Sputtering onto liquids: how does the liquid viscosity affect the formation of nanoparticles and metal films?
This paper reports on the effect of the solvent viscosity on the formation of gold nanoparticles (Au NPs) during the sputtering onto liquid (SoL) process. All other parameters related to the plasma and the host liquid are kept constant. SoL is a simple highly reproducible approach for the preparatio...
Uloženo v:
| Vydáno v: | Physical chemistry chemical physics : PCCP Ročník 25; číslo 4; s. 2803 |
|---|---|
| Hlavní autoři: | , , , , , , |
| Médium: | Journal Article |
| Jazyk: | angličtina |
| Vydáno: |
England
27.01.2023
|
| ISSN: | 1463-9084, 1463-9084 |
| On-line přístup: | Zjistit podrobnosti o přístupu |
| Tagy: |
Přidat tag
Žádné tagy, Buďte první, kdo vytvoří štítek k tomuto záznamu!
|
| Abstract | This paper reports on the effect of the solvent viscosity on the formation of gold nanoparticles (Au NPs) during the sputtering onto liquid (SoL) process. All other parameters related to the plasma and the host liquid are kept constant. SoL is a simple highly reproducible approach for the preparation of colloidal dispersions of small naked NPs. The properties of the final product are determined by both the sputtering parameters and the host liquid characteristics. As a model system we chose to sputter a gold target by a direct-current magnetron discharge onto a line of polymerized rapeseed oils having similar surface tension (32.6-33.1 mJ m
at RT). It was found that well-dispersed Au NPs grow in the bulk solution of oils with low viscosities (below 630 cP at 25 °C), while a gold film forms onto the surface of high viscosity liquids (more than 1000 cP at 25 °C). The mean diameter of the individual Au NPs is in the range of about 2.1-2.5 nm according to transmission electron microscopy. |
|---|---|
| AbstractList | This paper reports on the effect of the solvent viscosity on the formation of gold nanoparticles (Au NPs) during the sputtering onto liquid (SoL) process. All other parameters related to the plasma and the host liquid are kept constant. SoL is a simple highly reproducible approach for the preparation of colloidal dispersions of small naked NPs. The properties of the final product are determined by both the sputtering parameters and the host liquid characteristics. As a model system we chose to sputter a gold target by a direct-current magnetron discharge onto a line of polymerized rapeseed oils having similar surface tension (32.6-33.1 mJ m-2 at RT). It was found that well-dispersed Au NPs grow in the bulk solution of oils with low viscosities (below 630 cP at 25 °C), while a gold film forms onto the surface of high viscosity liquids (more than 1000 cP at 25 °C). The mean diameter of the individual Au NPs is in the range of about 2.1-2.5 nm according to transmission electron microscopy.This paper reports on the effect of the solvent viscosity on the formation of gold nanoparticles (Au NPs) during the sputtering onto liquid (SoL) process. All other parameters related to the plasma and the host liquid are kept constant. SoL is a simple highly reproducible approach for the preparation of colloidal dispersions of small naked NPs. The properties of the final product are determined by both the sputtering parameters and the host liquid characteristics. As a model system we chose to sputter a gold target by a direct-current magnetron discharge onto a line of polymerized rapeseed oils having similar surface tension (32.6-33.1 mJ m-2 at RT). It was found that well-dispersed Au NPs grow in the bulk solution of oils with low viscosities (below 630 cP at 25 °C), while a gold film forms onto the surface of high viscosity liquids (more than 1000 cP at 25 °C). The mean diameter of the individual Au NPs is in the range of about 2.1-2.5 nm according to transmission electron microscopy. This paper reports on the effect of the solvent viscosity on the formation of gold nanoparticles (Au NPs) during the sputtering onto liquid (SoL) process. All other parameters related to the plasma and the host liquid are kept constant. SoL is a simple highly reproducible approach for the preparation of colloidal dispersions of small naked NPs. The properties of the final product are determined by both the sputtering parameters and the host liquid characteristics. As a model system we chose to sputter a gold target by a direct-current magnetron discharge onto a line of polymerized rapeseed oils having similar surface tension (32.6-33.1 mJ m at RT). It was found that well-dispersed Au NPs grow in the bulk solution of oils with low viscosities (below 630 cP at 25 °C), while a gold film forms onto the surface of high viscosity liquids (more than 1000 cP at 25 °C). The mean diameter of the individual Au NPs is in the range of about 2.1-2.5 nm according to transmission electron microscopy. |
| Author | Sergievskaya, Anastasiya Chauvin, Adrien Godfroid, Thomas Absil, Rémi Yusenko, Kirill V Veselý, Jozef Konstantinidis, Stephanos |
| Author_xml | – sequence: 1 givenname: Anastasiya orcidid: 0000-0001-9589-9546 surname: Sergievskaya fullname: Sergievskaya, Anastasiya email: stephanos.konstantinidis@umons.ac.be organization: Plasma-Surface Interaction Chemistry (ChIPS), University of Mons, 23 Place du Parc, B-7000 Mons, Belgium. stephanos.konstantinidis@umons.ac.be – sequence: 2 givenname: Rémi surname: Absil fullname: Absil, Rémi organization: Green Frix S.A., Rue de la forêt 2, 7522 Blandain, Belgium – sequence: 3 givenname: Adrien orcidid: 0000-0003-1896-8776 surname: Chauvin fullname: Chauvin, Adrien email: stephanos.konstantinidis@umons.ac.be organization: Department of Condensed Matter Physics, Faculty of Mathematics and Physics, Charles University, Ke Karlovu 5, 121 16 Praha 2, Czech Republic – sequence: 4 givenname: Kirill V orcidid: 0000-0002-8390-4288 surname: Yusenko fullname: Yusenko, Kirill V organization: BAM Federal Institute for Materials Research and Testing, Richard-Willstätter Str. 11, D-12489 Berlin, Germany – sequence: 5 givenname: Jozef orcidid: 0000-0002-7395-0301 surname: Veselý fullname: Veselý, Jozef organization: Department of Physics of Materials, Faculty of Mathematics and Physics, Charles University, Ke Karlovu 5, 121 16 Praha 2, Czech Republic – sequence: 6 givenname: Thomas surname: Godfroid fullname: Godfroid, Thomas organization: Materia Nova Research Center, 3 Avenue Nicolas Copernic, Parc Initialis, 7000 Mons, Belgium – sequence: 7 givenname: Stephanos orcidid: 0000-0002-1672-309X surname: Konstantinidis fullname: Konstantinidis, Stephanos email: stephanos.konstantinidis@umons.ac.be organization: Plasma-Surface Interaction Chemistry (ChIPS), University of Mons, 23 Place du Parc, B-7000 Mons, Belgium. stephanos.konstantinidis@umons.ac.be |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/36412107$$D View this record in MEDLINE/PubMed |
| BookMark | eNpNkEtLxDAUhYOMOM7oxh8gWbqp5tW0dSMy-IIBF-q63ObhRNqk06TK_HuLjuDqHs757uVwF2jmgzcInVFySQmvrjRTPeGEl3CAjqmQPKtIKWb_9BwtYvwghNCc8iM051JQRklxjLqXfkzJDM6_4-BTwK3bjk7Ha7wJX1gHE3HamL2LP11UIbq0w2CtUekns2HoILngcbDYgw89DMmpdloFr3FnErTYuraLNyfo0EIbzel-LtHb_d3r6jFbPz88rW7XmWKySNlUsmCSKlpoTnKqoNJlY3JOCi7KBiZDCwFFzm2j8qopBRDCG5DCMtVoLdkSXfze7YewHU1MdTc1N20L3oQx1qzgFZFSUjKh53t0bDqj635wHQy7-u9F7BsZ32sU |
| CitedBy_id | crossref_primary_10_1021_acselectrochem_5c00036 crossref_primary_10_3390_toxins17080378 crossref_primary_10_1016_j_mattod_2025_03_007 crossref_primary_10_1088_1361_6463_adc276 |
| ContentType | Journal Article |
| DBID | NPM 7X8 |
| DOI | 10.1039/d2cp03038a |
| DatabaseName | PubMed MEDLINE - Academic |
| DatabaseTitle | PubMed MEDLINE - Academic |
| DatabaseTitleList | MEDLINE - Academic PubMed |
| Database_xml | – sequence: 1 dbid: NPM name: PubMed url: http://www.ncbi.nlm.nih.gov/entrez/query.fcgi?db=PubMed sourceTypes: Index Database – sequence: 2 dbid: 7X8 name: MEDLINE - Academic url: https://search.proquest.com/medline sourceTypes: Aggregation Database |
| DeliveryMethod | no_fulltext_linktorsrc |
| Discipline | Chemistry |
| EISSN | 1463-9084 |
| ExternalDocumentID | 36412107 |
| Genre | Journal Article |
| GroupedDBID | --- -DZ -JG -~X 0-7 0R~ 123 29O 4.4 53G 705 70~ 7~J 87K AAEMU AAIWI AAJAE AAMEH AANOJ AAWGC AAXHV AAXPP ABASK ABDVN ABEMK ABJNI ABPDG ABRYZ ABXOH ACGFO ACGFS ACIWK ACLDK ACNCT ADMRA ADSRN AEFDR AENEX AENGV AESAV AETIL AFLYV AFOGI AFRDS AFRZK AFVBQ AGEGJ AGKEF AGRSR AGSTE AHGCF ALMA_UNASSIGNED_HOLDINGS ANUXI APEMP ASKNT AUDPV AZFZN BLAPV BSQNT C6K CS3 D0L DU5 EBS ECGLT EE0 EF- F5P GGIMP GNO H13 HZ~ H~N IDZ J3G J3I M4U N9A NHB NPM O9- OK1 P2P R7B R7C RAOCF RCNCU RNS RPMJG RRA RRC RSCEA SKA SKF SLH TN5 TWZ UCJ UHB VH6 WH7 YNT 7X8 AKMSF ALUYA R56 |
| ID | FETCH-LOGICAL-c267t-5137261c17d3051ca9d8be5307348ba1cad44a753fbc59b84a003ba64f2cbdd62 |
| IEDL.DBID | 7X8 |
| ISICitedReferencesCount | 6 |
| ISICitedReferencesURI | http://www.webofscience.com/api/gateway?GWVersion=2&SrcApp=Summon&SrcAuth=ProQuest&DestLinkType=CitingArticles&DestApp=WOS_CPL&KeyUT=000890551100001&url=https%3A%2F%2Fcvtisr.summon.serialssolutions.com%2F%23%21%2Fsearch%3Fho%3Df%26include.ft.matches%3Dt%26l%3Dnull%26q%3D |
| ISSN | 1463-9084 |
| IngestDate | Fri Jul 11 09:23:10 EDT 2025 Wed Feb 19 02:25:15 EST 2025 |
| IsPeerReviewed | true |
| IsScholarly | true |
| Issue | 4 |
| Language | English |
| LinkModel | DirectLink |
| MergedId | FETCHMERGED-LOGICAL-c267t-5137261c17d3051ca9d8be5307348ba1cad44a753fbc59b84a003ba64f2cbdd62 |
| Notes | ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 23 |
| ORCID | 0000-0003-1896-8776 0000-0001-9589-9546 0000-0002-1672-309X 0000-0002-8390-4288 0000-0002-7395-0301 |
| PMID | 36412107 |
| PQID | 2739066610 |
| PQPubID | 23479 |
| ParticipantIDs | proquest_miscellaneous_2739066610 pubmed_primary_36412107 |
| PublicationCentury | 2000 |
| PublicationDate | 2023-01-27 |
| PublicationDateYYYYMMDD | 2023-01-27 |
| PublicationDate_xml | – month: 01 year: 2023 text: 2023-01-27 day: 27 |
| PublicationDecade | 2020 |
| PublicationPlace | England |
| PublicationPlace_xml | – name: England |
| PublicationTitle | Physical chemistry chemical physics : PCCP |
| PublicationTitleAlternate | Phys Chem Chem Phys |
| PublicationYear | 2023 |
| SSID | ssj0001513 |
| Score | 2.4407682 |
| Snippet | This paper reports on the effect of the solvent viscosity on the formation of gold nanoparticles (Au NPs) during the sputtering onto liquid (SoL) process. All... |
| SourceID | proquest pubmed |
| SourceType | Aggregation Database Index Database |
| StartPage | 2803 |
| Title | Sputtering onto liquids: how does the liquid viscosity affect the formation of nanoparticles and metal films? |
| URI | https://www.ncbi.nlm.nih.gov/pubmed/36412107 https://www.proquest.com/docview/2739066610 |
| Volume | 25 |
| WOSCitedRecordID | wos000890551100001&url=https%3A%2F%2Fcvtisr.summon.serialssolutions.com%2F%23%21%2Fsearch%3Fho%3Df%26include.ft.matches%3Dt%26l%3Dnull%26q%3D |
| hasFullText | |
| inHoldings | 1 |
| isFullTextHit | |
| isPrint | |
| link | http://cvtisr.summon.serialssolutions.com/2.0.0/link/0/eLvHCXMwpV1LS8NAEF7UCnrx_agvVvAaanc32cRLkWLxoKWgQm9hnxhok9S0Ff-9s3nYkyB4yWHDQpjMznyzO_t9CN1Yrm0QAXILBWEeE0p7gmgDCw9yhR9QQSrVkic-HIbjcTSqN9yKuq2yiYlloNaZcnvkHUizkcPa3dtePvOcapQ7Xa0lNNZRiwKUcV7Nxyu2cMhmtLpdRL3oNmQNPSmNOpqoHPybhuJ3aFmmmMHufz9uD-3U4BLfV96wj9ZMeoC2-o2m2yGavuSlMDXkK-yIC_AkmS0SXdzh9-wT68wUGABhPYqXSaFcT9cXFmXXR_nu57YjzixORQpFd91bh0Wq8dQAmsc2mUyL3hF6Gzy89h-9WnDBUyTgcw_MxaGiUl2uIQx0lYh0KI3vwgALpYABzZiAAsdK5UcyZAJighQBs0RJrQNyjDbSLDWnCEviuM0MVGPaMKulUL4G5CIB_1BJLWuj68aSMdjAnVKI1GSLIl7Zso1Oqt8R5xXzRkwD5gjP-NkfZp-jbScN77ZLCL9ALQvL2VyiTbWcJ8XHVekp8ByOnr8Bz9zK0g |
| linkProvider | ProQuest |
| openUrl | ctx_ver=Z39.88-2004&ctx_enc=info%3Aofi%2Fenc%3AUTF-8&rfr_id=info%3Asid%2Fsummon.serialssolutions.com&rft_val_fmt=info%3Aofi%2Ffmt%3Akev%3Amtx%3Ajournal&rft.genre=article&rft.atitle=Sputtering+onto+liquids%3A+how+does+the+liquid+viscosity+affect+the+formation+of+nanoparticles+and+metal+films%3F&rft.jtitle=Physical+chemistry+chemical+physics+%3A+PCCP&rft.au=Sergievskaya%2C+Anastasiya&rft.au=Absil%2C+R%C3%A9mi&rft.au=Chauvin%2C+Adrien&rft.au=Yusenko%2C+Kirill+V&rft.date=2023-01-27&rft.issn=1463-9084&rft.eissn=1463-9084&rft.volume=25&rft.issue=4&rft.spage=2803&rft_id=info:doi/10.1039%2Fd2cp03038a&rft.externalDBID=NO_FULL_TEXT |
| thumbnail_l | http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/lc.gif&issn=1463-9084&client=summon |
| thumbnail_m | http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/mc.gif&issn=1463-9084&client=summon |
| thumbnail_s | http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/sc.gif&issn=1463-9084&client=summon |