Effect of temperature variation on the corrosion behaviour and semiconducting properties of the passive film formed on chromium oxide coatings exposed to saline solution
•RF sputtered chromium oxide coatings were tested in saline solution at a temperature range 25 to 65° C.•The prepared coatings were confirmed to be mainly chromium (III) oxide.•The passive oxide layers on the coatings possess p-type semiconductor property.•The acceptor defect densities and corrosion...
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| Published in: | Corrosion science Vol. 154; pp. 28 - 35 |
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| Main Authors: | , , , , |
| Format: | Journal Article |
| Language: | English |
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Amsterdam
Elsevier Ltd
01.07.2019
Elsevier BV |
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| ISSN: | 0010-938X, 1879-0496 |
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| Abstract | •RF sputtered chromium oxide coatings were tested in saline solution at a temperature range 25 to 65° C.•The prepared coatings were confirmed to be mainly chromium (III) oxide.•The passive oxide layers on the coatings possess p-type semiconductor property.•The acceptor defect densities and corrosion of the coatings were found to be temperature dependent.•Coatings tested at lower temperatures showed superior pitting corrosion resistance compared to those tested at higher temperatures.
The corrosion behaviour of chromium oxide coatings and semiconducting properties of the passive film formed on the surface of the coated samples when exposed to saline solution at a temperature range 25 °C–65 °C was investigated. The cyclic polarisation results revealed that the coatings tested at a electrolyte temperature range 25 °C–35 °C possess superior resistance to pitting corrosion when compared to coatings tested at higher temperatures. Our Mott-Schottky analysis suggests that this variation in corrosion resistance can be linked to the increase in the amount of the defect density present in the films and enhanced diffusion at higher temperatures. |
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| AbstractList | •RF sputtered chromium oxide coatings were tested in saline solution at a temperature range 25 to 65° C.•The prepared coatings were confirmed to be mainly chromium (III) oxide.•The passive oxide layers on the coatings possess p-type semiconductor property.•The acceptor defect densities and corrosion of the coatings were found to be temperature dependent.•Coatings tested at lower temperatures showed superior pitting corrosion resistance compared to those tested at higher temperatures.
The corrosion behaviour of chromium oxide coatings and semiconducting properties of the passive film formed on the surface of the coated samples when exposed to saline solution at a temperature range 25 °C–65 °C was investigated. The cyclic polarisation results revealed that the coatings tested at a electrolyte temperature range 25 °C–35 °C possess superior resistance to pitting corrosion when compared to coatings tested at higher temperatures. Our Mott-Schottky analysis suggests that this variation in corrosion resistance can be linked to the increase in the amount of the defect density present in the films and enhanced diffusion at higher temperatures. The corrosion behaviour of chromium oxide coatings and semiconducting properties of the passive film formed on the surface of the coated samples when exposed to saline solution at a temperature range 25 °C–65 °C was investigated. The cyclic polarisation results revealed that the coatings tested at a electrolyte temperature range 25 °C–35 °C possess superior resistance to pitting corrosion when compared to coatings tested at higher temperatures. Our Mott-Schottky analysis suggests that this variation in corrosion resistance can be linked to the increase in the amount of the defect density present in the films and enhanced diffusion at higher temperatures. |
| Author | Rahman, S.Ur Ogwu, A.A. Oje, A.M. Oje, Alex.I. Tsendzughul, Nathaniel |
| Author_xml | – sequence: 1 givenname: A.M. surname: Oje fullname: Oje, A.M. email: Michael.oje@uws.ac.uk organization: School of Engineering and Computing, University of the West of Scotland, High Street, Paisley, PA1 2BE, Scotland, UK – sequence: 2 givenname: A.A. surname: Ogwu fullname: Ogwu, A.A. organization: East Kazakhstan State Technical University, Ust-Kamenogorsk, Republic of Kazakhstan – sequence: 3 givenname: S.Ur surname: Rahman fullname: Rahman, S.Ur organization: School of Engineering and Computing, University of the West of Scotland, High Street, Paisley, PA1 2BE, Scotland, UK – sequence: 4 givenname: Alex.I. surname: Oje fullname: Oje, Alex.I. organization: School of Engineering and Computing, University of the West of Scotland, High Street, Paisley, PA1 2BE, Scotland, UK – sequence: 5 givenname: Nathaniel surname: Tsendzughul fullname: Tsendzughul, Nathaniel organization: School of Engineering and Computing, University of the West of Scotland, High Street, Paisley, PA1 2BE, Scotland, UK |
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| Keywords | Elevated temperatures Semiconducting properties Corrosion Saline solution Chromium oxide coatings |
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| Snippet | •RF sputtered chromium oxide coatings were tested in saline solution at a temperature range 25 to 65° C.•The prepared coatings were confirmed to be mainly... The corrosion behaviour of chromium oxide coatings and semiconducting properties of the passive film formed on the surface of the coated samples when exposed... |
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| SubjectTerms | Chromium oxide coatings Chromium oxides Corrosion Corrosion effects Corrosion resistance Elevated temperatures Enhanced diffusion Oxide coatings Pitting (corrosion) Protective coatings Saline solution Saline solutions Semiconducting properties Temperature Temperature effects |
| Title | Effect of temperature variation on the corrosion behaviour and semiconducting properties of the passive film formed on chromium oxide coatings exposed to saline solution |
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