Displacement of disordered water molecules from hydrophobic pocket creates enthalpic signature: Binding of phosphonamidate to the S1'-pocket of thermolysin

Prerequisite for the design of tight binding protein inhibitors and prediction of their properties is an in-depth understanding of the structural and thermodynamic details of the binding process. A series of closely related phosphonamidates was studied to elucidate the forces underlying their bindin...

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Veröffentlicht in:Biochimica et biophysica acta Jg. 1800; H. 11; S. 1192 - 1202
Hauptverfasser: Englert, L., Biela, A., Zayed, M., Heine, A., Hangauer, D., Klebe, G.
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Sprache:Englisch
Veröffentlicht: Netherlands 01.11.2010
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Abstract Prerequisite for the design of tight binding protein inhibitors and prediction of their properties is an in-depth understanding of the structural and thermodynamic details of the binding process. A series of closely related phosphonamidates was studied to elucidate the forces underlying their binding affinity to thermolysin. The investigated inhibitors are identical except for the parts penetrating into the hydrophobic S₁'-pocket. A correlation of structural, kinetic and thermodynamic data was carried out by X-ray crystallography, kinetic inhibition assay and isothermal titration calorimetry. Binding affinity increases with larger ligand hydrophobic P₁'-moieties accommodating the S₁'-pocket. Surprisingly, larger P₁'-side chain modifications are accompanied by an increase in the enthalpic contribution to binding. In agreement with other studies, it is suggested that the release of largely disordered waters from an imperfectly hydrated pocket results in an enthalpically favourable integration of these water molecules into bulk water upon inhibitor binding. This enthalpically favourable process contributes more strongly to the binding energetics than the entropy increase resulting from the release of water molecules from the S₁'-pocket or the formation of apolar interactions between protein and inhibitor. Displacement of highly disordered water molecules from a rather imperfectly hydrated and hydrophobic specificity pocket can reveal an enthalpic signature of inhibitor binding.
AbstractList Prerequisite for the design of tight binding protein inhibitors and prediction of their properties is an in-depth understanding of the structural and thermodynamic details of the binding process. A series of closely related phosphonamidates was studied to elucidate the forces underlying their binding affinity to thermolysin. The investigated inhibitors are identical except for the parts penetrating into the hydrophobic S₁'-pocket.BACKGROUNDPrerequisite for the design of tight binding protein inhibitors and prediction of their properties is an in-depth understanding of the structural and thermodynamic details of the binding process. A series of closely related phosphonamidates was studied to elucidate the forces underlying their binding affinity to thermolysin. The investigated inhibitors are identical except for the parts penetrating into the hydrophobic S₁'-pocket.A correlation of structural, kinetic and thermodynamic data was carried out by X-ray crystallography, kinetic inhibition assay and isothermal titration calorimetry.METHODSA correlation of structural, kinetic and thermodynamic data was carried out by X-ray crystallography, kinetic inhibition assay and isothermal titration calorimetry.Binding affinity increases with larger ligand hydrophobic P₁'-moieties accommodating the S₁'-pocket. Surprisingly, larger P₁'-side chain modifications are accompanied by an increase in the enthalpic contribution to binding. In agreement with other studies, it is suggested that the release of largely disordered waters from an imperfectly hydrated pocket results in an enthalpically favourable integration of these water molecules into bulk water upon inhibitor binding. This enthalpically favourable process contributes more strongly to the binding energetics than the entropy increase resulting from the release of water molecules from the S₁'-pocket or the formation of apolar interactions between protein and inhibitor.RESULTS AND CONCLUSIONSBinding affinity increases with larger ligand hydrophobic P₁'-moieties accommodating the S₁'-pocket. Surprisingly, larger P₁'-side chain modifications are accompanied by an increase in the enthalpic contribution to binding. In agreement with other studies, it is suggested that the release of largely disordered waters from an imperfectly hydrated pocket results in an enthalpically favourable integration of these water molecules into bulk water upon inhibitor binding. This enthalpically favourable process contributes more strongly to the binding energetics than the entropy increase resulting from the release of water molecules from the S₁'-pocket or the formation of apolar interactions between protein and inhibitor.Displacement of highly disordered water molecules from a rather imperfectly hydrated and hydrophobic specificity pocket can reveal an enthalpic signature of inhibitor binding.GENERAL SIGNIFICANCEDisplacement of highly disordered water molecules from a rather imperfectly hydrated and hydrophobic specificity pocket can reveal an enthalpic signature of inhibitor binding.
Prerequisite for the design of tight binding protein inhibitors and prediction of their properties is an in-depth understanding of the structural and thermodynamic details of the binding process. A series of closely related phosphonamidates was studied to elucidate the forces underlying their binding affinity to thermolysin. The investigated inhibitors are identical except for the parts penetrating into the hydrophobic S₁'-pocket. A correlation of structural, kinetic and thermodynamic data was carried out by X-ray crystallography, kinetic inhibition assay and isothermal titration calorimetry. Binding affinity increases with larger ligand hydrophobic P₁'-moieties accommodating the S₁'-pocket. Surprisingly, larger P₁'-side chain modifications are accompanied by an increase in the enthalpic contribution to binding. In agreement with other studies, it is suggested that the release of largely disordered waters from an imperfectly hydrated pocket results in an enthalpically favourable integration of these water molecules into bulk water upon inhibitor binding. This enthalpically favourable process contributes more strongly to the binding energetics than the entropy increase resulting from the release of water molecules from the S₁'-pocket or the formation of apolar interactions between protein and inhibitor. Displacement of highly disordered water molecules from a rather imperfectly hydrated and hydrophobic specificity pocket can reveal an enthalpic signature of inhibitor binding.
Author Englert, L.
Biela, A.
Heine, A.
Zayed, M.
Hangauer, D.
Klebe, G.
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Cites_doi 10.1021/bi051346v
10.1107/S0021889892009944
10.1038/newbio238041a0
10.1111/j.1432-1033.1986.tb09664.x
10.1093/protein/11.12.1235
10.1101/SQB.1987.052.01.012
10.1126/science.653353
10.1038/nrd3054
10.1107/S0907444998003254
10.1016/0022-2836(77)90286-8
10.1107/S0907444904019158
10.1107/S090744490200584X
10.1126/science.3810156
10.1016/0003-9861(71)90331-6
10.1007/s00894-008-0279-y
10.1016/0141-8130(82)90048-4
10.1021/ja0527525
10.1021/bi00289a002
10.1016/0022-2836(87)90124-0
10.1002/anie.200602227
10.1016/j.ab.2006.02.029
10.1126/science.8052849
10.1006/immu.1993.1053
10.1126/science.271.5245.72
10.1021/ja060070r
10.1002/cmdc.201000084
10.1002/anie.200701169
10.1002/(SICI)1097-0134(199604)24:4<433::AID-PROT3>3.0.CO;2-F
10.1016/S0006-291X(67)80122-0
10.1021/bi00159a016
10.1073/pnas.0407968101
10.1016/j.jmb.2009.04.051
10.1073/pnas.0610202104
10.1016/0003-2697(89)90213-3
10.1021/ma60030a031
10.1021/bi00400a008
10.1016/0022-2836(82)90319-9
10.1002/pro.61
10.1002/anie.200300644
10.1073/pnas.0806307105
10.1016/0003-9861(75)90085-5
10.1021/cr9804543
10.1016/j.drudis.2007.05.004
10.1021/ci980154m
10.1016/j.jmb.2009.06.016
10.1002/bip.360310802
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References Williams (10.1016/j.bbagen.2010.06.009_bib38) 2004; 43
Wolfenden (10.1016/j.bbagen.2010.06.009_bib30) 1994; 265
Patchett (10.1016/j.bbagen.2010.06.009_bib9) 1985; 57
Matthews (10.1016/j.bbagen.2010.06.009_bib28) 2009; 18
Gerlach (10.1016/j.bbagen.2010.06.009_bib5) 2007; 46
Young (10.1016/j.bbagen.2010.06.009_bib37) 2007; 104
Emsley (10.1016/j.bbagen.2010.06.009_bib43) 2004; 60
Laskowski (10.1016/j.bbagen.2010.06.009_bib49) 1993; 26
Jeffrey (10.1016/j.bbagen.2010.06.009_bib20) 1982; 4
Morihara (10.1016/j.bbagen.2010.06.009_bib7) 1967; 26
Juers (10.1016/j.bbagen.2010.06.009_bib10) 2005; 44
Holden (10.1016/j.bbagen.2010.06.009_bib15) 1987; 26
Whittaker (10.1016/j.bbagen.2010.06.009_bib12) 1999; 99
Zhang (10.1016/j.bbagen.2010.06.009_bib31) 1996; 24
Vaitheeswaran (10.1016/j.bbagen.2010.06.009_bib32) 2004; 101
Burling (10.1016/j.bbagen.2010.06.009_bib34) 1996; 271
Holmes (10.1016/j.bbagen.2010.06.009_bib39) 1982; 160
Shimokhina (10.1016/j.bbagen.2010.06.009_bib26) 2006; 45
Sheriff (10.1016/j.bbagen.2010.06.009_bib45) 1993; 3
Ladbury (10.1016/j.bbagen.2010.06.009_bib4) 2010; 9
Komiyama (10.1016/j.bbagen.2010.06.009_bib23) 1975; 171
Harrison (10.1016/j.bbagen.2010.06.009_bib11) 1992; 31
Tronrud (10.1016/j.bbagen.2010.06.009_bib14) 1986; 157
Sheriff (10.1016/j.bbagen.2010.06.009_bib46) 1987; 197
Baum (10.1016/j.bbagen.2010.06.009_bib3) 2009; 391
Englert (10.1016/j.bbagen.2010.06.009_bib24) 2010; 5
Tronrud (10.1016/j.bbagen.2010.06.009_bib18) 1987; 235
Matthews (10.1016/j.bbagen.2010.06.009_bib6) 1972; 238
Sheldrick (10.1016/j.bbagen.2010.06.009_bib42) 1997; Vol. 277
Weimer (10.1016/j.bbagen.2010.06.009_bib47) 2006; 352
Tanford (10.1016/j.bbagen.2010.06.009_bib27) 1978; 200
Homans (10.1016/j.bbagen.2010.06.009_bib36) 2007; 12
Otwinowski (10.1016/j.bbagen.2010.06.009_bib40) 1997; Vol. 276
Weaver (10.1016/j.bbagen.2010.06.009_bib19) 1977; 114
Hausrath (10.1016/j.bbagen.2010.06.009_bib22) 2002; 58
Sansom (10.1016/j.bbagen.2010.06.009_bib13) 1998; 11
Wade (10.1016/j.bbagen.2010.06.009_bib29) 1991; 31
Brunger (10.1016/j.bbagen.2010.06.009_bib41) 1998; 54
Clark (10.1016/j.bbagen.2010.06.009_bib21) 2008; 14
Bartlett (10.1016/j.bbagen.2010.06.009_bib16) 1987; 52
Bartlett (10.1016/j.bbagen.2010.06.009_bib17) 1983; 22
Matthews (10.1016/j.bbagen.2010.06.009_bib44) 1972; 5
Liu (10.1016/j.bbagen.2010.06.009_bib33) 2008; 105
Drucker (10.1016/j.bbagen.2010.06.009_bib8) 1971; 147
Barratt (10.1016/j.bbagen.2010.06.009_bib35) 2005; 127
Leatherbarrow (10.1016/j.bbagen.2010.06.009_bib48) 1998
Wiseman (10.1016/j.bbagen.2010.06.009_bib50) 1989; 179
Krishnamurthy (10.1016/j.bbagen.2010.06.009_bib1) 2006; 128
Viswanadhan (10.1016/j.bbagen.2010.06.009_bib25) 1999; 39
Baum (10.1016/j.bbagen.2010.06.009_bib2) 2009; 390
References_xml – volume: 44
  start-page: 16524
  year: 2005
  ident: 10.1016/j.bbagen.2010.06.009_bib10
  article-title: Structural analysis of silanediols as transition-state-analogue inhibitors of the benchmark metalloprotease thermolysin
  publication-title: Biochemistry
  doi: 10.1021/bi051346v
– volume: 26
  start-page: 283
  year: 1993
  ident: 10.1016/j.bbagen.2010.06.009_bib49
  article-title: PROCHECK: a program to check the stereochemical quality of protein structures
  publication-title: J. Appl. Crystallogr
  doi: 10.1107/S0021889892009944
– volume: 238
  start-page: 41
  year: 1972
  ident: 10.1016/j.bbagen.2010.06.009_bib6
  article-title: Structure of thermolysin
  publication-title: Nat. New Biol.
  doi: 10.1038/newbio238041a0
– volume: 157
  start-page: 261
  year: 1986
  ident: 10.1016/j.bbagen.2010.06.009_bib14
  article-title: Crystallographic structural analysis of phosphoramidates as inhibitors and transition-state analogs of thermolysin
  publication-title: Eur. J. Biochem.
  doi: 10.1111/j.1432-1033.1986.tb09664.x
– volume: 11
  start-page: 1235
  year: 1998
  ident: 10.1016/j.bbagen.2010.06.009_bib13
  article-title: Molecular modelling and site-directed mutagenesis of the active site of endothelin-converting enzyme
  publication-title: Protein Eng.
  doi: 10.1093/protein/11.12.1235
– volume: 52
  start-page: 83
  year: 1987
  ident: 10.1016/j.bbagen.2010.06.009_bib16
  article-title: Phosphorus-containing peptide analogs as peptidase inhibitors
  publication-title: Cold Spring Harbor Symp. Quant. Biol.
  doi: 10.1101/SQB.1987.052.01.012
– volume: Vol. 276
  start-page: 307
  year: 1997
  ident: 10.1016/j.bbagen.2010.06.009_bib40
– volume: 200
  start-page: 1012
  year: 1978
  ident: 10.1016/j.bbagen.2010.06.009_bib27
  article-title: The hydrophobic effect and the organization of living matter
  publication-title: Science
  doi: 10.1126/science.653353
– volume: Vol. 277
  start-page: 319
  year: 1997
  ident: 10.1016/j.bbagen.2010.06.009_bib42
– volume: 9
  start-page: 23
  year: 2010
  ident: 10.1016/j.bbagen.2010.06.009_bib4
  article-title: Adding calorimetric data to decision making in lead discovery: a hot tip
  publication-title: Nat. Rev. Drug Discov.
  doi: 10.1038/nrd3054
– volume: 54
  start-page: 905
  year: 1998
  ident: 10.1016/j.bbagen.2010.06.009_bib41
  article-title: Crystallography & NMR system: a new software suite for macromolecular structure determination
  publication-title: Acta Crystallogr., Sect. D: Biol. Crystallogr.
  doi: 10.1107/S0907444998003254
– volume: 114
  start-page: 119
  year: 1977
  ident: 10.1016/j.bbagen.2010.06.009_bib19
  article-title: A crystallographic study of the complex of phosphoramidon with thermolysin. A model for the presumed catalytic transition state and for the binding of extended substances
  publication-title: J. Mol. Biol.
  doi: 10.1016/0022-2836(77)90286-8
– volume: 60
  start-page: 2126
  year: 2004
  ident: 10.1016/j.bbagen.2010.06.009_bib43
  article-title: Coot: model-building tools for molecular graphics
  publication-title: Acta Crystallogr., Sect. D: Biol. Crystallogr.
  doi: 10.1107/S0907444904019158
– year: 1998
  ident: 10.1016/j.bbagen.2010.06.009_bib48
– volume: 58
  start-page: 1002
  year: 2002
  ident: 10.1016/j.bbagen.2010.06.009_bib22
  article-title: Thermolysin in the absence of substrate has an open conformation
  publication-title: Acta Crystallogr., Sect. D: Biol. Crystallogr.
  doi: 10.1107/S090744490200584X
– volume: 235
  start-page: 571
  year: 1987
  ident: 10.1016/j.bbagen.2010.06.009_bib18
  article-title: Structures of two thermolysin–inhibitor complexes that differ by a single hydrogen bond
  publication-title: Science
  doi: 10.1126/science.3810156
– volume: 147
  start-page: 242
  year: 1971
  ident: 10.1016/j.bbagen.2010.06.009_bib8
  article-title: The role of calcium in thermolysin: effect on kinetic properties and autodigestion
  publication-title: Arch. Biochem. Biophys.
  doi: 10.1016/0003-9861(71)90331-6
– volume: 14
  start-page: 689
  year: 2008
  ident: 10.1016/j.bbagen.2010.06.009_bib21
  article-title: Why are dimethyl sulfoxide and dimethyl sulfone such good solvents?
  publication-title: J. Mol. Model.
  doi: 10.1007/s00894-008-0279-y
– volume: 4
  start-page: 173
  year: 1982
  ident: 10.1016/j.bbagen.2010.06.009_bib20
  publication-title: Int. J. Biol. Macromol.
  doi: 10.1016/0141-8130(82)90048-4
– volume: 127
  start-page: 11827
  year: 2005
  ident: 10.1016/j.bbagen.2010.06.009_bib35
  article-title: Van der Waals interactions dominate ligand–protein association in a protein binding site occluded from solvent water
  publication-title: J. Am. Chem. Soc.
  doi: 10.1021/ja0527525
– volume: 22
  start-page: 4618
  year: 1983
  ident: 10.1016/j.bbagen.2010.06.009_bib17
  article-title: Phosphonamidates as transition-state analogue inhibitors of thermolysin
  publication-title: Biochemistry
  doi: 10.1021/bi00289a002
– volume: 197
  start-page: 273
  year: 1987
  ident: 10.1016/j.bbagen.2010.06.009_bib46
  article-title: Structure of myohemerythrin in the azidomet state at 1.7/1.3 A resolution
  publication-title: J. Mol. Biol.
  doi: 10.1016/0022-2836(87)90124-0
– volume: 45
  start-page: 6374
  year: 2006
  ident: 10.1016/j.bbagen.2010.06.009_bib26
  article-title: Contribution of ligand desolvation to binding thermodynamics in a ligand–protein interaction
  publication-title: Angew. Chem. Int. Ed. Engl.
  doi: 10.1002/anie.200602227
– volume: 352
  start-page: 110
  year: 2006
  ident: 10.1016/j.bbagen.2010.06.009_bib47
  article-title: A quenched fluorescent dipeptide for assaying dispase- and thermolysin-like proteases
  publication-title: Anal. Biochem.
  doi: 10.1016/j.ab.2006.02.029
– volume: 265
  start-page: 936
  year: 1994
  ident: 10.1016/j.bbagen.2010.06.009_bib30
  article-title: On the probability of finding a water molecule in a nonpolar cavity
  publication-title: Science
  doi: 10.1126/science.8052849
– volume: 3
  start-page: 191
  year: 1993
  ident: 10.1016/j.bbagen.2010.06.009_bib45
  article-title: Some methods for examining the interactions between two molecules
  publication-title: Immunomethods
  doi: 10.1006/immu.1993.1053
– volume: 271
  start-page: 72
  year: 1996
  ident: 10.1016/j.bbagen.2010.06.009_bib34
  article-title: Direct observation of protein solvation and discrete disorder with experimental crystallographic phases
  publication-title: Science
  doi: 10.1126/science.271.5245.72
– volume: 128
  start-page: 5802
  year: 2006
  ident: 10.1016/j.bbagen.2010.06.009_bib1
  article-title: The paradoxical thermodynamic basis for the interaction of ethylene glycol, glycine, and sarcosine chains with bovine carbonic anhydrase II: an unexpected manifestation of enthalpy/entropy compensation
  publication-title: J. Am. Chem. Soc.
  doi: 10.1021/ja060070r
– volume: 5
  start-page: 930
  year: 2010
  ident: 10.1016/j.bbagen.2010.06.009_bib24
  article-title: Fragment-based lead discovery: screening and optimizing fragments for thermolysin inhibition
  publication-title: ChemMedChem
  doi: 10.1002/cmdc.201000084
– volume: 46
  start-page: 8511
  year: 2007
  ident: 10.1016/j.bbagen.2010.06.009_bib5
  article-title: Thermodynamic inhibition profile of a cyclopentyl and a cyclohexyl derivative towards thrombin: the same but for different reasons
  publication-title: Angew. Chem. Int. Ed. Engl.
  doi: 10.1002/anie.200701169
– volume: 24
  start-page: 433
  year: 1996
  ident: 10.1016/j.bbagen.2010.06.009_bib31
  article-title: Hydrophilicity of cavities in proteins
  publication-title: Proteins
  doi: 10.1002/(SICI)1097-0134(199604)24:4<433::AID-PROT3>3.0.CO;2-F
– volume: 26
  start-page: 656
  year: 1967
  ident: 10.1016/j.bbagen.2010.06.009_bib7
  article-title: The specificities of various neutral and alkaline proteinases from microorganisms
  publication-title: Biochem. Biophys. Res. Commun.
  doi: 10.1016/S0006-291X(67)80122-0
– volume: 31
  start-page: 10757
  year: 1992
  ident: 10.1016/j.bbagen.2010.06.009_bib11
  article-title: Mechanistic studies on the human matrix metalloproteinase stromelysin
  publication-title: Biochemistry
  doi: 10.1021/bi00159a016
– volume: 57
  start-page: 1
  year: 1985
  ident: 10.1016/j.bbagen.2010.06.009_bib9
  article-title: The design and properties of N-carboxyalkyldipeptide inhibitors of angiotensin-converting enzyme
  publication-title: Adv. Enzymol. Relat. Areas Mol. Biol.
– volume: 101
  start-page: 17002
  year: 2004
  ident: 10.1016/j.bbagen.2010.06.009_bib32
  article-title: Water clusters in nonpolar cavities
  publication-title: Proc. Natl Acad. Sci. U. S. A.
  doi: 10.1073/pnas.0407968101
– volume: 390
  start-page: 56
  year: 2009
  ident: 10.1016/j.bbagen.2010.06.009_bib2
  article-title: More than a simple lipophilic contact: a detailed thermodynamic analysis of nonbasic residues in the S1 pocket of thrombin
  publication-title: J. Mol. Biol.
  doi: 10.1016/j.jmb.2009.04.051
– volume: 104
  start-page: 808
  year: 2007
  ident: 10.1016/j.bbagen.2010.06.009_bib37
  article-title: Motifs for molecular recognition exploiting hydrophobic enclosure in protein–ligand binding
  publication-title: Proc. Natl Acad. Sci. U. S. A.
  doi: 10.1073/pnas.0610202104
– volume: 179
  start-page: 131
  year: 1989
  ident: 10.1016/j.bbagen.2010.06.009_bib50
  article-title: Rapid measurement of binding constants and heats of binding using a new titration calorimeter
  publication-title: Anal. Biochem.
  doi: 10.1016/0003-2697(89)90213-3
– volume: 5
  start-page: 818
  year: 1972
  ident: 10.1016/j.bbagen.2010.06.009_bib44
  article-title: The gamma-turn. Evidence for a new folded conformation in proteins
  publication-title: Macromolecules
  doi: 10.1021/ma60030a031
– volume: 26
  start-page: 8542
  year: 1987
  ident: 10.1016/j.bbagen.2010.06.009_bib15
  article-title: Slow- and fast-binding inhibitors of thermolysin display different modes of binding: crystallographic analysis of extended phosphonamidate transition-state analogues
  publication-title: Biochemistry
  doi: 10.1021/bi00400a008
– volume: 160
  start-page: 623
  year: 1982
  ident: 10.1016/j.bbagen.2010.06.009_bib39
  article-title: Structure of thermolysin refined at 1.6 A resolution
  publication-title: J. Mol. Biol.
  doi: 10.1016/0022-2836(82)90319-9
– volume: 18
  start-page: 494
  year: 2009
  ident: 10.1016/j.bbagen.2010.06.009_bib28
  article-title: A review about nothing: are apolar cavities in proteins really empty?
  publication-title: Protein Sci.
  doi: 10.1002/pro.61
– volume: 43
  start-page: 6596
  year: 2004
  ident: 10.1016/j.bbagen.2010.06.009_bib38
  article-title: Understanding noncovalent interactions: ligand binding energy and catalytic efficiency from ligand-induced reductions in motion within receptors and enzymes
  publication-title: Angew. Chem. Int. Ed. Engl.
  doi: 10.1002/anie.200300644
– volume: 105
  start-page: 14406
  year: 2008
  ident: 10.1016/j.bbagen.2010.06.009_bib33
  article-title: Use of experimental crystallographic phases to examine the hydration of polar and nonpolar cavities in T4 lysozyme
  publication-title: Proc. Natl Acad. Sci. U. S. A.
  doi: 10.1073/pnas.0806307105
– volume: 171
  start-page: 727
  year: 1975
  ident: 10.1016/j.bbagen.2010.06.009_bib23
  article-title: Studies on inhibitory effect of phosphoramidon and its analogs on thermolysin
  publication-title: Arch. Biochem. Biophys.
  doi: 10.1016/0003-9861(75)90085-5
– volume: 99
  start-page: 2735
  year: 1999
  ident: 10.1016/j.bbagen.2010.06.009_bib12
  article-title: Design and therapeutic application of matrix metalloproteinase inhibitors
  publication-title: Chem. Rev.
  doi: 10.1021/cr9804543
– volume: 12
  start-page: 534
  year: 2007
  ident: 10.1016/j.bbagen.2010.06.009_bib36
  article-title: Water, water everywhere—except where it matters?
  publication-title: Drug Discovery Today
  doi: 10.1016/j.drudis.2007.05.004
– volume: 39
  start-page: 405
  year: 1999
  ident: 10.1016/j.bbagen.2010.06.009_bib25
  article-title: Prediction of solvation free energies of small organic molecules: additive-constitutive models based on molecular fingerprints and atomic constants
  publication-title: J. Chem. Inf. Comput. Sci.
  doi: 10.1021/ci980154m
– volume: 391
  start-page: 552
  year: 2009
  ident: 10.1016/j.bbagen.2010.06.009_bib3
  article-title: Think twice: understanding the high potency of bis(phenyl)methane inhibitors of thrombin
  publication-title: J. Mol. Biol.
  doi: 10.1016/j.jmb.2009.06.016
– volume: 31
  start-page: 919
  year: 1991
  ident: 10.1016/j.bbagen.2010.06.009_bib29
  article-title: A molecular dynamics study of thermodynamic and structural aspects of the hydration of cavities in proteins
  publication-title: Biopolymers
  doi: 10.1002/bip.360310802
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Snippet Prerequisite for the design of tight binding protein inhibitors and prediction of their properties is an in-depth understanding of the structural and...
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SubjectTerms Binding Sites
Crystallography, X-Ray
Entropy
Hydrophobic and Hydrophilic Interactions
Models, Molecular
Organophosphorus Compounds - chemistry
Organophosphorus Compounds - metabolism
Phosphoamino Acids - chemistry
Protein Binding
Protein Structure, Tertiary
Thermodynamics
Thermolysin - metabolism
Water - chemistry
Water - metabolism
Title Displacement of disordered water molecules from hydrophobic pocket creates enthalpic signature: Binding of phosphonamidate to the S1'-pocket of thermolysin
URI https://www.ncbi.nlm.nih.gov/pubmed/20600625
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