Nonradical oxidation processes in PMS-based heterogeneous catalytic system: Generation, identification, oxidation characteristics, challenges response and application prospects
[Display omitted] •The nonradical mechanisms in PMS-based heterogeneous catalytic system were arranged.•The evolutionary pathways were summarized and analyzed.•Common identification methods were summarized and evaluated.•Nonradical exhibited its unique oxidation advantages.•Nonradical has extensive...
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| Published in: | Chemical engineering journal (Lausanne, Switzerland : 1996) Vol. 410; p. 128312 |
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| Main Authors: | , , , , |
| Format: | Journal Article |
| Language: | English |
| Published: |
Elsevier B.V
15.04.2021
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| Subjects: | |
| ISSN: | 1385-8947, 1873-3212 |
| Online Access: | Get full text |
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| Abstract | [Display omitted]
•The nonradical mechanisms in PMS-based heterogeneous catalytic system were arranged.•The evolutionary pathways were summarized and analyzed.•Common identification methods were summarized and evaluated.•Nonradical exhibited its unique oxidation advantages.•Nonradical has extensive application prospect in environmental remediation.
Recently, various nonradical oxidation mechanisms different from traditional free radicals have been discovered in peroxymonosulfate (PMS)-based heterogeneous catalytic system. These nonradical oxidation mechanisms have given rise to much controversy in many aspects due to their variety and complex evolutionary pathways. In this paper, we systematically summarized and compared these nonradical oxidation mechanisms. Mainly including the evolutionary pathways, identification methods (qualitative and quantitative), and oxidation characteristics. Moreover,the challenges and strategies for the further development of these oxidation mechanisms, as well as the research and application prospects are proposed. Our work can deepen systematic understanding of the nonradical oxidation mechanism among relevant researchers, and provides some enlightenment for using nonradical oxidation mechanism to deal with the environmental crisis. |
|---|---|
| AbstractList | [Display omitted]
•The nonradical mechanisms in PMS-based heterogeneous catalytic system were arranged.•The evolutionary pathways were summarized and analyzed.•Common identification methods were summarized and evaluated.•Nonradical exhibited its unique oxidation advantages.•Nonradical has extensive application prospect in environmental remediation.
Recently, various nonradical oxidation mechanisms different from traditional free radicals have been discovered in peroxymonosulfate (PMS)-based heterogeneous catalytic system. These nonradical oxidation mechanisms have given rise to much controversy in many aspects due to their variety and complex evolutionary pathways. In this paper, we systematically summarized and compared these nonradical oxidation mechanisms. Mainly including the evolutionary pathways, identification methods (qualitative and quantitative), and oxidation characteristics. Moreover,the challenges and strategies for the further development of these oxidation mechanisms, as well as the research and application prospects are proposed. Our work can deepen systematic understanding of the nonradical oxidation mechanism among relevant researchers, and provides some enlightenment for using nonradical oxidation mechanism to deal with the environmental crisis. |
| ArticleNumber | 128312 |
| Author | Chen, Zhuqi Zhao, Qindi Wang, Jia Zhou, Xinquan Chen, Zhulei |
| Author_xml | – sequence: 1 givenname: Xinquan surname: Zhou fullname: Zhou, Xinquan organization: Hubei Provincial Engineering Laboratory of Solid Waste Treatment, Disposal and Recycling, School of Environmental Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, PR China – sequence: 2 givenname: Qindi surname: Zhao fullname: Zhao, Qindi organization: Key Laboratory of Material Chemistry for Energy Conversion and Storage, Ministry of Education, Hubei Key Laboratory of Material Chemistry and Service Failure, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Wuhan 430074, PR China – sequence: 3 givenname: Jia surname: Wang fullname: Wang, Jia organization: Hubei Provincial Engineering Laboratory of Solid Waste Treatment, Disposal and Recycling, School of Environmental Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, PR China – sequence: 4 givenname: Zhulei surname: Chen fullname: Chen, Zhulei organization: Hubei Provincial Engineering Laboratory of Solid Waste Treatment, Disposal and Recycling, School of Environmental Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, PR China – sequence: 5 givenname: Zhuqi surname: Chen fullname: Chen, Zhuqi email: zqchen@hust.edu.cn organization: Key Laboratory of Material Chemistry for Energy Conversion and Storage, Ministry of Education, Hubei Key Laboratory of Material Chemistry and Service Failure, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Wuhan 430074, PR China |
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