Thermo-viscoplastic constitutive modeling of semicrystalline polymers with a novel perturbation-based return-mapping algorithm

The elasto-viscoplastic behavior of semicrystalline polymers is modeled using an implicit finite element framework across three distinct temperature regimes: below, near, and above the glass transition temperature. The study considers varying strain rates under both isothermal and adiabatic conditio...

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Published in:International journal of non-linear mechanics Vol. 180; p. 105252
Main Authors: Vadizadeh, Rahele, Zajkani, Asghar, Mirkhalaf, Mohsen
Format: Journal Article
Language:English
Published: Elsevier Ltd 01.01.2026
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ISSN:0020-7462
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Abstract The elasto-viscoplastic behavior of semicrystalline polymers is modeled using an implicit finite element framework across three distinct temperature regimes: below, near, and above the glass transition temperature. The study considers varying strain rates under both isothermal and adiabatic conditions. A phenomenological DSGZ (Duan, Saigal, Greif, and Zimmerman) viscoplastic model is developed specifically for semi-crystalline thermoplastics with high thermal and mechanical resistances. To address the challenges of highly nonlinear terms, a novel perturbation-based return-mapping approach is introduced, ensuring stable and efficient stress integration. Additionally, an optimized procedure is seamlessly integrated to facilitate material parameter identification essential for the viscoplasticity model. Simulation results exhibit strong agreement with a wide range of experimental data, highlighting the necessity of temperature-specific parameter sets. Furthermore, a sensitivity analysis is conducted to assess the influence of key parameters on mechanical response. These findings establish a robust computational framework for accurately simulating and designing thermoplastic components subjected to complex thermo-mechanical loading scenarios. •Finite element modeling of viscoplastic responses of semicrystalline polymers is considered.•Novel perturbation return mapping algorithm is introduced for implicit constitutive equations.•Consistent DSGZ model parameters related to quasi-static and dynamic strain rates are obtained.•Efficient parameter identification using an optimization scheme improves simulation results.•Distinct parameter sets identified for different temperature regimes at various strain rates.
AbstractList The elasto-viscoplastic behavior of semicrystalline polymers is modeled using an implicit finite element framework across three distinct temperature regimes: below, near, and above the glass transition temperature. The study considers varying strain rates under both isothermal and adiabatic conditions. A phenomenological DSGZ (Duan, Saigal, Greif, and Zimmerman) viscoplastic model is developed specifically for semi-crystalline thermoplastics with high thermal and mechanical resistances. To address the challenges of highly nonlinear terms, a novel perturbation-based return-mapping approach is introduced, ensuring stable and efficient stress integration. Additionally, an optimized procedure is seamlessly integrated to facilitate material parameter identification essential for the viscoplasticity model. Simulation results exhibit strong agreement with a wide range of experimental data, highlighting the necessity of temperature-specific parameter sets. Furthermore, a sensitivity analysis is conducted to assess the influence of key parameters on mechanical response. These findings establish a robust computational framework for accurately simulating and designing thermoplastic components subjected to complex thermo-mechanical loading scenarios.
The elasto-viscoplastic behavior of semicrystalline polymers is modeled using an implicit finite element framework across three distinct temperature regimes: below, near, and above the glass transition temperature. The study considers varying strain rates under both isothermal and adiabatic conditions. A phenomenological DSGZ (Duan, Saigal, Greif, and Zimmerman) viscoplastic model is developed specifically for semi-crystalline thermoplastics with high thermal and mechanical resistances. To address the challenges of highly nonlinear terms, a novel perturbation-based return-mapping approach is introduced, ensuring stable and efficient stress integration. Additionally, an optimized procedure is seamlessly integrated to facilitate material parameter identification essential for the viscoplasticity model. Simulation results exhibit strong agreement with a wide range of experimental data, highlighting the necessity of temperature-specific parameter sets. Furthermore, a sensitivity analysis is conducted to assess the influence of key parameters on mechanical response. These findings establish a robust computational framework for accurately simulating and designing thermoplastic components subjected to complex thermo-mechanical loading scenarios. •Finite element modeling of viscoplastic responses of semicrystalline polymers is considered.•Novel perturbation return mapping algorithm is introduced for implicit constitutive equations.•Consistent DSGZ model parameters related to quasi-static and dynamic strain rates are obtained.•Efficient parameter identification using an optimization scheme improves simulation results.•Distinct parameter sets identified for different temperature regimes at various strain rates.
ArticleNumber 105252
Author Zajkani, Asghar
Vadizadeh, Rahele
Mirkhalaf, Mohsen
Author_xml – sequence: 1
  givenname: Rahele
  surname: Vadizadeh
  fullname: Vadizadeh, Rahele
  organization: Department of Mechanical Engineering, Imam Khomeini International University, P.O.Box: 34149-16818, Qazvin, Iran
– sequence: 2
  givenname: Asghar
  orcidid: 0000-0003-3718-9807
  surname: Zajkani
  fullname: Zajkani, Asghar
  email: zajkani@eng.ikiu.ac.ir
  organization: Department of Mechanical Engineering, Imam Khomeini International University, P.O.Box: 34149-16818, Qazvin, Iran
– sequence: 3
  givenname: Mohsen
  surname: Mirkhalaf
  fullname: Mirkhalaf, Mohsen
  organization: Department of Physics, University of Gothenburg, Gothenburg 41296, Sweden
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Keywords Finite element method
Material identification
Viscoplastic constitutive model
Semicrystalline polymers
Radial return mapping algorithm
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Snippet The elasto-viscoplastic behavior of semicrystalline polymers is modeled using an implicit finite element framework across three distinct temperature regimes:...
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StartPage 105252
SubjectTerms Applied Mechanics
Finite element method
Material identification
Radial return mapping algorithm
Semicrystalline polymers
Teknisk mekanik
Viscoplastic constitutive model
Title Thermo-viscoplastic constitutive modeling of semicrystalline polymers with a novel perturbation-based return-mapping algorithm
URI https://dx.doi.org/10.1016/j.ijnonlinmec.2025.105252
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