Electrochemical quinuclidine-mediated Minisci-type acylation of N-heterocycles with aldehydes
The electro-generation of acyl radicals from both aromatic and aliphatic aldehydes remains an unmet challenge. We provide a solution to this challenge by merging electro-oxidation and a quinuclidine-mediated hydrogen atom transfer strategy. The generation of acyl radicals at decreased applied potent...
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| Vydané v: | Chemical communications (Cambridge, England) Ročník 60; číslo 48; s. 6174 - 6177 |
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| Jazyk: | English |
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Royal Soc Chemistry
11.06.2024
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| Abstract | The electro-generation of acyl radicals from both aromatic and aliphatic aldehydes remains an unmet challenge. We provide a solution to this challenge by merging electro-oxidation and a quinuclidine-mediated hydrogen atom transfer strategy. The generation of acyl radicals at decreased applied potentials compared to that of formyl oxidation exhibits excellent functional group compatibility.
The electro-generation of acyl radicals from both aromatic and aliphatic aldehydes is a synthetic challenge. We addressed this challenge by merging electro-oxidation and a quinuclidine-mediated HAT strategy. |
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| AbstractList | The electro-generation of acyl radicals from both aromatic and aliphatic aldehydes remains an unmet challenge. We provide a solution to this challenge by merging electro-oxidation and a quinuclidine-mediated hydrogen atom transfer strategy. The generation of acyl radicals at decreased applied potentials compared to that of formyl oxidation exhibits excellent functional group compatibility.The electro-generation of acyl radicals from both aromatic and aliphatic aldehydes remains an unmet challenge. We provide a solution to this challenge by merging electro-oxidation and a quinuclidine-mediated hydrogen atom transfer strategy. The generation of acyl radicals at decreased applied potentials compared to that of formyl oxidation exhibits excellent functional group compatibility. The electro-generation of acyl radicals from both aromatic and aliphatic aldehydes remains an unmet challenge. We provide a solution to this challenge by merging electro-oxidation and a quinuclidine-mediated hydrogen atom transfer strategy. The generation of acyl radicals at decreased applied potentials compared to that of formyl oxidation exhibits excellent functional group compatibility. The electro-generation of acyl radicals from both aromatic and aliphatic aldehydes remains an unmet challenge. We provide a solution to this challenge by merging electro-oxidation and a quinuclidine-mediated hydrogen atom transfer strategy. The generation of acyl radicals at decreased applied potentials compared to that of formyl oxidation exhibits excellent functional group compatibility. The electro-generation of acyl radicals from both aromatic and aliphatic aldehydes is a synthetic challenge. We addressed this challenge by merging electro-oxidation and a quinuclidine-mediated HAT strategy. |
| Author | Li, Yongmei Zeng, Cheng-Chu Huang, Shengyang Xu, Kun Sun, Liangbo |
| Author_xml | – sequence: 1 givenname: Yongmei surname: Li fullname: Li, Yongmei organization: Beijing Univ Technol, Coll Chem & Life Sci, Beijing 100124, Peoples R China – sequence: 2 givenname: Liangbo surname: Sun fullname: Sun, Liangbo organization: Beijing Univ Technol, Coll Chem & Life Sci, Beijing 100124, Peoples R China – sequence: 3 givenname: Shengyang surname: Huang fullname: Huang, Shengyang organization: Beijing Univ Technol, Coll Chem & Life Sci, Beijing 100124, Peoples R China – sequence: 4 givenname: Kun orcidid: 0000-0002-0419-8822 surname: Xu fullname: Xu, Kun email: kunxu@bjut.edu.cn organization: Beijing Univ Technol, Coll Chem & Life Sci, Beijing 100124, Peoples R China – sequence: 5 givenname: Cheng-Chu orcidid: 0000-0002-5659-291X surname: Zeng fullname: Zeng, Cheng-Chu email: zengcc@bjut.edu.cn organization: Beijing Univ Technol, Coll Chem & Life Sci, Beijing 100124, Peoples R China |
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