A new Ag‐based photocatalyst for efficient degradation of antibiotic nitrofurantoin

In this paper, a new 0D Ag(I)‐based coordination polymer [Ag2(dib)(H2L)2](1) is proposed as a photocatalyst for the photocatalytic degradation of nitrofurantoin (NFT) under ultraviolet irradiation. The catalytic 1 was analyzed by various methods such as PXRD, SEM, FT‐IR, TGA, UV–vis, DRS, and electr...

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Published in:Applied organometallic chemistry Vol. 38; no. 7
Main Authors: Liu, Yichen, Zhou, Changxin, Xiang, Ruifang, Xiong, Dingqi, Li, Duqingcuo, Qin, Tianrui, Dong, Xiuyan, Muddassir, Mohd, Pan, Ying
Format: Journal Article
Language:English
Published: Chichester Wiley Subscription Services, Inc 01.07.2024
Subjects:
Ag(I)‐based coordination polymer
Antibiotics
Coordination polymers
Decomposition reactions
Free radicals
Irradiation
nitrofurantoin
Photocatalysis
photocatalyst
Photocatalysts
photocatalytic degradation
Photodecomposition
Photodegradation
Ultraviolet radiation
ISSN:0268-2605, 1099-0739
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Abstract In this paper, a new 0D Ag(I)‐based coordination polymer [Ag2(dib)(H2L)2](1) is proposed as a photocatalyst for the photocatalytic degradation of nitrofurantoin (NFT) under ultraviolet irradiation. The catalytic 1 was analyzed by various methods such as PXRD, SEM, FT‐IR, TGA, UV–vis, DRS, and electrochemical tests. The experimental result shows that 1 is an n‐type semiconductor, which can effectively catalyze the photodegradation of NFT under ultraviolet irradiation. Under the optimal reaction conditions, the photodegradation rate of NFT was 97.95% within 60 min when the concentration of NFT was 30 ppm. The experiment of free radical capture shows that O2˙− is the main active substance for photodecomposition, and the possible mechanism of 1 catalytic degradation of NFT is proposed. This research will lay the foundation for Ag(I)‐based coordination polymers in the field of antibiotic photocatalytic degradation. A new 0D Ag(I)‐based coordination polymer [Ag2(dib)(H2L)2](1) photocatalyzed NFT degradation rate of 97.95%. O2˙− is the main active substance for photodecomposition, and the possible mechanism of 1 catalytic degradation of NFT is proposed.
AbstractList In this paper, a new 0D Ag(I)‐based coordination polymer [Ag2(dib)(H2L)2](1) is proposed as a photocatalyst for the photocatalytic degradation of nitrofurantoin (NFT) under ultraviolet irradiation. The catalytic 1 was analyzed by various methods such as PXRD, SEM, FT‐IR, TGA, UV–vis, DRS, and electrochemical tests. The experimental result shows that 1 is an n‐type semiconductor, which can effectively catalyze the photodegradation of NFT under ultraviolet irradiation. Under the optimal reaction conditions, the photodegradation rate of NFT was 97.95% within 60 min when the concentration of NFT was 30 ppm. The experiment of free radical capture shows that O2˙− is the main active substance for photodecomposition, and the possible mechanism of 1 catalytic degradation of NFT is proposed. This research will lay the foundation for Ag(I)‐based coordination polymers in the field of antibiotic photocatalytic degradation. A new 0D Ag(I)‐based coordination polymer [Ag2(dib)(H2L)2](1) photocatalyzed NFT degradation rate of 97.95%. O2˙− is the main active substance for photodecomposition, and the possible mechanism of 1 catalytic degradation of NFT is proposed.
In this paper, a new 0D Ag(I)‐based coordination polymer [Ag 2 (dib)(H 2 L) 2 ]( 1 ) is proposed as a photocatalyst for the photocatalytic degradation of nitrofurantoin (NFT) under ultraviolet irradiation. The catalytic 1 was analyzed by various methods such as PXRD, SEM, FT‐IR, TGA, UV–vis, DRS, and electrochemical tests. The experimental result shows that 1 is an n ‐type semiconductor, which can effectively catalyze the photodegradation of NFT under ultraviolet irradiation. Under the optimal reaction conditions, the photodegradation rate of NFT was 97.95% within 60 min when the concentration of NFT was 30 ppm. The experiment of free radical capture shows that O 2 ˙ − is the main active substance for photodecomposition, and the possible mechanism of 1 catalytic degradation of NFT is proposed. This research will lay the foundation for Ag(I)‐based coordination polymers in the field of antibiotic photocatalytic degradation.
In this paper, a new 0D Ag(I)‐based coordination polymer [Ag2(dib)(H2L)2](1) is proposed as a photocatalyst for the photocatalytic degradation of nitrofurantoin (NFT) under ultraviolet irradiation. The catalytic 1 was analyzed by various methods such as PXRD, SEM, FT‐IR, TGA, UV–vis, DRS, and electrochemical tests. The experimental result shows that 1 is an n‐type semiconductor, which can effectively catalyze the photodegradation of NFT under ultraviolet irradiation. Under the optimal reaction conditions, the photodegradation rate of NFT was 97.95% within 60 min when the concentration of NFT was 30 ppm. The experiment of free radical capture shows that O2˙− is the main active substance for photodecomposition, and the possible mechanism of 1 catalytic degradation of NFT is proposed. This research will lay the foundation for Ag(I)‐based coordination polymers in the field of antibiotic photocatalytic degradation.
Author Liu, Yichen
Muddassir, Mohd
Xiong, Dingqi
Qin, Tianrui
Zhou, Changxin
Li, Duqingcuo
Dong, Xiuyan
Pan, Ying
Xiang, Ruifang
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  surname: Pan
  fullname: Pan, Ying
  email: panying@gdmu.edu.cn
  organization: Guangdong Medical University
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Snippet In this paper, a new 0D Ag(I)‐based coordination polymer [Ag2(dib)(H2L)2](1) is proposed as a photocatalyst for the photocatalytic degradation of...
In this paper, a new 0D Ag(I)‐based coordination polymer [Ag 2 (dib)(H 2 L) 2 ]( 1 ) is proposed as a photocatalyst for the photocatalytic degradation of...
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SubjectTerms Ag(I)‐based coordination polymer
Antibiotics
Coordination polymers
Decomposition reactions
Free radicals
Irradiation
nitrofurantoin
Photocatalysis
photocatalyst
Photocatalysts
photocatalytic degradation
Photodecomposition
Photodegradation
Ultraviolet radiation
Title A new Ag‐based photocatalyst for efficient degradation of antibiotic nitrofurantoin
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