Effects of Inorganic Fillers on the Thermal and Mechanical Properties of Poly(lactic acid)

Addition of filler to polylactic acid (PLA) may affect its crystallization behavior and mechanical properties. The effects of talc and hydroxyapatite (HA) on the thermal and mechanical properties of two types of PLA (one amorphous and one semicrystalline) have been investigated. The composites were...

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Vydáno v:International Journal of Polymer Science Ročník 2014; číslo 2; s. 129 - 136
Hlavní autoři: Yang, Mingshu, Chow, Laurence C., Wang, Tongxin, Liu, Xingxun, Mitchell, James W.
Médium: Journal Article
Jazyk:angličtina
Vydáno: Cairo, Egypt Hindawi Limiteds 01.01.2014
Hindawi Publishing Corporation
John Wiley & Sons, Inc
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ISSN:1687-9422, 1687-9430
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Abstract Addition of filler to polylactic acid (PLA) may affect its crystallization behavior and mechanical properties. The effects of talc and hydroxyapatite (HA) on the thermal and mechanical properties of two types of PLA (one amorphous and one semicrystalline) have been investigated. The composites were prepared by melt blending followed by injection molding. The molecular weight, morphology, mechanical properties, and thermal properties have been characterized by gel permeation chromatography (GPC), scanning electron microscope (SEM), instron tensile tester, thermogravimetric analysis (TGA), differential scanning calorimetry (DSC), and dynamic mechanical analysis (DMA). It was found that the melting blending led to homogeneous distribution of the inorganic filler within the PLA matrix but decreased the molecular weight of PLA. Regarding the filler, addition of talc increased the crystallinity of PLA, but HA decreased the crystallinity of PLA. The tensile strength of the composites depended on the crystallinity of PLA and the interfacial properties between PLA and the filler, but both talc and HA filler increased the toughness of PLA.
AbstractList Addition of filler to polylactic acid (PLA) may affect its crystallization behavior and mechanical properties. The effects of talc and hydroxyapatite (HA) on the thermal and mechanical properties of two types of PLA (one amorphous and one semicrystalline) have been investigated. The composites were prepared by melt blending followed by injection molding. The molecular weight, morphology, mechanical properties, and thermal properties have been characterized by gel permeation chromatography (GPC), scanning electron microscope (SEM), instron tensile tester, thermogravimetric analysis (TGA), differential scanning calorimetry (DSC), and dynamic mechanical analysis (DMA). It was found that the melting blending led to homogeneous distribution of the inorganic filler within the PLA matrix but decreased the molecular weight of PLA. Regarding the filler, addition of talc increased the crystallinity of PLA, but HA decreased the crystallinity of PLA. The tensile strength of the composites depended on the crystallinity of PLA and the interfacial properties between PLA and the filler, but both talc and HA filler increased the toughness of PLA.
Addition of filler to polylactic acid (PLA) may affect its crystallization behavior and mechanical properties. The effects of talc and hydroxyapatite (HA) on the thermal and mechanical properties of two types of PLA (one amorphous and one semicrystalline) have been investigated. The composites were prepared by melt blending followed by injection molding. The molecular weight, morphology, mechanical properties, and thermal properties have been characterized by gel permeation chromatography (GPC), scanning electron microscope (SEM), instron tensile tester, thermogravimetric analysis (TGA), differential scanning calorimetry (DSC), and dynamic mechanical analysis (DMA). It was found that the melting blending led to homogeneous distribution of the inorganic filler within the PLA matrix but decreased the molecular weight of PLA. Regarding the filler, addition of talc increased the crystallinity of PLA, but HA decreased the crystallinity of PLA. The tensile strength of the composites depended on the crystallinity of PLA and the interfacial properties between PLA and the filler, but both talc and HA filler increased the toughness of PLA.Addition of filler to polylactic acid (PLA) may affect its crystallization behavior and mechanical properties. The effects of talc and hydroxyapatite (HA) on the thermal and mechanical properties of two types of PLA (one amorphous and one semicrystalline) have been investigated. The composites were prepared by melt blending followed by injection molding. The molecular weight, morphology, mechanical properties, and thermal properties have been characterized by gel permeation chromatography (GPC), scanning electron microscope (SEM), instron tensile tester, thermogravimetric analysis (TGA), differential scanning calorimetry (DSC), and dynamic mechanical analysis (DMA). It was found that the melting blending led to homogeneous distribution of the inorganic filler within the PLA matrix but decreased the molecular weight of PLA. Regarding the filler, addition of talc increased the crystallinity of PLA, but HA decreased the crystallinity of PLA. The tensile strength of the composites depended on the crystallinity of PLA and the interfacial properties between PLA and the filler, but both talc and HA filler increased the toughness of PLA.
Audience Academic
Author Liu, Xingxun
Mitchell, James W.
Chow, Laurence C.
Yang, Mingshu
Wang, Tongxin
AuthorAffiliation 2 Crest Center for Nanomaterials, College of Engineering, Howard University, Washington, DC 20059, USA
1 College of Dentistry, Howard University, Washington, DC 20059, USA
4 CAS Key Laboratory of Engineering Plastics, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China
3 American Dental Association Foundation, Dr. Anthony Volpe Research Center, National Institute of Standards and Technology, Gaithersburg, MD 20899, USA
AuthorAffiliation_xml – name: 2 Crest Center for Nanomaterials, College of Engineering, Howard University, Washington, DC 20059, USA
– name: 1 College of Dentistry, Howard University, Washington, DC 20059, USA
– name: 4 CAS Key Laboratory of Engineering Plastics, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China
– name: 3 American Dental Association Foundation, Dr. Anthony Volpe Research Center, National Institute of Standards and Technology, Gaithersburg, MD 20899, USA
Author_xml – sequence: 1
  fullname: Yang, Mingshu
– sequence: 2
  fullname: Chow, Laurence C.
– sequence: 3
  fullname: Wang, Tongxin
– sequence: 4
  fullname: Liu, Xingxun
– sequence: 5
  fullname: Mitchell, James W.
BackLink https://www.ncbi.nlm.nih.gov/pubmed/25717339$$D View this record in MEDLINE/PubMed
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ContentType Journal Article
Copyright Copyright © 2014 Xingxun Liu et al.
COPYRIGHT 2014 John Wiley & Sons, Inc.
Copyright © 2014 Xingxun Liu et al. Xingxun Liu et al. This is an open access article distributed under the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.
Copyright © 2014 Xingxun Liu et al. 2014
Copyright_xml – notice: Copyright © 2014 Xingxun Liu et al.
– notice: COPYRIGHT 2014 John Wiley & Sons, Inc.
– notice: Copyright © 2014 Xingxun Liu et al. Xingxun Liu et al. This is an open access article distributed under the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.
– notice: Copyright © 2014 Xingxun Liu et al. 2014
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Snippet Addition of filler to polylactic acid (PLA) may affect its crystallization behavior and mechanical properties. The effects of talc and hydroxyapatite (HA) on...
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StartPage 129
SubjectTerms Annealing
Colleges & universities
Crystallinity
Crystallization
Differential scanning calorimetry
Fillers
Hydroxyapatite
Mechanical properties
Methods
Molecular weight
Phase transitions
Polyesters
Polylactic acid
Scanning electron microscopy
Talcs
Tensile strength
Thermal properties
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Title Effects of Inorganic Fillers on the Thermal and Mechanical Properties of Poly(lactic acid)
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