ya. Sydor, and V. M. Posuvailo, “Thermodynamics of the interaction of aluminum, magnesium, and zirconium with components of an electrolytic plasma,” Fiz.-Khim. Mekh. Mater.,36, No. 1, 56–64 (2000), English translation: Mater. Sci.,36, No. 1, 66–79 (2000). N. I. Blok, Qualitative Chemical Analysis [in Russian], GNTIKhL, Moscow-Leningrad (1952). 540_CR3 RO Hussein (540_CR6) 2013; 112 540_CR1 540_CR2 540_CR14 540_CR17 TA Borisenkova (540_CR15) 2009; 11 V Pokhmurskii (540_CR16) 2010; 21 540_CR9 540_CR7 540_CR8 540_CR5 VM Posuvailo (540_CR11) 2020; 105 LO Snizhko (540_CR4) 2004; 49 540_CR10 540_CR13 540_CR12
References_xml	– reference: V. Hutsaylyuk, M. Student, V. Posuvailo, O. Student, Y. Sirak, V. Hvozdets’kyi, P. Maruchak, and H. Veselivska, “The properties of oxide-ceramic layers with Cu and Ni inclusions synthesizing by PEO method on top of the gas-spraying coatings on aluminum alloys,” Vacuum,179, 109–514 (2020). – reference: HusseinRONieXNorthwoodDOAn investigation of ceramic coating growth mechanisms in plasma-electrolytic oxidation (PEO) processingElectrochim. Acta20131121111191:CAS:528:DC%2BC3sXhvFSksbjK10.1016/j.electacta.2013.08.137 – reference: V. I. Chernenko, L. A. Snezhko, and I. I., Papanov, Application of Coatings by Anode-Arc Electrolysis [in Russian], Khimiya, Leningrad (1991), 127 pp. – reference: M. M. Student, V. M. Posuvailo, H. H. Veselivs’ka, Ya. Ya. Sirak, and R. А. Yatsyuk, “Corrosion resistance of plasma-electrolytic layers on alloys and coatings of the Al–Cu–Mg system for various modes of heat treatment,” Fiz.-Khim. Mekh. Mater.,53, No. 6, 42–47 (2017), English translation: Mater. Sci.,53, No. 6, 789–795 (2017). – reference: PosuvailoVMKulykVVDuriaginaZAStudentMMVasylivBDThe effect of electrolyte composition on the plasma electrolyte oxidation and phase composition of oxide ceramic coatings formed on 2024 aluminum alloyArch. Mat. Sci. Eng.202010524955 – reference: I. V. Suminov, P. M. Belkin, A. V. Èpel’fel’d, V. B. Lyudin, B. L. Krit, and A. M. Borisov, Plasma-Electrolytic Modification of the Surfaces of Metals and Alloys [in Russian], Vols. 1-2, , Vol. 2, Tekhnosfera, Moscow (2011). – reference: M. M. Student, V. M. Dovhunyk, V. M. Posuvailo, I. V. Koval’chuk, and V. M. Hvozdets’kyi, “Friction behavior of iron-carbon alloys in couples with plasma-electrolytic oxide-ceramic layers synthesized on D16T alloy,” Fiz.-Khim. Mekh. Mater.,53, No. 2, 63–70 (2017), English translation: Mater. Sci.,53, No. 2, 359–367 (2017). – reference: L. A. Snezhko, A. L. Erokhin, O. A. Kalinichenko, and D. O. Misnyankin, “Hydrogen release on the anode in the course of plasma electrolytic oxidation of aluminum,” Fiz.-Khim. Mekh. Mater.,52, No. 3, 111–119 (2016), English translation: Mater. Sci.,52, No. 3, 421–430 (2016). – reference: I. B. Ivasenko, V. M. Posuvailo, H. H. Veselivska, and V. Vynar, “Porosity segmentation and analysis of oxide ceramic coatings of D16T alloy,” in: Proc. of the IEEE 15th Internat. Sci. -Techn. Conf. on Computer Sciences and Information Technologies, CSIT 2020, Vol. 2 (2020), pp. 50–53. – reference: PokhmurskiiVKorniySKopyletsVThe theoretical study of interaction of water chloride containing environment components with CuAl2 intermetallic surfaceJ. of Cluster Sci.201021135431:CAS:528:DC%2BC3cXis1entLY%3D10.1007/s10876-010-0279-9 – reference: M. D. Klapkiv, O. S. Chuchmarev, P. Ya. Sydor, and V. M. Posuvailo, “Thermodynamics of the interaction of aluminum, magnesium, and zirconium with components of an electrolytic plasma,” Fiz.-Khim. Mekh. Mater.,36, No. 1, 56–64 (2000), English translation: Mater. Sci.,36, No. 1, 66–79 (2000). – reference: M. M. Student, H. H. Veselivska, O. S. Kalakhan, V. M. Hvozdetskyi, Kh. R. Zadorozhna, and Ya. Ya. Sirak, “Influence of the conditions of plasma-electrolytic treatment of D16T aluminum alloy on its corrosion resistance in 3% NaCl solution,” Fiz.-Khim. Mekh. Mater.,56, No. 4, 105–114 (2020), English translation: Mater. Sci.,56, No. 4, 550–559 (2021). – reference: BorisenkovaTAKaluzhinaSAAnodic behavior of aluminum in neutral electrolytes with different anionic compositionsKondens. Sredy Mezhph. Gran.20091121061091:CAS:528:DC%2BC3MXhtFyit7nM – reference: N. I. Blok, Qualitative Chemical Analysis [in Russian], GNTIKhL, Moscow-Leningrad (1952). – reference: M. D. Klapkiv, “Simulation of synthesis of oxide-ceramic coatings in discharge channels of a metal-electrolyte system,” Fiz.-Khim. Mekh. Mater.,35, No. 2, 111–114 (1999), English translation: Mater. Sci.,35, No. 2, 279–283 (1999). – reference: SnizhkoLOYerohinALPilkingtonAGurevinaNLMisnyankinaDOLeylandAMatthewsAAnodic processes in plasma electrolytic oxidation of aluminum in alkaline solutionsElectrochim. Acta200449208520951:CAS:528:DC%2BD2cXhs1Ckt7w%3D10.1016/j.electacta.2003.11.027 – reference: M. M. Student, I. B. Ivasenko, V. M. Posuvailo, Y. Y. Sirak, and V. M. Yus’kiv, “Influence of the porosity of a plasma-electrolytic coating on the corrosion resistance of D16 alloy,” Fiz.-Khim. Mekh. Mater.,54, No. 4, 130–137 (2018), English translation: Mater. Sci.,54, No. 6, 899–906 (2019). – ident: 540_CR3 doi: 10.1007/s11003-017-0083-x – ident: 540_CR9 doi: 10.1007/s11003-016-9974-5 – ident: 540_CR14 – ident: 540_CR13 – volume: 11 start-page: 106 issue: 2 year: 2009 ident: 540_CR15 publication-title: Kondens. Sredy Mezhph. Gran. – ident: 540_CR10 doi: 10.1007/978-3-030-63270-0_52 – ident: 540_CR8 doi: 10.1007/BF02805119 – ident: 540_CR12 doi: 10.1007/s11003-021-00463-z – ident: 540_CR7 doi: 10.1016/j.vacuum.2020.109514 – volume: 21 start-page: 35 issue: 1 year: 2010 ident: 540_CR16 publication-title: J. of Cluster Sci. doi: 10.1007/s10876-010-0279-9 – ident: 540_CR17 doi: 10.1007/s11003-019-00278-z – volume: 49 start-page: 2085 year: 2004 ident: 540_CR4 publication-title: Electrochim. Acta doi: 10.1016/j.electacta.2003.11.027 – ident: 540_CR1 – volume: 112 start-page: 111 year: 2013 ident: 540_CR6 publication-title: Electrochim. Acta doi: 10.1016/j.electacta.2013.08.137 – ident: 540_CR2 doi: 10.1007/s11003-018-0137-8 – ident: 540_CR5 doi: 10.1007/BF02359992 – volume: 105 start-page: 49 issue: 2 year: 2020 ident: 540_CR11 publication-title: Arch. Mat. Sci. Eng.
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SubjectTerms	Alloys Aluminum base alloys Analysis Aqueous solutions Ceramic coatings Ceramic glazes Ceramics Characterization and Evaluation of Materials Chemistry and Materials Science Copper Corrosion resistance Electrochemical impedance spectroscopy Magnesium Materials Materials Science Protective coatings Sodium chloride Solid Mechanics Specialty metals industry Structural Materials
Title	Corrosion Properties of Oxide Ceramic Coatings Based on Alloys of the Al–Cu–Mg and Al–Mg Systems
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