CMAS corrosion characteristics of YSZ and Al2O3-YSZ thermal barrier coatings at 1250 °C–1350 °C
The calcium-magnesium-aluminum-silicate (CMAS) corrosion is now a great threat to thermal barrier coatings (TBCs), inducing coating spallation readily. The CMAS corrosion characteristics of both 7YSZ and 20 wt.%Al2O3-YSZ TBCs at a broad temperature range of 1250 °C to 1350 °C were investigated. 7YSZ...
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| Vydáno v: | Journal of the European Ceramic Society Ročník 44; číslo 15; s. 116789 |
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| Jazyk: | angličtina |
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Elsevier Ltd
01.12.2024
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| ISSN: | 0955-2219 |
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| Abstract | The calcium-magnesium-aluminum-silicate (CMAS) corrosion is now a great threat to thermal barrier coatings (TBCs), inducing coating spallation readily. The CMAS corrosion characteristics of both 7YSZ and 20 wt.%Al2O3-YSZ TBCs at a broad temperature range of 1250 °C to 1350 °C were investigated. 7YSZ coatings were completely degraded by CMAS at 1250 °C while the increased corrosion temperatures induced more serious destruction. This is due to that the viscosity of CMAS melt significantly decreased with corrosion temperature increasing, promoting melt fluidity and infiltration. The Al2O3-YSZ composite TBCs demonstrated superior resistance to CMAS corrosion at 1250°C-1350 °C. The intensive chemical reactions between Al2O3 and CMAS melt promoted the formation of anorthite products with either short rod-shaped or blocky morphologies. These products closely interconnected and stacked up to generate a dense layer, physically blocking CMAS melt infiltration and effectively improving the anti-CMAS corrosion properties of TBCs at higher temperatures. Furthermore, the corrosion temperatures critically influenced anorthite formation and present morphologies. |
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| AbstractList | The calcium-magnesium-aluminum-silicate (CMAS) corrosion is now a great threat to thermal barrier coatings (TBCs), inducing coating spallation readily. The CMAS corrosion characteristics of both 7YSZ and 20 wt.%Al2O3-YSZ TBCs at a broad temperature range of 1250 °C to 1350 °C were investigated. 7YSZ coatings were completely degraded by CMAS at 1250 °C while the increased corrosion temperatures induced more serious destruction. This is due to that the viscosity of CMAS melt significantly decreased with corrosion temperature increasing, promoting melt fluidity and infiltration. The Al2O3-YSZ composite TBCs demonstrated superior resistance to CMAS corrosion at 1250°C-1350 °C. The intensive chemical reactions between Al2O3 and CMAS melt promoted the formation of anorthite products with either short rod-shaped or blocky morphologies. These products closely interconnected and stacked up to generate a dense layer, physically blocking CMAS melt infiltration and effectively improving the anti-CMAS corrosion properties of TBCs at higher temperatures. Furthermore, the corrosion temperatures critically influenced anorthite formation and present morphologies. |
| ArticleNumber | 116789 |
| Author | Han, Jiasen Gao, Wei Wu, Dongting Zhang, Yongang Dou, Mengfan Xue, Ting Zou, Yong |
| Author_xml | – sequence: 1 givenname: Mengfan surname: Dou fullname: Dou, Mengfan organization: Key Laboratory for Liquid-Solid Structural Evolution and Processing of Materials, Ministry of Education, School of Materials Science and Engineering, Shandong University, Jinan 250061, China – sequence: 2 givenname: Wei surname: Gao fullname: Gao, Wei organization: Key Laboratory for Liquid-Solid Structural Evolution and Processing of Materials, Ministry of Education, School of Materials Science and Engineering, Shandong University, Jinan 250061, China – sequence: 3 givenname: Ting surname: Xue fullname: Xue, Ting organization: Key Laboratory for Liquid-Solid Structural Evolution and Processing of Materials, Ministry of Education, School of Materials Science and Engineering, Shandong University, Jinan 250061, China – sequence: 4 givenname: Jiasen surname: Han fullname: Han, Jiasen organization: State Key Laboratory of Solidification Processing, Northwestern Polytechnical University, Xi'an 710072, China – sequence: 5 givenname: Dongting surname: Wu fullname: Wu, Dongting organization: Key Laboratory for Liquid-Solid Structural Evolution and Processing of Materials, Ministry of Education, School of Materials Science and Engineering, Shandong University, Jinan 250061, China – sequence: 6 givenname: Yong surname: Zou fullname: Zou, Yong organization: Key Laboratory for Liquid-Solid Structural Evolution and Processing of Materials, Ministry of Education, School of Materials Science and Engineering, Shandong University, Jinan 250061, China – sequence: 7 givenname: Yongang surname: Zhang fullname: Zhang, Yongang email: yongang.zhang@sdu.edu.cn organization: Key Laboratory for Liquid-Solid Structural Evolution and Processing of Materials, Ministry of Education, School of Materials Science and Engineering, Shandong University, Jinan 250061, China |
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| Keywords | CMAS corrosion Al2O3-7YSZ composite coating Thermal barrier coating Interfacial reactions |
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