A systematic process synthesis method towards sustainable extractive distillation processes with pre-concentration for separating the binary minimum azeotropes
•A systematic synthesis method for extractive distillation with pre-concentration.•The energy consumption bottleneck of the extractive distillation column was analyzed.•Replacing the pre-concentration column with a pre-stripper lower remixing effect.•The modified two-column configuration could enhan...
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| Published in: | Chemical engineering science Vol. 227; p. 115932 |
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| Format: | Journal Article |
| Language: | English |
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14.12.2020
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| ISSN: | 0009-2509, 1873-4405 |
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| Abstract | •A systematic synthesis method for extractive distillation with pre-concentration.•The energy consumption bottleneck of the extractive distillation column was analyzed.•Replacing the pre-concentration column with a pre-stripper lower remixing effect.•The modified two-column configuration could enhance overall sustainability.•A further intensified dividing-wall column was found not always advantageous.
A systematic process synthesis method is investigated towards sustainable extractive distillation with pre-concentration. To approach energy saving, it is one of the common senses to eliminate the infamous remixing effects. In detail, the energy consumption bottleneck is initially analyzed to come at the inspiration to replace the pre-concentration column with a pre-stripper. Afterwards, a two-column scheme is synthesized by combining the pre-stripper with either the extractive distillation column or entrainer recovery column. Finally, an extractive dividing wall column (EDWC) scheme is synthesized. A fair comparison of all configurations is given under a simulation-based framework employing a stochastic algorithm to optimize all decision variables including the usually arbitrarily fixed operating pressure. The results demonstrate two-column schemes to be more promising, saving more than 30% of economic and environmental costs, and improving energy efficiency by 1–2 times compared to the conventional system. Besides, EDWC structures are not always advantageous in sustainability. |
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| AbstractList | •A systematic synthesis method for extractive distillation with pre-concentration.•The energy consumption bottleneck of the extractive distillation column was analyzed.•Replacing the pre-concentration column with a pre-stripper lower remixing effect.•The modified two-column configuration could enhance overall sustainability.•A further intensified dividing-wall column was found not always advantageous.
A systematic process synthesis method is investigated towards sustainable extractive distillation with pre-concentration. To approach energy saving, it is one of the common senses to eliminate the infamous remixing effects. In detail, the energy consumption bottleneck is initially analyzed to come at the inspiration to replace the pre-concentration column with a pre-stripper. Afterwards, a two-column scheme is synthesized by combining the pre-stripper with either the extractive distillation column or entrainer recovery column. Finally, an extractive dividing wall column (EDWC) scheme is synthesized. A fair comparison of all configurations is given under a simulation-based framework employing a stochastic algorithm to optimize all decision variables including the usually arbitrarily fixed operating pressure. The results demonstrate two-column schemes to be more promising, saving more than 30% of economic and environmental costs, and improving energy efficiency by 1–2 times compared to the conventional system. Besides, EDWC structures are not always advantageous in sustainability. |
| ArticleNumber | 115932 |
| Author | He, Jie Zhang, Xiaodong Cui, Chengtian Sun, Jinsheng |
| Author_xml | – sequence: 1 givenname: Xiaodong surname: Zhang fullname: Zhang, Xiaodong organization: School of Chemical Engineering and Technology, Tianjin University, Tianjin 300072, PR China – sequence: 2 givenname: Jie surname: He fullname: He, Jie organization: School of Chemical Engineering and Technology, Tianjin University, Tianjin 300072, PR China – sequence: 3 givenname: Chengtian surname: Cui fullname: Cui, Chengtian email: ctcui@tju.edu.cn organization: School of Chemical Engineering and Technology, Tianjin University, Tianjin 300072, PR China – sequence: 4 givenname: Jinsheng surname: Sun fullname: Sun, Jinsheng email: jssun2006@vip.163.com organization: School of Chemical Engineering and Technology, Tianjin University, Tianjin 300072, PR China |
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| Keywords | Extractive distillation Systematic process synthesis method Dividing-wall columns Remixing elimination Pressure optimization |
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