The ultramicropore biochar derived from waste distiller’s grains for wet-process phosphoric acid purification: Removal performance and mechanisms of Cr(VI)
Solid waste and heavy metal pollution are long-term and challenging subjects in the field of environmental engineering. In this study, we propose a sustainable approach to “treating waste with waste” by utilizing the ultramicropore biochar derived from solid waste distiller’s grains as a means to re...
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| Vydáno v: | Chemosphere (Oxford) Ročník 349; s. 140877 |
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| Hlavní autoři: | , , , , , , |
| Médium: | Journal Article |
| Jazyk: | angličtina |
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England
Elsevier Ltd
01.02.2024
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| ISSN: | 0045-6535, 1879-1298, 1879-1298 |
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| Abstract | Solid waste and heavy metal pollution are long-term and challenging subjects in the field of environmental engineering. In this study, we propose a sustainable approach to “treating waste with waste” by utilizing the ultramicropore biochar derived from solid waste distiller’s grains as a means to remove Cr(VI) from simulated wastewater and wet phosphoric acid. The biochar prepared in this research exhibit extremely high specific surface areas (up to 2973 m2/g) and a well-developed pore structure, resulting in a maximum Cr(VI) adsorption capacity of 426.0 mg/g and over 99% removal efficiency of Cr(VI). Furthermore, the adsorbent can be reused for up to eight cycles without significant reduction in its Cr(VI) adsorption performance. Mechanistic investigations suggest that the exceptional Cr(VI) adsorption capacity can be attributed to the synergistic effect of electrostatic interaction and reduction adsorption. This study offers an alternative approach for the resource utilization of solid waste distiller’s grains, and the prepared biochar holds promise for the removal of Cr(VI) from wastewater and wet-process phosphoric acid.
[Display omitted]
•Biochar derived from distiller’s grains is used for removal Cr(VI).•Biochar exhibits a remarkably high specific surface area.•A maximum adsorption capacity for Cr(VI) of 426.0 mg/g is acquired.•A combined physical and chemical interaction for Cr(VI) removal is proposed. |
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| AbstractList | Solid waste and heavy metal pollution are long-term and challenging subjects in the field of environmental engineering. In this study, we propose a sustainable approach to "treating waste with waste" by utilizing the ultramicropore biochar derived from solid waste distiller's grains as a means to remove Cr(VI) from simulated wastewater and wet phosphoric acid. The biochar prepared in this research exhibit extremely high specific surface areas (up to 2973 m2/g) and a well-developed pore structure, resulting in a maximum Cr(VI) adsorption capacity of 426.0 mg/g and over 99% removal efficiency of Cr(VI). Furthermore, the adsorbent can be reused for up to eight cycles without significant reduction in its Cr(VI) adsorption performance. Mechanistic investigations suggest that the exceptional Cr(VI) adsorption capacity can be attributed to the synergistic effect of electrostatic interaction and reduction adsorption. This study offers an alternative approach for the resource utilization of solid waste distiller's grains, and the prepared biochar holds promise for the removal of Cr(VI) from wastewater and wet-process phosphoric acid.Solid waste and heavy metal pollution are long-term and challenging subjects in the field of environmental engineering. In this study, we propose a sustainable approach to "treating waste with waste" by utilizing the ultramicropore biochar derived from solid waste distiller's grains as a means to remove Cr(VI) from simulated wastewater and wet phosphoric acid. The biochar prepared in this research exhibit extremely high specific surface areas (up to 2973 m2/g) and a well-developed pore structure, resulting in a maximum Cr(VI) adsorption capacity of 426.0 mg/g and over 99% removal efficiency of Cr(VI). Furthermore, the adsorbent can be reused for up to eight cycles without significant reduction in its Cr(VI) adsorption performance. Mechanistic investigations suggest that the exceptional Cr(VI) adsorption capacity can be attributed to the synergistic effect of electrostatic interaction and reduction adsorption. This study offers an alternative approach for the resource utilization of solid waste distiller's grains, and the prepared biochar holds promise for the removal of Cr(VI) from wastewater and wet-process phosphoric acid. Solid waste and heavy metal pollution are long-term and challenging subjects in the field of environmental engineering. In this study, we propose a sustainable approach to “treating waste with waste” by utilizing the ultramicropore biochar derived from solid waste distiller’s grains as a means to remove Cr(VI) from simulated wastewater and wet phosphoric acid. The biochar prepared in this research exhibit extremely high specific surface areas (up to 2973 m2/g) and a well-developed pore structure, resulting in a maximum Cr(VI) adsorption capacity of 426.0 mg/g and over 99% removal efficiency of Cr(VI). Furthermore, the adsorbent can be reused for up to eight cycles without significant reduction in its Cr(VI) adsorption performance. Mechanistic investigations suggest that the exceptional Cr(VI) adsorption capacity can be attributed to the synergistic effect of electrostatic interaction and reduction adsorption. This study offers an alternative approach for the resource utilization of solid waste distiller’s grains, and the prepared biochar holds promise for the removal of Cr(VI) from wastewater and wet-process phosphoric acid. [Display omitted] •Biochar derived from distiller’s grains is used for removal Cr(VI).•Biochar exhibits a remarkably high specific surface area.•A maximum adsorption capacity for Cr(VI) of 426.0 mg/g is acquired.•A combined physical and chemical interaction for Cr(VI) removal is proposed. Solid waste and heavy metal pollution are long-term and challenging subjects in the field of environmental engineering. In this study, we propose a sustainable approach to “treating waste with waste” by utilizing the ultramicropore biochar derived from solid waste distiller’s grains as a means to remove Cr(VI) from simulated wastewater and wet phosphoric acid. The biochar prepared in this research exhibit extremely high specific surface areas (up to 2973 m²/g) and a well-developed pore structure, resulting in a maximum Cr(VI) adsorption capacity of 426.0 mg/g and over 99% removal efficiency of Cr(VI). Furthermore, the adsorbent can be reused for up to eight cycles without significant reduction in its Cr(VI) adsorption performance. Mechanistic investigations suggest that the exceptional Cr(VI) adsorption capacity can be attributed to the synergistic effect of electrostatic interaction and reduction adsorption. This study offers an alternative approach for the resource utilization of solid waste distiller’s grains, and the prepared biochar holds promise for the removal of Cr(VI) from wastewater and wet-process phosphoric acid. Solid waste and heavy metal pollution are long-term and challenging subjects in the field of environmental engineering. In this study, we propose a sustainable approach to "treating waste with waste" by utilizing the ultramicropore biochar derived from solid waste distiller's grains as a means to remove Cr(VI) from simulated wastewater and wet phosphoric acid. The biochar prepared in this research exhibit extremely high specific surface areas (up to 2973 m /g) and a well-developed pore structure, resulting in a maximum Cr(VI) adsorption capacity of 426.0 mg/g and over 99% removal efficiency of Cr(VI). Furthermore, the adsorbent can be reused for up to eight cycles without significant reduction in its Cr(VI) adsorption performance. Mechanistic investigations suggest that the exceptional Cr(VI) adsorption capacity can be attributed to the synergistic effect of electrostatic interaction and reduction adsorption. This study offers an alternative approach for the resource utilization of solid waste distiller's grains, and the prepared biochar holds promise for the removal of Cr(VI) from wastewater and wet-process phosphoric acid. |
| ArticleNumber | 140877 |
| Author | Lin, Qian Hu, Guotao Zhao, Tianxiang Pan, Hongyan Su, Kai Dong, Huinan Yang, Yi |
| Author_xml | – sequence: 1 givenname: Kai surname: Su fullname: Su, Kai organization: Key Laboratory of Green Chemical and Clean Energy Technology, Engineering Research Center of Efficient Utilization for Industrial Waste, School of Chemistry and Chemical Engineering, Guizhou University, Guiyang, 550025, PR China – sequence: 2 givenname: Guotao surname: Hu fullname: Hu, Guotao organization: Guizhou Wengfu (Group) Co., Ltd., Guiyang, 550025, PR China – sequence: 3 givenname: Tianxiang surname: Zhao fullname: Zhao, Tianxiang email: txzhao3@gzu.edu.cn organization: Key Laboratory of Green Chemical and Clean Energy Technology, Engineering Research Center of Efficient Utilization for Industrial Waste, School of Chemistry and Chemical Engineering, Guizhou University, Guiyang, 550025, PR China – sequence: 4 givenname: Huinan surname: Dong fullname: Dong, Huinan organization: Key Laboratory of Green Chemical and Clean Energy Technology, Engineering Research Center of Efficient Utilization for Industrial Waste, School of Chemistry and Chemical Engineering, Guizhou University, Guiyang, 550025, PR China – sequence: 5 givenname: Yi surname: Yang fullname: Yang, Yi organization: Guizhou Wengfu (Group) Co., Ltd., Guiyang, 550025, PR China – sequence: 6 givenname: Hongyan surname: Pan fullname: Pan, Hongyan email: cepanhongyan@163.com organization: Key Laboratory of Green Chemical and Clean Energy Technology, Engineering Research Center of Efficient Utilization for Industrial Waste, School of Chemistry and Chemical Engineering, Guizhou University, Guiyang, 550025, PR China – sequence: 7 givenname: Qian surname: Lin fullname: Lin, Qian email: celinqianphy@163.com organization: Key Laboratory of Green Chemical and Clean Energy Technology, Engineering Research Center of Efficient Utilization for Industrial Waste, School of Chemistry and Chemical Engineering, Guizhou University, Guiyang, 550025, PR China |
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| Keywords | Phosphoric acid purification Cr(VI) adsorption Biochar Distiller’s grains Wet-process phosphoric acid |
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| SubjectTerms | adsorbents adsorption Biochar Cr(VI) adsorption Distiller’s grains electrostatic interactions heavy metals phosphoric acid Phosphoric acid purification pollution solid wastes synergism wastewater Wet-process phosphoric acid |
| Title | The ultramicropore biochar derived from waste distiller’s grains for wet-process phosphoric acid purification: Removal performance and mechanisms of Cr(VI) |
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