NO and NO2 as non-innocent ligands: A comparison
•Redox systems (NO)n and (NO2)n are presented to reveal parallels and differences.•The suitability of (NO)n and (NO2)n for metal coordination is contrasted.•The scarcity of metal complexes with (NO2)n ligands (n = 0,+) is discussed.•Strategies to stabilize an NO2 ligand are pointed out.•The systems...
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| Vydáno v: | Coordination chemistry reviews Ročník 404; s. 213114 |
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| Jazyk: | angličtina |
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Elsevier B.V
01.02.2020
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| ISSN: | 0010-8545, 1873-3840 |
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| Abstract | •Redox systems (NO)n and (NO2)n are presented to reveal parallels and differences.•The suitability of (NO)n and (NO2)n for metal coordination is contrasted.•The scarcity of metal complexes with (NO2)n ligands (n = 0,+) is discussed.•Strategies to stabilize an NO2 ligand are pointed out.•The systems {O-NO}n and {M-NO}n are compared.
The potential of environmentally and technically relevant NO2 for non-innocent ligand behavior in coordination compounds is being evaluated in comparison with the well-studied metal complexes of nitrosyl, NOn (n = +,0,-,2-). A ruthenium semiquinone (Q−) radical complex platform [Ru(Q)(L)(NOx)] (x = 1 or 2, L = mer tridentate ligand) can serve to contrast the ligand characteristics of (NO)n and (NO2)n. Strategies to stabilize metal coordinated nitrogen dioxide (as “nitro” ligand NO2) versus the well established nitrite NO2− are suggested. |
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| AbstractList | •Redox systems (NO)n and (NO2)n are presented to reveal parallels and differences.•The suitability of (NO)n and (NO2)n for metal coordination is contrasted.•The scarcity of metal complexes with (NO2)n ligands (n = 0,+) is discussed.•Strategies to stabilize an NO2 ligand are pointed out.•The systems {O-NO}n and {M-NO}n are compared.
The potential of environmentally and technically relevant NO2 for non-innocent ligand behavior in coordination compounds is being evaluated in comparison with the well-studied metal complexes of nitrosyl, NOn (n = +,0,-,2-). A ruthenium semiquinone (Q−) radical complex platform [Ru(Q)(L)(NOx)] (x = 1 or 2, L = mer tridentate ligand) can serve to contrast the ligand characteristics of (NO)n and (NO2)n. Strategies to stabilize metal coordinated nitrogen dioxide (as “nitro” ligand NO2) versus the well established nitrite NO2− are suggested. |
| ArticleNumber | 213114 |
| Author | Záliš, Stanislav Sarkar, Biprajit Fiedler, Jan Das, Atanu Kaim, Wolfgang |
| Author_xml | – sequence: 1 givenname: Wolfgang surname: Kaim fullname: Kaim, Wolfgang email: kaim@iac.uni-stuttgart.de organization: Institut fuer Anorganische Chemie, Universitaet Stuttgart, D-70550 Stuttgart, Germany – sequence: 2 givenname: Atanu surname: Das fullname: Das, Atanu organization: Institut fuer Anorganische Chemie, Universitaet Stuttgart, D-70550 Stuttgart, Germany – sequence: 3 givenname: Jan surname: Fiedler fullname: Fiedler, Jan organization: The Czech Academy of Sciences, J. Heyrovský Institute of Physical Chemistry, Dolejškova 3, 18223 Prague, Czech Republic – sequence: 4 givenname: Stanislav surname: Záliš fullname: Záliš, Stanislav organization: The Czech Academy of Sciences, J. Heyrovský Institute of Physical Chemistry, Dolejškova 3, 18223 Prague, Czech Republic – sequence: 5 givenname: Biprajit surname: Sarkar fullname: Sarkar, Biprajit email: Biprajit.Sarkar@fu-berlin.de organization: Institut für Chemie und Biochemie, Freie Universität Berlin, Fabeckstraße 34-36, D-14195 Berlin, Germany |
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| Title | NO and NO2 as non-innocent ligands: A comparison |
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