Thermal and mechanical properties of Ta2O5 doped La2Ce2O7 thermal barrier coatings prepared by atmospheric plasma spraying

La2Ce2O7 (LC) is a new promising thermal barrier coating (TBC) material for high-temperature applications. However, the sudden decrease of thermal expansion coefficient (TEC) at ∼623 K limits its application. In this study, the plasma-sprayed La2Ce1.7Ta0.3O7.15 (LCT) coating was developed by partial...

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Vydané v:	Journal of the European Ceramic Society Ročník 39; číslo 7; s. 2379 - 2388
Hlavní autori:	Zhang, Hao, Sun, Junbin, Duo, Shuwang, Zhou, Xin, Yuan, Jieyan, Dong, Shujuan, Yang, Xiong, Zeng, Jinyan, Jiang, Jianing, Deng, Longhui, Cao, Xueqiang
Médium:	Journal Article
Jazyk:	English
Vydavateľské údaje:	Elsevier Ltd 01.07.2019
Predmet:	Failure mechanism La2Ce2O7 Ta2O5 doping Thermal conductivity Failure mechanism Ta2O5 doping Thermal conductivity La2Ce2O7
ISSN:	0955-2219, 1873-619X
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Abstract	La2Ce2O7 (LC) is a new promising thermal barrier coating (TBC) material for high-temperature applications. However, the sudden decrease of thermal expansion coefficient (TEC) at ∼623 K limits its application. In this study, the plasma-sprayed La2Ce1.7Ta0.3O7.15 (LCT) coating was developed by partial substitution of Ce4+ in LC with Ta5+. LCT coating shows lower thermal conductivity between 298 K and 1273 K (0.54–0.71 W/(m·K)) than LC coating (0.65–0.85 W/(m·K)) and the traditional yttria partially stabilized zirconia (YSZ) coating (1.53–1.72 W/(m·K)). It also exhibits excellent thermal stability at least up to 1573 K for 1000 h. What is more, the sudden TEC drop is suppressed owing to the reduced oxygen vacancy concentration governed by Ta5+-substitution content. As a result, LCT TBC shows an improved thermal cycling lifetime in an air furnace as compared to LC TBC.
AbstractList	La2Ce2O7 (LC) is a new promising thermal barrier coating (TBC) material for high-temperature applications. However, the sudden decrease of thermal expansion coefficient (TEC) at ∼623 K limits its application. In this study, the plasma-sprayed La2Ce1.7Ta0.3O7.15 (LCT) coating was developed by partial substitution of Ce4+ in LC with Ta5+. LCT coating shows lower thermal conductivity between 298 K and 1273 K (0.54–0.71 W/(m·K)) than LC coating (0.65–0.85 W/(m·K)) and the traditional yttria partially stabilized zirconia (YSZ) coating (1.53–1.72 W/(m·K)). It also exhibits excellent thermal stability at least up to 1573 K for 1000 h. What is more, the sudden TEC drop is suppressed owing to the reduced oxygen vacancy concentration governed by Ta5+-substitution content. As a result, LCT TBC shows an improved thermal cycling lifetime in an air furnace as compared to LC TBC.
Author	Sun, Junbin Yuan, Jieyan Deng, Longhui Duo, Shuwang Zhou, Xin Zhang, Hao Cao, Xueqiang Zeng, Jinyan Dong, Shujuan Yang, Xiong Jiang, Jianing
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Snippet	La2Ce2O7 (LC) is a new promising thermal barrier coating (TBC) material for high-temperature applications. However, the sudden decrease of thermal expansion...
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SubjectTerms	Failure mechanism La2Ce2O7 Ta2O5 doping Thermal conductivity
Title	Thermal and mechanical properties of Ta2O5 doped La2Ce2O7 thermal barrier coatings prepared by atmospheric plasma spraying
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