Tailoring multifunctionality in coaxial twisted inorganic-organic core-shell yarns via composite design principles
Intelligent fabrics boasting capabilities in health protection, motion monitoring, and sensing play a pivotal role in advancing smart health management. However, achieving multifunctionality and mechanical robustness while ensuring sustainability remains a persistent challenge. Here, a biomimetic or...
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| Veröffentlicht in: | Chemical engineering journal (Lausanne, Switzerland : 1996) Jg. 525; S. 170458 |
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| Format: | Journal Article |
| Sprache: | Englisch |
| Veröffentlicht: |
Elsevier B.V
01.12.2025
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| ISSN: | 1385-8947 |
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| Abstract | Intelligent fabrics boasting capabilities in health protection, motion monitoring, and sensing play a pivotal role in advancing smart health management. However, achieving multifunctionality and mechanical robustness while ensuring sustainability remains a persistent challenge. Here, a biomimetic organic-inorganic strategy is proposed to develop a yarn with a coaxial multi-layer winding structure. It integrates high-strength basalt filament (BF) with degradable cotton slivers (CS), functionalized via a dynamic hydrogen-bonded epoxy soybean oil-based polymer. Leveraging the synergistic hydrogen-bonding interactions and coaxial winding structure, functional particles are stably incorporated into the yarn, endowing it with high tensile strength (182.84 MPa), remarkable impact resistance (85 % ± 1.2 % impact force attenuation), adjustable fluorescence for damage visualization, and self-healing capacity via reversible hydrogen bonds. Additionally, it exhibits biodegradability (12.7 % strength loss after 8 days) and component recyclability. When integrated into wearable systems, the yarn enables sensitive perception of environmental safety and real-time human health monitoring. This research effectively addresses the long-standing dilemma of balancing multifunctionality and environment sustainability in intelligent textiles, providing novel insights for developing next-generation advanced wearable multifunctional protective smart fabrics.
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•Bioinspired organic-inorganic composite yarns with coaxial twisted structures•Biodegradable bio-based composite fiber system with dynamically reversible crosslinking networks•High mechanical properties (tensile strength: 182.84 MPa; attenuate >80 % of impact force)•Having cluster luminescence effect and can autonomous self-healing•Wireless-enabled intelligent protection fabric sensor for real-time perception monitoring |
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| AbstractList | Intelligent fabrics boasting capabilities in health protection, motion monitoring, and sensing play a pivotal role in advancing smart health management. However, achieving multifunctionality and mechanical robustness while ensuring sustainability remains a persistent challenge. Here, a biomimetic organic-inorganic strategy is proposed to develop a yarn with a coaxial multi-layer winding structure. It integrates high-strength basalt filament (BF) with degradable cotton slivers (CS), functionalized via a dynamic hydrogen-bonded epoxy soybean oil-based polymer. Leveraging the synergistic hydrogen-bonding interactions and coaxial winding structure, functional particles are stably incorporated into the yarn, endowing it with high tensile strength (182.84 MPa), remarkable impact resistance (85 % ± 1.2 % impact force attenuation), adjustable fluorescence for damage visualization, and self-healing capacity via reversible hydrogen bonds. Additionally, it exhibits biodegradability (12.7 % strength loss after 8 days) and component recyclability. When integrated into wearable systems, the yarn enables sensitive perception of environmental safety and real-time human health monitoring. This research effectively addresses the long-standing dilemma of balancing multifunctionality and environment sustainability in intelligent textiles, providing novel insights for developing next-generation advanced wearable multifunctional protective smart fabrics.
[Display omitted]
•Bioinspired organic-inorganic composite yarns with coaxial twisted structures•Biodegradable bio-based composite fiber system with dynamically reversible crosslinking networks•High mechanical properties (tensile strength: 182.84 MPa; attenuate >80 % of impact force)•Having cluster luminescence effect and can autonomous self-healing•Wireless-enabled intelligent protection fabric sensor for real-time perception monitoring |
| ArticleNumber | 170458 |
| Author | Wang, Zihao Lavorgna, Marino Yang, Pengcheng Liu, Jize Lv, Kun Wu, Guilin Lei, Mengdie Hu, Jiaman Cai, Guangming |
| Author_xml | – sequence: 1 givenname: Mengdie surname: Lei fullname: Lei, Mengdie organization: State Key Laboratory of New Textile Materials and Advanced Processing Technologies & School of Textile Science and Engineering, Wuhan Textile University, Wuhan, 430200, China – sequence: 2 givenname: Jiaman surname: Hu fullname: Hu, Jiaman organization: School of Materials Science and Engineering, Hainan University, Haikou, 570228, China – sequence: 3 givenname: Guilin surname: Wu fullname: Wu, Guilin organization: State Key Laboratory of New Textile Materials and Advanced Processing Technologies & School of Textile Science and Engineering, Wuhan Textile University, Wuhan, 430200, China – sequence: 4 givenname: Zihao surname: Wang fullname: Wang, Zihao organization: School of Materials Science and Engineering, Hainan University, Haikou, 570228, China – sequence: 5 givenname: Kun surname: Lv fullname: Lv, Kun organization: School of Materials Science and Engineering, Hainan University, Haikou, 570228, China – sequence: 6 givenname: Pengcheng surname: Yang fullname: Yang, Pengcheng organization: Institute of Polymers, Composites and Biomaterials, National Research Council of Italy, 80055, Portici, NA, Italy – sequence: 7 givenname: Marino surname: Lavorgna fullname: Lavorgna, Marino organization: Institute of Polymers, Composites and Biomaterials, National Research Council of Italy, 80055, Portici, NA, Italy – sequence: 8 givenname: Jize surname: Liu fullname: Liu, Jize email: ljz@hainanu.edu.cn organization: School of Materials Science and Engineering, Hainan University, Haikou, 570228, China – sequence: 9 givenname: Guangming surname: Cai fullname: Cai, Guangming email: guangmingcai2006@163.com organization: State Key Laboratory of New Textile Materials and Advanced Processing Technologies & School of Textile Science and Engineering, Wuhan Textile University, Wuhan, 430200, China |
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| Keywords | Coaxial multi-layered wrapping Bionic structure Intelligent sensing Organic-inorganic composite yarn Bio-based materials |
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