A highly sensitive and selective fluorescent chemosensor for the sequential recognition of Zn2+ and S2− in living cells and aqueous media
A new highly selective chemosensor 1 (E)-5-((2-hydroxybenzylidene)amino)-1H-imidazole-4-carboxamide was designed and synthesized for the sequential recognition of Zn2+ and S2− in a near-perfect aqueous media. The sensor 1 exhibited a green color fluorescence in the presence of Zn2+. The detection li...
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| Veröffentlicht in: | Sensors and actuators. B, Chemical Jg. 255; S. 3108 - 3116 |
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| Format: | Journal Article |
| Sprache: | Englisch |
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Elsevier B.V
01.02.2018
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| ISSN: | 0925-4005, 1873-3077 |
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| Abstract | A new highly selective chemosensor 1 (E)-5-((2-hydroxybenzylidene)amino)-1H-imidazole-4-carboxamide was designed and synthesized for the sequential recognition of Zn2+ and S2− in a near-perfect aqueous media. The sensor 1 exhibited a green color fluorescence in the presence of Zn2+. The detection limit (1.18μM) of 1 for Zn2+ is much lower than World Health Organization guideline (76μM) in drinking water. 1 can detect and quantify Zn2+ in real water samples and the sensing mechanism of Zn2+ by 1 was explained by DFT calculations. Moreover, resulting 1-Zn2+ complex can detect hydrogen sulfide through turn-off fluorescent change, without any anion interference. The detection limit (2.60μM) of 1-Zn2+ complex for S2− was much lower than EPA guideline (7.8mM) by odor in drinking water. Furthermore, sensor 1 could detect sequentially Zn2+ and S2− in living cells. |
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| AbstractList | A new highly selective chemosensor 1 (E)-5-((2-hydroxybenzylidene)amino)-1H-imidazole-4-carboxamide was designed and synthesized for the sequential recognition of Zn2+ and S2− in a near-perfect aqueous media. The sensor 1 exhibited a green color fluorescence in the presence of Zn2+. The detection limit (1.18μM) of 1 for Zn2+ is much lower than World Health Organization guideline (76μM) in drinking water. 1 can detect and quantify Zn2+ in real water samples and the sensing mechanism of Zn2+ by 1 was explained by DFT calculations. Moreover, resulting 1-Zn2+ complex can detect hydrogen sulfide through turn-off fluorescent change, without any anion interference. The detection limit (2.60μM) of 1-Zn2+ complex for S2− was much lower than EPA guideline (7.8mM) by odor in drinking water. Furthermore, sensor 1 could detect sequentially Zn2+ and S2− in living cells. |
| Author | Kim, Cheal Jang, Hyo Jung Han, Jiyeon Yun, Jin Yeong Jo, Tae Geun Lim, Mi Hee |
| Author_xml | – sequence: 1 givenname: Jin Yeong surname: Yun fullname: Yun, Jin Yeong organization: Department of Fine Chemistry and Department of Interdisciplinary Bio IT Materials, Seoul National University of Science and Technology, Seoul 139-743, Republic of Korea – sequence: 2 givenname: Tae Geun surname: Jo fullname: Jo, Tae Geun organization: Department of Fine Chemistry and Department of Interdisciplinary Bio IT Materials, Seoul National University of Science and Technology, Seoul 139-743, Republic of Korea – sequence: 3 givenname: Jiyeon surname: Han fullname: Han, Jiyeon organization: Department of Chemistry, Ulsan National Institute of Science and Technology (UNIST), Ulsan 44919, Republic of Korea – sequence: 4 givenname: Hyo Jung surname: Jang fullname: Jang, Hyo Jung organization: Department of Fine Chemistry and Department of Interdisciplinary Bio IT Materials, Seoul National University of Science and Technology, Seoul 139-743, Republic of Korea – sequence: 5 givenname: Mi Hee surname: Lim fullname: Lim, Mi Hee organization: Department of Chemistry, Ulsan National Institute of Science and Technology (UNIST), Ulsan 44919, Republic of Korea – sequence: 6 givenname: Cheal surname: Kim fullname: Kim, Cheal email: chealkim@seoultech.ac.kr organization: Department of Fine Chemistry and Department of Interdisciplinary Bio IT Materials, Seoul National University of Science and Technology, Seoul 139-743, Republic of Korea |
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| Title | A highly sensitive and selective fluorescent chemosensor for the sequential recognition of Zn2+ and S2− in living cells and aqueous media |
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