Design and fabrication of nitrogen-doped graphene-promoted Na3MnTi(PO4)3@C cathode with three-electron reactions for sodium-ion storage
As a novel cathode material for sodium-ion batteries, Na3MnTi(PO4)3 (denoted as NMTP) has received great attention because of its abundant natural resources, excellent safety, low toxicity as well as three-electron reactions. Unfortunately, the pure NMTP cathode displays a bad conductivity, resultin...
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| Vydáno v: | Solid state sciences Ročník 156; s. 107678 |
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| Hlavní autoři: | , , , , , , |
| Médium: | Journal Article |
| Jazyk: | angličtina |
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Elsevier Masson SAS
01.10.2024
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| ISSN: | 1293-2558 |
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| Abstract | As a novel cathode material for sodium-ion batteries, Na3MnTi(PO4)3 (denoted as NMTP) has received great attention because of its abundant natural resources, excellent safety, low toxicity as well as three-electron reactions. Unfortunately, the pure NMTP cathode displays a bad conductivity, resulting in an inferior electrochemical performance for sodium energy storage. Herein, we introduce a good route to fabricate the nitrogen-doped graphene-decorated NMTP@C (denoted as NG-NMTP@C) composite with superior rate property and superior cycle stability for the first time. In this fabricated material, the nitrogen-doped graphene nanosheets are dispersed into the NMTP@C particles. Compared to NMTP@C, the prepared NG-NMTP@C cathode possesses better cycle stability and higher capacity. It shows the capacity of 173.1 mAh g−1 at 0.1 C and presents the high capacity retention of around 97.1 % at 10.0 C over 400 cycles. Therefore, this fabricated NG-NMTP@C nanocomposite can be employed as the novel positive electrode in sodium-ion storage.
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•N-doped graphene-decorated Na3MnTi(PO4)3@C has been synthesized for the first time.•N-doped graphene can greatly enhance the conductivity of Na3MnTi(PO4)3@C.•The resulted cathode presents superior high-rate capability and cycling stability. |
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| AbstractList | As a novel cathode material for sodium-ion batteries, Na3MnTi(PO4)3 (denoted as NMTP) has received great attention because of its abundant natural resources, excellent safety, low toxicity as well as three-electron reactions. Unfortunately, the pure NMTP cathode displays a bad conductivity, resulting in an inferior electrochemical performance for sodium energy storage. Herein, we introduce a good route to fabricate the nitrogen-doped graphene-decorated NMTP@C (denoted as NG-NMTP@C) composite with superior rate property and superior cycle stability for the first time. In this fabricated material, the nitrogen-doped graphene nanosheets are dispersed into the NMTP@C particles. Compared to NMTP@C, the prepared NG-NMTP@C cathode possesses better cycle stability and higher capacity. It shows the capacity of 173.1 mAh g−1 at 0.1 C and presents the high capacity retention of around 97.1 % at 10.0 C over 400 cycles. Therefore, this fabricated NG-NMTP@C nanocomposite can be employed as the novel positive electrode in sodium-ion storage.
[Display omitted]
•N-doped graphene-decorated Na3MnTi(PO4)3@C has been synthesized for the first time.•N-doped graphene can greatly enhance the conductivity of Na3MnTi(PO4)3@C.•The resulted cathode presents superior high-rate capability and cycling stability. |
| ArticleNumber | 107678 |
| Author | Ma, Xiuhua Yan, Ruihan Xiao, Hua Luo, Peifang Wang, Tingyu Huang, Zan Zhao, Gengfeng |
| Author_xml | – sequence: 1 givenname: Peifang surname: Luo fullname: Luo, Peifang organization: Foundation Department, Guangzhou Maritime University, Guangzhou, Guangdong, 510725, PR China – sequence: 2 givenname: Zan orcidid: 0000-0002-8310-9321 surname: Huang fullname: Huang, Zan email: zhuanggz@aliyun.com organization: School of Naval Architecture and Ocean Engineering, Guangzhou Maritime University, Guangzhou, Guangdong, 510725, PR China – sequence: 3 givenname: Tingyu surname: Wang fullname: Wang, Tingyu organization: School of Naval Architecture and Ocean Engineering, Guangzhou Maritime University, Guangzhou, Guangdong, 510725, PR China – sequence: 4 givenname: Hua surname: Xiao fullname: Xiao, Hua organization: School of Naval Architecture and Ocean Engineering, Guangzhou Maritime University, Guangzhou, Guangdong, 510725, PR China – sequence: 5 givenname: Xiuhua surname: Ma fullname: Ma, Xiuhua organization: School of Naval Architecture and Ocean Engineering, Guangzhou Maritime University, Guangzhou, Guangdong, 510725, PR China – sequence: 6 givenname: Ruihan surname: Yan fullname: Yan, Ruihan organization: School of Naval Architecture and Ocean Engineering, Guangzhou Maritime University, Guangzhou, Guangdong, 510725, PR China – sequence: 7 givenname: Gengfeng surname: Zhao fullname: Zhao, Gengfeng organization: School of Naval Architecture and Ocean Engineering, Guangzhou Maritime University, Guangzhou, Guangdong, 510725, PR China |
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| Keywords | Battery performance Nitrogen-doped graphene Carbon coating NMTP Sodium-ion storage |
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| SubjectTerms | Battery performance Carbon coating Nitrogen-doped graphene NMTP Sodium-ion storage |
| Title | Design and fabrication of nitrogen-doped graphene-promoted Na3MnTi(PO4)3@C cathode with three-electron reactions for sodium-ion storage |
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