Laser-engineered rattan evaporators for scalable and sustainable solar desalination
Scalable and sustainable solar-driven interfacial evaporators are vital to addressing global freshwater scarcity and sustainability challenges. However, the applicability of biomass-based evaporators is often limited by costly and complex fabrication processes. Here, we report a high-performance rat...
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| Vydáno v: | Chemical engineering journal (Lausanne, Switzerland : 1996) Ročník 526; s. 170795 |
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| Hlavní autoři: | , , , , , |
| Médium: | Journal Article |
| Jazyk: | angličtina |
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Elsevier B.V
15.12.2025
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| Témata: | |
| ISSN: | 1385-8947 |
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| Abstract | Scalable and sustainable solar-driven interfacial evaporators are vital to addressing global freshwater scarcity and sustainability challenges. However, the applicability of biomass-based evaporators is often limited by costly and complex fabrication processes. Here, we report a high-performance rattan-based solar evaporator fabricated via a one-step laser-induced carbonization process. This direct approach creates a multi-dimensional hierarchical light-harvesting layer with a pronounced 3D periodic protrusion array, achieving a high solar absorptance of 88.32 %. This structure significantly enhances evaporation by increasing the effective evaporation area, promoting omnidirectional vapor escape and inducing dual Marangoni flows that facilitate liquid circulation and salt backflow. The evaporator achieves a high energy conversion efficiency of 95.32 % and water evaporation rate of 1.80 kg·m−2·h−1 in simulated seawater, with a significant reduction in evaporation latent heat to 1.62 MJ·kg−1, outperforming many previously reported carbon- or bio-based evaporators. Integrated into a closed-loop desalination-cultivation system, the generated freshwater supports wheat cultivation over an area 3 times larger than the evaporation surface, yielding plant growth comparable to tap water irrigation. Life cycle assessment reveals the rattan-based evaporator produces over two orders of magnitude lower CO2-equivalent emissions and substantially reduces overall environmental impacts compared to conventional solar evaporators. This work demonstrates a scalable and environmentally friendly strategy to transform natural biomass into high-performance sustainable solar evaporators, advancing decentralized water-food solutions under resource-constrained conditions.
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•CO2 laser-carbonized rattan enables efficient, scalable solar desalination.•Natural rattan microchannels enable fast water transport and salt backflow.•Multi-dimensional light harvest enhanced efficiency without extra energy input.•3D periodic protrusion array induces dual-Marangoni flow sustaining salt-rejection.•Freshwater generation for low-carbon closed-loop desalination-cultivation system. |
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| AbstractList | Scalable and sustainable solar-driven interfacial evaporators are vital to addressing global freshwater scarcity and sustainability challenges. However, the applicability of biomass-based evaporators is often limited by costly and complex fabrication processes. Here, we report a high-performance rattan-based solar evaporator fabricated via a one-step laser-induced carbonization process. This direct approach creates a multi-dimensional hierarchical light-harvesting layer with a pronounced 3D periodic protrusion array, achieving a high solar absorptance of 88.32 %. This structure significantly enhances evaporation by increasing the effective evaporation area, promoting omnidirectional vapor escape and inducing dual Marangoni flows that facilitate liquid circulation and salt backflow. The evaporator achieves a high energy conversion efficiency of 95.32 % and water evaporation rate of 1.80 kg·m−2·h−1 in simulated seawater, with a significant reduction in evaporation latent heat to 1.62 MJ·kg−1, outperforming many previously reported carbon- or bio-based evaporators. Integrated into a closed-loop desalination-cultivation system, the generated freshwater supports wheat cultivation over an area 3 times larger than the evaporation surface, yielding plant growth comparable to tap water irrigation. Life cycle assessment reveals the rattan-based evaporator produces over two orders of magnitude lower CO2-equivalent emissions and substantially reduces overall environmental impacts compared to conventional solar evaporators. This work demonstrates a scalable and environmentally friendly strategy to transform natural biomass into high-performance sustainable solar evaporators, advancing decentralized water-food solutions under resource-constrained conditions.
[Display omitted]
•CO2 laser-carbonized rattan enables efficient, scalable solar desalination.•Natural rattan microchannels enable fast water transport and salt backflow.•Multi-dimensional light harvest enhanced efficiency without extra energy input.•3D periodic protrusion array induces dual-Marangoni flow sustaining salt-rejection.•Freshwater generation for low-carbon closed-loop desalination-cultivation system. |
| ArticleNumber | 170795 |
| Author | Woon, Pei Qi Liu, Yingpeng Li, Bofan Xu, Xinwu Xu, Haocheng Chen, Meiling |
| Author_xml | – sequence: 1 givenname: Haocheng surname: Xu fullname: Xu, Haocheng organization: Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, College of Materials Science and Engineering, Nanjing Forestry University, Jiangsu, 210037, China – sequence: 2 givenname: Yingpeng surname: Liu fullname: Liu, Yingpeng organization: Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, College of Materials Science and Engineering, Nanjing Forestry University, Jiangsu, 210037, China – sequence: 3 givenname: Pei Qi surname: Woon fullname: Woon, Pei Qi organization: Institute of Sustainability for Chemicals, Energy and Environment (ISCE2), Agency for Science, Technology, and Research (ASTAR), Singapore, 627833, Singapore – sequence: 4 givenname: Meiling surname: Chen fullname: Chen, Meiling email: meiling_chen@njfu.edu.cn organization: Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, College of Materials Science and Engineering, Nanjing Forestry University, Jiangsu, 210037, China – sequence: 5 givenname: Xinwu surname: Xu fullname: Xu, Xinwu email: xucarpenter@njfu.edu.cn organization: Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, College of Materials Science and Engineering, Nanjing Forestry University, Jiangsu, 210037, China – sequence: 6 givenname: Bofan surname: Li fullname: Li, Bofan email: li_bofan@a-star.edu.sg organization: Institute of Sustainability for Chemicals, Energy and Environment (ISCE2), Agency for Science, Technology, and Research (ASTAR), Singapore, 627833, Singapore |
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| Keywords | Biomass-based evaporator Solar-driven interfacial evaporation Rattan Laser-induced carbonization Low-carbon desalination |
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