Performance comparison of thin-film nanocomposite polyamide nanofiltration membranes for heavy metal/salt wastewater treatment

For the treatment of wastewater and water resources, membrane technologies are rapidly developing. Also, water pollution by heavy metals, dyes, oil, medicinal, and salts leads to lower water quality and water shortages. In this research, thin-film nanocomposite nanofiltration (TFN) membranes were pr...

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Veröffentlicht in:	Journal of nanoparticle research : an interdisciplinary forum for nanoscale science and technology Jg. 25; H. 4; S. 77
Hauptverfasser:	Fouladi, Mona, Kavousi Heidari, Maryam, Tavakoli, Omid
Format:	Journal Article
Sprache:	Englisch
Veröffentlicht:	Dordrecht Springer Netherlands 01.04.2023 Springer Nature B.V
Schlagworte:	Aluminum Characterization and Evaluation of Materials Chemistry and Materials Science Contact angle Graphene Heavy metals Hydrophilicity Inorganic Chemistry Lasers Materials Science Membranes Metal-organic frameworks Monomers Nanocomposites Nanofiltration Nanoparticles Nanostructure Nanotechnology NMR Nuclear magnetic resonance Oil pollution Optical Devices Optics Phenylenediamine Photonics Physical Chemistry Polyamide resins Polyamides Rejection Research Paper Sodium sulfate Thin films Wastewater treatment Water pollution Water quality Water resources Water shortages Zeta potential Interfacial polymerization Metal-organic framework Hydrophilicity Graphene oxide nanosheet Wastewater Thin-film nanocomposite membrane
ISSN:	1388-0764, 1572-896X
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Abstract	For the treatment of wastewater and water resources, membrane technologies are rapidly developing. Also, water pollution by heavy metals, dyes, oil, medicinal, and salts leads to lower water quality and water shortages. In this research, thin-film nanocomposite nanofiltration (TFN) membranes were produced via the interfacial polymerization (IP) method between trimesoyl chloride (TMC) and m-phenylenediamine (MPD) monomers at the top surface of PES/(UF) membrane and modified by graphene oxide (GO) and aluminum fumarate (AlFu) metal-organic framework (MOF) nanostructures to remove heavy metal and (divalent and monovalent) salts. The FTIR, NMR, SEM, XRD, and zeta potential analyses investigated the modified thin-film nanocomposite membrane properties. Also, the hydrophilicity of the membrane was determined via contact angle analysis. Compared to the polyamide (PA) and PA/AlFu membranes, the as-synthesized TFN membrane contains 0.3 wt% GO had the highest water flux, 110.86 l/m 2 ·h, rejection of Na 2 SO 4 salt and Cr 2+ about 98.94% and 97.5%, respectively. Generally, using nanostructures like GO and AlFu (MOF) opens a novel path to improve hydrophilicity, negative charge, water flux, and rejection of polyamide nanocomposite membrane. Graphical Abstract
AbstractList	For the treatment of wastewater and water resources, membrane technologies are rapidly developing. Also, water pollution by heavy metals, dyes, oil, medicinal, and salts leads to lower water quality and water shortages. In this research, thin-film nanocomposite nanofiltration (TFN) membranes were produced via the interfacial polymerization (IP) method between trimesoyl chloride (TMC) and m-phenylenediamine (MPD) monomers at the top surface of PES/(UF) membrane and modified by graphene oxide (GO) and aluminum fumarate (AlFu) metal-organic framework (MOF) nanostructures to remove heavy metal and (divalent and monovalent) salts. The FTIR, NMR, SEM, XRD, and zeta potential analyses investigated the modified thin-film nanocomposite membrane properties. Also, the hydrophilicity of the membrane was determined via contact angle analysis. Compared to the polyamide (PA) and PA/AlFu membranes, the as-synthesized TFN membrane contains 0.3 wt% GO had the highest water flux, 110.86 l/m 2 ·h, rejection of Na 2 SO 4 salt and Cr 2+ about 98.94% and 97.5%, respectively. Generally, using nanostructures like GO and AlFu (MOF) opens a novel path to improve hydrophilicity, negative charge, water flux, and rejection of polyamide nanocomposite membrane. Graphical Abstract For the treatment of wastewater and water resources, membrane technologies are rapidly developing. Also, water pollution by heavy metals, dyes, oil, medicinal, and salts leads to lower water quality and water shortages. In this research, thin-film nanocomposite nanofiltration (TFN) membranes were produced via the interfacial polymerization (IP) method between trimesoyl chloride (TMC) and m-phenylenediamine (MPD) monomers at the top surface of PES/(UF) membrane and modified by graphene oxide (GO) and aluminum fumarate (AlFu) metal-organic framework (MOF) nanostructures to remove heavy metal and (divalent and monovalent) salts. The FTIR, NMR, SEM, XRD, and zeta potential analyses investigated the modified thin-film nanocomposite membrane properties. Also, the hydrophilicity of the membrane was determined via contact angle analysis. Compared to the polyamide (PA) and PA/AlFu membranes, the as-synthesized TFN membrane contains 0.3 wt% GO had the highest water flux, 110.86 l/m2·h, rejection of Na2SO4 salt and Cr2+ about 98.94% and 97.5%, respectively. Generally, using nanostructures like GO and AlFu (MOF) opens a novel path to improve hydrophilicity, negative charge, water flux, and rejection of polyamide nanocomposite membrane.
ArticleNumber	77
Author	Tavakoli, Omid Fouladi, Mona Kavousi Heidari, Maryam
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SubjectTerms	Aluminum Characterization and Evaluation of Materials Chemistry and Materials Science Contact angle Graphene Heavy metals Hydrophilicity Inorganic Chemistry Lasers Materials Science Membranes Metal-organic frameworks Monomers Nanocomposites Nanofiltration Nanoparticles Nanostructure Nanotechnology NMR Nuclear magnetic resonance Oil pollution Optical Devices Optics Phenylenediamine Photonics Physical Chemistry Polyamide resins Polyamides Rejection Research Paper Sodium sulfate Thin films Wastewater treatment Water pollution Water quality Water resources Water shortages Zeta potential
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Title	Performance comparison of thin-film nanocomposite polyamide nanofiltration membranes for heavy metal/salt wastewater treatment
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