Multiple site occupancies of Eu3+ in differently oriented ZnMgO:Eu epilayers
•High-resolution XRD analysis and reciprocal space mapping of polar and non-polar ZnMgO:Eu epilayers.•Temperature-dependent PL and PLE analyses.•Luminescence decay kinetics of Eu3+ in ZnMgO is presented at 4.6 K, 90 K and room temperature.•Eu3+ ions exhibit long radiative lifetime in ZnMgO random al...
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| Vydané v: | Materials research bulletin Ročník 188; s. 113403 |
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| Hlavní autori: | , , , , , , |
| Médium: | Journal Article |
| Jazyk: | English |
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Elsevier Ltd
01.08.2025
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| ISSN: | 0025-5408 |
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| Abstract | •High-resolution XRD analysis and reciprocal space mapping of polar and non-polar ZnMgO:Eu epilayers.•Temperature-dependent PL and PLE analyses.•Luminescence decay kinetics of Eu3+ in ZnMgO is presented at 4.6 K, 90 K and room temperature.•Eu3+ ions exhibit long radiative lifetime in ZnMgO random alloy.•Multiple site occupancies of Eu3+ ions in ZnMgO random alloy are confirmed.
ZnMgO:Eu epilayers were grown on polar c-plane and non-polar r-plane Al2O3 substrates via oxygen plasma-assisted molecular beam epitaxy. The effect of crystal orientation on the luminescence properties is investigated in the as-grown and annealed ZnMgO:Eu crystals. The structural characteristics were accurately evaluated using the symmetrical and asymmetrical reciprocal space maps of high-resolution XRD measurements. Photoluminescence (PL), PL excitation properties and PL decay kinetics were studied at room- and low- temperatures. Regardless of the crystal orientation, annealed ZnMgO:Eu epilayers exhibit an intense Eu3+ red emission boosted by efficient host-to-dopant energy transfer and charge transfer mechanisms. However, ZnMgO:Eu/r-Al2O3 presents intrinsic defect luminescence centres, relatively quenching Eu3+ PL. Multiple emission lines are identified in the 5D0 to 7FJ=0 transition range. PL decay kinetics of Eu3+ showcases a long luminescence lifetime and multi-exponential behaviour under resonant and non-resonant excitations. Temperature-dependent luminescence analyses confirm multiple site occupancies of Eu3+ in ZnMgO.
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| AbstractList | •High-resolution XRD analysis and reciprocal space mapping of polar and non-polar ZnMgO:Eu epilayers.•Temperature-dependent PL and PLE analyses.•Luminescence decay kinetics of Eu3+ in ZnMgO is presented at 4.6 K, 90 K and room temperature.•Eu3+ ions exhibit long radiative lifetime in ZnMgO random alloy.•Multiple site occupancies of Eu3+ ions in ZnMgO random alloy are confirmed.
ZnMgO:Eu epilayers were grown on polar c-plane and non-polar r-plane Al2O3 substrates via oxygen plasma-assisted molecular beam epitaxy. The effect of crystal orientation on the luminescence properties is investigated in the as-grown and annealed ZnMgO:Eu crystals. The structural characteristics were accurately evaluated using the symmetrical and asymmetrical reciprocal space maps of high-resolution XRD measurements. Photoluminescence (PL), PL excitation properties and PL decay kinetics were studied at room- and low- temperatures. Regardless of the crystal orientation, annealed ZnMgO:Eu epilayers exhibit an intense Eu3+ red emission boosted by efficient host-to-dopant energy transfer and charge transfer mechanisms. However, ZnMgO:Eu/r-Al2O3 presents intrinsic defect luminescence centres, relatively quenching Eu3+ PL. Multiple emission lines are identified in the 5D0 to 7FJ=0 transition range. PL decay kinetics of Eu3+ showcases a long luminescence lifetime and multi-exponential behaviour under resonant and non-resonant excitations. Temperature-dependent luminescence analyses confirm multiple site occupancies of Eu3+ in ZnMgO.
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| ArticleNumber | 113403 |
| Author | Jakiela, Rafal Wierzbicka, Aleksandra Mathew, Juby Alphonsa Zhydachevskyy, Yaroslav Lysak, Anastasiia Kozanecki, Adrian Stachowicz, Marcin |
| Author_xml | – sequence: 1 givenname: Juby Alphonsa orcidid: 0000-0002-3047-9716 surname: Mathew fullname: Mathew, Juby Alphonsa email: mathewja@ifpan.edu.pl – sequence: 2 givenname: Aleksandra surname: Wierzbicka fullname: Wierzbicka, Aleksandra – sequence: 3 givenname: Rafal surname: Jakiela fullname: Jakiela, Rafal – sequence: 4 givenname: Yaroslav surname: Zhydachevskyy fullname: Zhydachevskyy, Yaroslav – sequence: 5 givenname: Anastasiia surname: Lysak fullname: Lysak, Anastasiia – sequence: 6 givenname: Marcin surname: Stachowicz fullname: Stachowicz, Marcin – sequence: 7 givenname: Adrian surname: Kozanecki fullname: Kozanecki, Adrian |
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| Keywords | Eu-doped ZnMgO alloy Optical material Luminescence decay kinetics Crystal orientation Molecular Beam Epitaxy |
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