Theoretical study of the magnetic properties and the magnetocaloric effect in lanthanum manganite lacunar compounds
•The La1-xxMnO3 (x = 0.1 and 0.2) compounds was successfully prepared by sol-gel method.•The variation of (M) vs. (T) reveals a ferromagnetic to paramagnetic phase transition around TC.•A concordance with the experimental results is noted. Based on the Monte Carlo method and using the Ising model, t...
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| Vydáno v: | Journal of alloys and compounds Ročník 905; s. 164196 |
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| Hlavní autoři: | , , , , , |
| Médium: | Journal Article |
| Jazyk: | angličtina |
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Lausanne
Elsevier B.V
05.06.2022
Elsevier BV |
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| ISSN: | 0925-8388, 1873-4669 |
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| Abstract | •The La1-xxMnO3 (x = 0.1 and 0.2) compounds was successfully prepared by sol-gel method.•The variation of (M) vs. (T) reveals a ferromagnetic to paramagnetic phase transition around TC.•A concordance with the experimental results is noted.
Based on the Monte Carlo method and using the Ising model, the magnetic as well as the magnetocaloric properties of lacunar compounds La1-xxMnO3 (x = 0.1 and 0.2) were investigated. Free boundary conditions for our system were applied to simulate the 3D-Ising Hamiltonian of these systems. Cubic magnetic sublattices of size L3, with L = 20, 24 and 28, were investigated in this study to compute the magnetization and the magnetic susceptibility as a function of temperature (T) at various applied fields. In order to calculate the variation of the magnetic entropy versus the applied magnetic field, we have examined an isothermal process by considering a term of magneto-crystalline anisotropy. In order to validate the results, many parameters were calculated. The results obtained are in good agreement with the experimental ones. The high relative cooling power values of our compounds leads to promising material for magnetic refrigeration technology. This material could be considered as a good candidate for applications requiring high values of TC. |
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| AbstractList | Based on the Monte Carlo method and using the Ising model, the magnetic as well as the magnetocaloric properties of lacunar compounds La1-xxMnO3 (x = 0.1 and 0.2) were investigated. Free boundary conditions for our system were applied to simulate the 3D-Ising Hamiltonian of these systems. Cubic magnetic sublattices of size L3, with L = 20, 24 and 28, were investigated in this study to compute the magnetization and the magnetic susceptibility as a function of temperature (T) at various applied fields. In order to calculate the variation of the magnetic entropy versus the applied magnetic field, we have examined an isothermal process by considering a term of magneto-crystalline anisotropy. In order to validate the results, many parameters were calculated. The results obtained are in good agreement with the experimental ones. The high relative cooling power values of our compounds leads to promising material for magnetic refrigeration technology. This material could be considered as a good candidate for applications requiring high values of TC. •The La1-xxMnO3 (x = 0.1 and 0.2) compounds was successfully prepared by sol-gel method.•The variation of (M) vs. (T) reveals a ferromagnetic to paramagnetic phase transition around TC.•A concordance with the experimental results is noted. Based on the Monte Carlo method and using the Ising model, the magnetic as well as the magnetocaloric properties of lacunar compounds La1-xxMnO3 (x = 0.1 and 0.2) were investigated. Free boundary conditions for our system were applied to simulate the 3D-Ising Hamiltonian of these systems. Cubic magnetic sublattices of size L3, with L = 20, 24 and 28, were investigated in this study to compute the magnetization and the magnetic susceptibility as a function of temperature (T) at various applied fields. In order to calculate the variation of the magnetic entropy versus the applied magnetic field, we have examined an isothermal process by considering a term of magneto-crystalline anisotropy. In order to validate the results, many parameters were calculated. The results obtained are in good agreement with the experimental ones. The high relative cooling power values of our compounds leads to promising material for magnetic refrigeration technology. This material could be considered as a good candidate for applications requiring high values of TC. |
| ArticleNumber | 164196 |
| Author | Omari, L.H. Benali, A. Mnasri, T. Dhahri, E. Henchiri, C. Valente, M.A. |
| Author_xml | – sequence: 1 givenname: C. surname: Henchiri fullname: Henchiri, C. email: chadha.henchiri@gmail.com organization: Laboratoire de Physique Appliquée, Faculté des Sciences de Sfax, B.P. 802, Université de Sfax, 3018, Tunisia – sequence: 2 givenname: L.H. surname: Omari fullname: Omari, L.H. organization: LPMAT, Faculty of Sciences Ain Chock, Hassan II University, B.P 5366 Maârif Casablanca, Morocco – sequence: 3 givenname: T. surname: Mnasri fullname: Mnasri, T. organization: Laboratory TEMI, Faculty of Science; University of Gafsa, 2112, Tunisia – sequence: 4 givenname: A. surname: Benali fullname: Benali, A. organization: Laboratoire de Physique Appliquée, Faculté des Sciences de Sfax, B.P. 802, Université de Sfax, 3018, Tunisia – sequence: 5 givenname: E. surname: Dhahri fullname: Dhahri, E. organization: Laboratoire de Physique Appliquée, Faculté des Sciences de Sfax, B.P. 802, Université de Sfax, 3018, Tunisia – sequence: 6 givenname: M.A. surname: Valente fullname: Valente, M.A. organization: I3N, Physics Department, University of Aveiro, 3810-193 Aveiro, Portugal |
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| Keywords | Crystallographic structure Magnetocaloric effect Ferromagnetic/antiferromagnetic Lacunar perovskite compound Computation/computing Magnetic properties |
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| Snippet | •The La1-xxMnO3 (x = 0.1 and 0.2) compounds was successfully prepared by sol-gel method.•The variation of (M) vs. (T) reveals a ferromagnetic to paramagnetic... Based on the Monte Carlo method and using the Ising model, the magnetic as well as the magnetocaloric properties of lacunar compounds La1-xxMnO3 (x = 0.1 and... |
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| SubjectTerms | Anisotropy Boundary conditions Computation/computing Crystallographic structure Ferromagnetic/antiferromagnetic Free boundaries Ising model Lacunar perovskite compound Lanthanum Lanthanum compounds Magnetic permeability Magnetic properties Magnetism Magnetocaloric effect Monte Carlo simulation |
| Title | Theoretical study of the magnetic properties and the magnetocaloric effect in lanthanum manganite lacunar compounds |
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