Multifaceted investigation of Sulfamerazine: Insights from computational methods, experimental techniques, and molecular simulations

•DFT and spectroscopic analysis of sulfamerazine Hirshfeld Surface, PED and MEP surface analysis.•FMO, UV-Vis analysis and NBO analysis for charge transfer studies.•Molecular docking and Molecular dynamic simulation of sulfamerazine with different Protein Receptors. The powerful sulfonamide antibiot...

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Vydáno v:Journal of molecular structure Ročník 1312; s. 138554
Hlavní autoři: Ahmad, Seraj, Reeda, V.S. Jeba, Aziz, Kashif, Arora, Himanshu, Kumar, Manoj, Garima, Km, Ali, Akram, Shahid, Mudassar, Muthu, S., Siddiqui, Nazia, Javed, Saleem
Médium: Journal Article
Jazyk:angličtina
Vydáno: Elsevier B.V 15.09.2024
Témata:
ISSN:0022-2860
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Abstract •DFT and spectroscopic analysis of sulfamerazine Hirshfeld Surface, PED and MEP surface analysis.•FMO, UV-Vis analysis and NBO analysis for charge transfer studies.•Molecular docking and Molecular dynamic simulation of sulfamerazine with different Protein Receptors. The powerful sulfonamide antibiotic Sulfamerazine has been the subject of in-depth study to clarify its complex molecular interactions. In order to understand Sulfamerazine's pharmacological behaviour and interactions with biological components, this comprehensive study uses computational tools such as Density Functional Theory (DFT) calculations, spectroscopic analyses, and molecular docking simulations. Exploitation B3LYP/6-311++G(d,p) basis set, DFT simulations have provided important new understandings of the structure, vibrational properties, and binding mechanisms of this system. Vibrational assignments have been conducted by analyzing individual vibrational modes and comparing them to experimental data. The molecule's weak interactions have been identified grounded on electron density using Reduced Density Gradient Analysis. Fukui and MEP plot analyses have been employed to pinpoint the molecule's electrophilic and nucleophilic sites. Frontier molecular orbital analysis supported the observation of charge transfer within the molecule. Sulfamerazine is a viable option for further pharmaceutical development, as shown by drug-likeness and ADME (absorption, distribution, metabolism, and excretion) studies. In docking analysis, the inhibitor 6qzh stood out as particularly potent, capable of forming up to three hydrogen bonds, resulting in a binding energy of -8.2 kcal/mol. Molecular dynamics simulations have also shed light on the stability, solubility, and possible interactions of Sulfamerazine in diverse settings. This all-encompassing strategy promises to increase our understanding of the mechanism of action of Sulfamerazine, creating new opportunities for the logical development of more potent pharmaceuticals. [Display omitted]
AbstractList •DFT and spectroscopic analysis of sulfamerazine Hirshfeld Surface, PED and MEP surface analysis.•FMO, UV-Vis analysis and NBO analysis for charge transfer studies.•Molecular docking and Molecular dynamic simulation of sulfamerazine with different Protein Receptors. The powerful sulfonamide antibiotic Sulfamerazine has been the subject of in-depth study to clarify its complex molecular interactions. In order to understand Sulfamerazine's pharmacological behaviour and interactions with biological components, this comprehensive study uses computational tools such as Density Functional Theory (DFT) calculations, spectroscopic analyses, and molecular docking simulations. Exploitation B3LYP/6-311++G(d,p) basis set, DFT simulations have provided important new understandings of the structure, vibrational properties, and binding mechanisms of this system. Vibrational assignments have been conducted by analyzing individual vibrational modes and comparing them to experimental data. The molecule's weak interactions have been identified grounded on electron density using Reduced Density Gradient Analysis. Fukui and MEP plot analyses have been employed to pinpoint the molecule's electrophilic and nucleophilic sites. Frontier molecular orbital analysis supported the observation of charge transfer within the molecule. Sulfamerazine is a viable option for further pharmaceutical development, as shown by drug-likeness and ADME (absorption, distribution, metabolism, and excretion) studies. In docking analysis, the inhibitor 6qzh stood out as particularly potent, capable of forming up to three hydrogen bonds, resulting in a binding energy of -8.2 kcal/mol. Molecular dynamics simulations have also shed light on the stability, solubility, and possible interactions of Sulfamerazine in diverse settings. This all-encompassing strategy promises to increase our understanding of the mechanism of action of Sulfamerazine, creating new opportunities for the logical development of more potent pharmaceuticals. [Display omitted]
ArticleNumber 138554
Author Arora, Himanshu
Aziz, Kashif
Ali, Akram
Javed, Saleem
Ahmad, Seraj
Shahid, Mudassar
Muthu, S.
Siddiqui, Nazia
Reeda, V.S. Jeba
Garima, Km
Kumar, Manoj
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  surname: Ahmad
  fullname: Ahmad, Seraj
  organization: Department of Chemistry, CMP College, University of Allahabad, Prayagraj, Uttar Pradesh 211002, India
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  givenname: V.S. Jeba
  surname: Reeda
  fullname: Reeda, V.S. Jeba
  organization: Department of Physics, Women's Christian College, Nagercoil, Tamil Nadu 629001, India
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  givenname: Kashif
  surname: Aziz
  fullname: Aziz, Kashif
  organization: Department of Chemistry, University of Allahabad, Prayagraj, Uttar Pradesh 211002, India
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  givenname: Himanshu
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  surname: Arora
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  organization: Department of Chemistry, CMP College, University of Allahabad, Prayagraj, Uttar Pradesh 211002, India
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  fullname: Ali, Akram
  organization: Department of Chemistry, CMP College, University of Allahabad, Prayagraj, Uttar Pradesh 211002, India
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  givenname: Mudassar
  surname: Shahid
  fullname: Shahid, Mudassar
  organization: Department of Pharmaceutics, College of Pharmacy, King Saud University, Riyadh 11451, Saudi Arabia
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  givenname: S.
  surname: Muthu
  fullname: Muthu, S.
  organization: Department of Physics, Aringnar Anna Govt. Arts College, Cheyyar 604407, India
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  givenname: Nazia
  surname: Siddiqui
  fullname: Siddiqui, Nazia
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  givenname: Saleem
  orcidid: 0000-0003-4623-100X
  surname: Javed
  fullname: Javed, Saleem
  email: saleem.7javed@gmail.com
  organization: Department of Chemistry, Jamia Millia Islamia, New Delhi, Delhi 110025, India
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DFT
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Vibrational behaviour
Molecular docking
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Snippet •DFT and spectroscopic analysis of sulfamerazine Hirshfeld Surface, PED and MEP surface analysis.•FMO, UV-Vis analysis and NBO analysis for charge transfer...
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SubjectTerms DFT
Hirshfeld analysis
Molecular docking
Molecular dynamics simulations
Vibrational behaviour
Title Multifaceted investigation of Sulfamerazine: Insights from computational methods, experimental techniques, and molecular simulations
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