A microarray immunoassay for simultaneous detection of proteins and bacteria

We report the development and characterization of an antibody microarray biosensor for the rapid detection of both protein and bacterial analytes under flow conditions. Using a noncontact microarray printer, biotinylated capture antibodies were immobilized at discrete locations on the surface of an...

Full description

Saved in:
Bibliographic Details
Published in:Analytical chemistry (Washington) Vol. 74; no. 21; p. 5681
Main Authors: Delehanty, James B, Ligler, Frances S
Format: Journal Article
Language:English
Published: United States 01.11.2002
Subjects:
ISSN:0003-2700
Online Access:Get more information
Tags: Add Tag
No Tags, Be the first to tag this record!
Abstract We report the development and characterization of an antibody microarray biosensor for the rapid detection of both protein and bacterial analytes under flow conditions. Using a noncontact microarray printer, biotinylated capture antibodies were immobilized at discrete locations on the surface of an avidin-coated glass microscope slide. Preservation of capture antibody function during the deposition process was accomplished with the use of a low-salt buffer containing sucrose and bovine serum albumin. The slide was fitted with a six-channel flow module that conducted analyte-containing solutions over the array of capture antibody microspots. Detection of bound analyte was subsequently achieved using fluorescent tracer antibodies. The pattern of fluorescent complexes was interrogated using a scanning confocal microscope equipped with a 635-nm laser. This microarray system was employed to detect protein and bacterial analytes both individually and in samples containing mixtures of analytes. Assays were completed in 15 min, and detection of cholera toxin, staphylococcal enterotoxin B, ricin, and Bacillus globigii was demonstrated at levels as low as 8 ng/mL, 4 ng/mL, 10 ng/mL, and 6.2 x 10(4) cfu/mL, respectively. The assays presented here are very fast, as compared to previously published methods for measuring antibody-antigen interactions using microarrays (minutes versus hours).
AbstractList We report the development and characterization of an antibody microarray biosensor for the rapid detection of both protein and bacterial analytes under flow conditions. Using a noncontact microarray printer, biotinylated capture antibodies were immobilized at discrete locations on the surface of an avidin-coated glass microscope slide. Preservation of capture antibody function during the deposition process was accomplished with the use of a low-salt buffer containing sucrose and bovine serum albumin. The slide was fitted with a six-channel flow module that conducted analyte-containing solutions over the array of capture antibody microspots. Detection of bound analyte was subsequently achieved using fluorescent tracer antibodies. The pattern of fluorescent complexes was interrogated using a scanning confocal microscope equipped with a 635-nm laser. This microarray system was employed to detect protein and bacterial analytes both individually and in samples containing mixtures of analytes. Assays were completed in 15 min, and detection of cholera toxin, staphylococcal enterotoxin B, ricin, and Bacillus globigii was demonstrated at levels as low as 8 ng/mL, 4 ng/mL, 10 ng/mL, and 6.2 x 10(4) cfu/mL, respectively. The assays presented here are very fast, as compared to previously published methods for measuring antibody-antigen interactions using microarrays (minutes versus hours).
We report the development and characterization of an antibody microarray biosensor for the rapid detection of both protein and bacterial analytes under flow conditions. Using a noncontact microarray printer, biotinylated capture antibodies were immobilized at discrete locations on the surface of an avidin-coated glass microscope slide. Preservation of capture antibody function during the deposition process was accomplished with the use of a low-salt buffer containing sucrose and bovine serum albumin. The slide was fitted with a six-channel flow module that conducted analyte-containing solutions over the array of capture antibody microspots. Detection of bound analyte was subsequently achieved using fluorescent tracer antibodies. The pattern of fluorescent complexes was interrogated using a scanning confocal microscope equipped with a 635-nm laser. This microarray system was employed to detect protein and bacterial analytes both individually and in samples containing mixtures of analytes. Assays were completed in 15 min, and detection of cholera toxin, staphylococcal enterotoxin B, ricin, and Bacillus globigii was demonstrated at levels as low as 8 ng/mL, 4 ng/mL, 10 ng/mL, and 6.2 x 10(4) cfu/mL, respectively. The assays presented here are very fast, as compared to previously published methods for measuring antibody-antigen interactions using microarrays (minutes versus hours).We report the development and characterization of an antibody microarray biosensor for the rapid detection of both protein and bacterial analytes under flow conditions. Using a noncontact microarray printer, biotinylated capture antibodies were immobilized at discrete locations on the surface of an avidin-coated glass microscope slide. Preservation of capture antibody function during the deposition process was accomplished with the use of a low-salt buffer containing sucrose and bovine serum albumin. The slide was fitted with a six-channel flow module that conducted analyte-containing solutions over the array of capture antibody microspots. Detection of bound analyte was subsequently achieved using fluorescent tracer antibodies. The pattern of fluorescent complexes was interrogated using a scanning confocal microscope equipped with a 635-nm laser. This microarray system was employed to detect protein and bacterial analytes both individually and in samples containing mixtures of analytes. Assays were completed in 15 min, and detection of cholera toxin, staphylococcal enterotoxin B, ricin, and Bacillus globigii was demonstrated at levels as low as 8 ng/mL, 4 ng/mL, 10 ng/mL, and 6.2 x 10(4) cfu/mL, respectively. The assays presented here are very fast, as compared to previously published methods for measuring antibody-antigen interactions using microarrays (minutes versus hours).
Author Delehanty, James B
Ligler, Frances S
Author_xml – sequence: 1
  givenname: James B
  surname: Delehanty
  fullname: Delehanty, James B
  organization: Center for Bio/Molecular Science & Engineering, Naval Research Laboratory, Washington, DC 20375-5348, USA
– sequence: 2
  givenname: Frances S
  surname: Ligler
  fullname: Ligler, Frances S
BackLink https://www.ncbi.nlm.nih.gov/pubmed/12433105$$D View this record in MEDLINE/PubMed
BookMark eNo1jz1PwzAURT0U0Q8Y-APIE1vg2Y7tZKwqKEiVWGCOHOdFMortYjtD_z2VWqZ7h6Orc9dkEWJAQh4YPDPg7MVY4FIJNi3ICgBExTXAkqxz_gFgDJi6JUvGayEYyBU5bKl3NkWTkjlR5_0cosn53MeYaHZ-nooJGOdMByxoi4uBxpEeUyzoQqYmDLQ3tmBy5o7cjGbKeH_NDfl-e_3avVeHz_3HbnuojBRQqkGOCtrGMCXqXom2rW2jGui1tmgE6tooVJoJy_qxASu1aMSo6kFqpZgdkG_I02X3bPE7Yy6dd9niNF1MO81V02ouz-DjFZx7j0N3TM6bdOr-__M_Pb9buA
CitedBy_id crossref_primary_10_1002_adhm_202100877
crossref_primary_10_1016_j_bios_2014_08_039
crossref_primary_10_1016_j_jelechem_2017_10_064
crossref_primary_10_1016_j_mimet_2007_11_004
crossref_primary_10_1016_j_talanta_2020_121174
crossref_primary_10_1002_smll_201801893
crossref_primary_10_3390_ijms26125641
crossref_primary_10_1016_j_aca_2008_12_035
crossref_primary_10_1016_j_aca_2010_05_017
crossref_primary_10_1016_j_aca_2005_12_038
crossref_primary_10_3390_su141912844
crossref_primary_10_1016_j_ab_2005_09_033
crossref_primary_10_1016_j_ab_2005_10_033
crossref_primary_10_1373_clinchem_2007_086975
crossref_primary_10_1021_ja210350d
crossref_primary_10_1016_j_jchromb_2009_08_038
crossref_primary_10_1016_j_bios_2020_112279
crossref_primary_10_1016_j_foodcont_2012_01_047
crossref_primary_10_1016_j_tsf_2006_10_060
crossref_primary_10_3390_s120202324
crossref_primary_10_1371_journal_pone_0068918
crossref_primary_10_1016_j_bios_2014_02_012
crossref_primary_10_1021_ja302970x
crossref_primary_10_1016_j_aca_2005_03_073
crossref_primary_10_1016_j_bios_2004_04_007
crossref_primary_10_1002_pmic_200300609
crossref_primary_10_1080_03067310903029822
crossref_primary_10_1080_08923970902740837
crossref_primary_10_1038_s41598_020_65563_3
crossref_primary_10_1366_00037020360696008
crossref_primary_10_1002_tpg2_70027
crossref_primary_10_3390_s17020256
crossref_primary_10_3724_SP_J_1123_2020_10001
crossref_primary_10_1007_s00216_006_0672_2
crossref_primary_10_1016_j_bios_2007_03_023
crossref_primary_10_1016_j_bios_2013_07_067
crossref_primary_10_1586_14737159_4_6_841
crossref_primary_10_1021_ja044539z
crossref_primary_10_2116_analsci_23_5
crossref_primary_10_1016_j_aca_2013_02_041
crossref_primary_10_1007_s00216_006_0574_3
crossref_primary_10_3390_s141222313
crossref_primary_10_1007_s42242_024_00285_3
crossref_primary_10_1007_s00216_008_2062_4
crossref_primary_10_1371_journal_pone_0225525
crossref_primary_10_1016_j_memsci_2006_02_009
crossref_primary_10_1016_j_tibtech_2005_02_004
crossref_primary_10_1111_j_1742_4658_2010_07626_x
crossref_primary_10_1016_j_chroma_2006_08_078
crossref_primary_10_1093_chromsci_bmw167
crossref_primary_10_1016_j_bios_2022_113991
crossref_primary_10_1007_s00216_015_8992_8
crossref_primary_10_1016_j_bios_2005_12_018
crossref_primary_10_1016_j_bios_2004_09_037
crossref_primary_10_1039_c0ja00232a
crossref_primary_10_1016_j_aca_2007_08_033
crossref_primary_10_1088_0957_4484_22_42_425502
crossref_primary_10_1016_j_proenv_2011_10_040
crossref_primary_10_1016_j_snb_2017_08_180
crossref_primary_10_4315_0362_028X_70_4_841
crossref_primary_10_1007_s10404_009_0422_9
crossref_primary_10_1016_j_aca_2007_08_029
crossref_primary_10_1016_j_microc_2006_02_005
crossref_primary_10_1002_pmic_200300705
crossref_primary_10_1016_j_bios_2014_08_063
crossref_primary_10_3390_molecules28062863
crossref_primary_10_3390_s121115467
crossref_primary_10_1016_j_foodcont_2019_106885
crossref_primary_10_1016_S1535_6108_03_00086_2
crossref_primary_10_1039_D2RA01788A
crossref_primary_10_1016_j_biomaterials_2006_11_007
crossref_primary_10_1002_jmr_625
crossref_primary_10_1016_j_bios_2004_10_016
crossref_primary_10_1016_j_ejca_2004_05_020
crossref_primary_10_1002_smll_200902406
crossref_primary_10_1002_elps_200500489
crossref_primary_10_1517_14728222_9_6_1189
crossref_primary_10_1038_s41598_020_75285_1
crossref_primary_10_1007_s10439_019_02256_7
crossref_primary_10_1016_j_bios_2005_01_013
crossref_primary_10_1016_j_bios_2011_07_045
crossref_primary_10_1016_j_snb_2011_02_035
crossref_primary_10_1016_j_bios_2008_04_019
crossref_primary_10_1586_14789450_2_1_41
crossref_primary_10_1002_anie_201411508
crossref_primary_10_1016_j_ab_2005_01_042
crossref_primary_10_1007_s00216_010_3990_3
crossref_primary_10_1517_17460441_2_7_961
crossref_primary_10_21300_19_3_2018_645
crossref_primary_10_1016_j_bios_2004_04_016
crossref_primary_10_1128_CMR_18_4_583_607_2005
crossref_primary_10_1002_adma_200501129
crossref_primary_10_1046_j_1365_2672_2003_02115_x
crossref_primary_10_1016_j_bios_2004_10_026
crossref_primary_10_1128_iai_00411_25
crossref_primary_10_1016_j_ab_2005_01_030
crossref_primary_10_1002_ange_201411508
crossref_primary_10_1007_s12033_007_0066_5
crossref_primary_10_1039_c000316f
crossref_primary_10_3390_s90604407
crossref_primary_10_3390_s90604804
crossref_primary_10_1373_clinchem_2004_037929
crossref_primary_10_1039_c3cs60141b
crossref_primary_10_1146_annurev_anchem_061010_114010
crossref_primary_10_1007_s11356_015_5758_y
crossref_primary_10_1016_j_snb_2008_06_043
crossref_primary_10_1134_S1068162009030078
crossref_primary_10_1016_j_bios_2010_12_040
crossref_primary_10_1128_JCM_43_7_3427_3430_2005
crossref_primary_10_1146_annurev_anchem_1_031207_112826
crossref_primary_10_1002_pmic_200300592
crossref_primary_10_1016_j_aca_2006_04_083
crossref_primary_10_1002_pmic_200300599
crossref_primary_10_1016_S0958_1669_03_00057_0
crossref_primary_10_1016_j_snb_2018_01_115
crossref_primary_10_3390_s22228606
crossref_primary_10_1016_j_aca_2011_08_011
crossref_primary_10_1007_s00216_008_2559_x
crossref_primary_10_1002_dta_27
crossref_primary_10_1351_pac200476040723
crossref_primary_10_1586_14789450_4_1_91
crossref_primary_10_3390_s120709234
crossref_primary_10_1007_s00253_006_0312_y
crossref_primary_10_1016_j_aca_2007_04_019
crossref_primary_10_1128_AEM_69_9_5212_5215_2003
crossref_primary_10_1016_j_ijpharm_2015_02_033
crossref_primary_10_1039_c2an35279f
crossref_primary_10_1016_j_jim_2004_04_013
crossref_primary_10_1039_c3cc45370g
crossref_primary_10_1016_j_biomaterials_2013_10_077
crossref_primary_10_2134_agronj2011_0210
crossref_primary_10_1016_j_jim_2006_01_007
crossref_primary_10_1016_j_microc_2015_07_007
crossref_primary_10_1002_bit_20401
crossref_primary_10_1016_j_snb_2004_08_034
crossref_primary_10_1016_j_biomaterials_2004_03_014
crossref_primary_10_1016_S1001_0742_09_60034_6
crossref_primary_10_1128_AEM_70_1_152_158_2004
crossref_primary_10_1007_s00216_010_3678_8
crossref_primary_10_1016_j_talanta_2010_03_052
crossref_primary_10_1080_03602530500205309
crossref_primary_10_1016_j_foodcont_2013_11_038
crossref_primary_10_1155_2023_5510791
crossref_primary_10_1373_clinchem_2003_029850
crossref_primary_10_1016_j_biotechadv_2014_11_012
crossref_primary_10_1007_s00216_008_2044_6
crossref_primary_10_1016_j_ab_2006_05_003
crossref_primary_10_1016_j_aca_2005_12_020
crossref_primary_10_1016_j_colsurfb_2007_06_018
crossref_primary_10_1007_s11095_010_0325_1
crossref_primary_10_1016_j_talanta_2014_08_001
crossref_primary_10_3390_molecules25225256
crossref_primary_10_1002_bit_21104
crossref_primary_10_1016_j_bios_2006_04_010
crossref_primary_10_1016_j_cocis_2023_101718
crossref_primary_10_1002_elps_200405888
crossref_primary_10_1016_j_snb_2017_10_017
crossref_primary_10_1517_14712598_4_1_83
crossref_primary_10_1089_nat_2012_0377
crossref_primary_10_1002_elps_200800297
crossref_primary_10_1109_JSEN_2005_848121
crossref_primary_10_3390_mi11080739
crossref_primary_10_1016_j_bios_2006_06_005
crossref_primary_10_1016_j_chroma_2007_01_046
crossref_primary_10_1007_s00705_021_04962_x
crossref_primary_10_1155_2024_4454744
ContentType Journal Article
Contributor Ligler, F S
Contributor_xml – sequence: 1
  givenname: F S
  surname: Ligler
  fullname: Ligler, F S
  organization: Naval Res Lab, Washington, DC
DBID CGR
CUY
CVF
ECM
EIF
NPM
7X8
DOI 10.1021/ac025631l
DatabaseName Medline
MEDLINE
MEDLINE (Ovid)
MEDLINE
MEDLINE
PubMed
MEDLINE - Academic
DatabaseTitle MEDLINE
Medline Complete
MEDLINE with Full Text
PubMed
MEDLINE (Ovid)
MEDLINE - Academic
DatabaseTitleList MEDLINE
MEDLINE - Academic
Database_xml – sequence: 1
  dbid: NPM
  name: PubMed
  url: http://www.ncbi.nlm.nih.gov/entrez/query.fcgi?db=PubMed
  sourceTypes: Index Database
– sequence: 2
  dbid: 7X8
  name: MEDLINE - Academic
  url: https://search.proquest.com/medline
  sourceTypes: Aggregation Database
DeliveryMethod no_fulltext_linktorsrc
Discipline Engineering
Chemistry
ExternalDocumentID 12433105
Genre Research Support, U.S. Gov't, Non-P.H.S
Research Support, Non-U.S. Gov't
Journal Article
GroupedDBID ---
-DZ
-~X
.DC
.GJ
.K2
186
23M
3EH
3O-
4.4
53G
55A
5GY
5RE
5VS
6J9
6TJ
7~N
85S
AABXI
AAHBH
AAUTI
ABDEX
ABHFT
ABHMW
ABJNI
ABMVS
ABOCM
ABPPZ
ABQRX
ABUCX
ACBEA
ACGFO
ACGFS
ACGOD
ACIWK
ACJ
ACKIV
ACKOT
ACNCT
ACPRK
ACPVT
ACRPL
ACS
ADHLV
ADNMO
AEESW
AENEX
AEYZD
AFEFF
AFFDN
AFFNX
AFRAH
AGXLV
AHGAQ
AIDAL
ALMA_UNASSIGNED_HOLDINGS
ANPPW
ANTXH
AQSVZ
BAANH
BKOMP
CGR
CS3
CUPRZ
CUY
CVF
D0L
EBS
ECM
ED~
EIF
EJD
F5P
GGK
GNL
IH9
IHE
JG~
KZ1
LG6
NHB
NPM
OHT
P2P
PQQKQ
ROL
RXW
TAE
TN5
UHB
UI2
UKR
VF5
VG9
VOH
VQA
VXZ
W1F
WH7
X6Y
XOL
XSW
YIN
YR5
YYP
YZZ
ZCA
ZCG
ZGI
~02
7X8
ABBLG
ABLBI
ABUFD
ADXHL
AETEA
AGQPQ
ID FETCH-LOGICAL-a530t-d5f6098a1634b63994c8680b77cea3e74a6e6713c1bf80c57383f64d57661cde2
IEDL.DBID 7X8
ISICitedReferencesCount 272
ISICitedReferencesURI http://www.webofscience.com/api/gateway?GWVersion=2&SrcApp=Summon&SrcAuth=ProQuest&DestLinkType=CitingArticles&DestApp=WOS_CPL&KeyUT=000179028300039&url=https%3A%2F%2Fcvtisr.summon.serialssolutions.com%2F%23%21%2Fsearch%3Fho%3Df%26include.ft.matches%3Dt%26l%3Dnull%26q%3D
ISSN 0003-2700
IngestDate Sun Nov 09 10:41:32 EST 2025
Wed Feb 19 02:36:44 EST 2025
IsPeerReviewed true
IsScholarly true
Issue 21
Keywords NASA Discipline Life Sciences Technologies
Non-NASA Center
Language English
LinkModel DirectLink
MergedId FETCHMERGED-LOGICAL-a530t-d5f6098a1634b63994c8680b77cea3e74a6e6713c1bf80c57383f64d57661cde2
Notes ObjectType-Article-1
SourceType-Scholarly Journals-1
ObjectType-Feature-2
content type line 23
PMID 12433105
PQID 72689725
PQPubID 23479
ParticipantIDs proquest_miscellaneous_72689725
pubmed_primary_12433105
PublicationCentury 2000
PublicationDate 2002-11-01
PublicationDateYYYYMMDD 2002-11-01
PublicationDate_xml – month: 11
  year: 2002
  text: 2002-11-01
  day: 01
PublicationDecade 2000
PublicationPlace United States
PublicationPlace_xml – name: United States
PublicationTitle Analytical chemistry (Washington)
PublicationTitleAlternate Anal Chem
PublicationYear 2002
SSID ssj0011016
Score 2.2359898
Snippet We report the development and characterization of an antibody microarray biosensor for the rapid detection of both protein and bacterial analytes under flow...
SourceID proquest
pubmed
SourceType Aggregation Database
Index Database
StartPage 5681
SubjectTerms Animals
Bacteria - isolation & purification
Biosensing Techniques - methods
Immunoassay - methods
Microscopy, Confocal
Protein Array Analysis - instrumentation
Protein Array Analysis - methods
Proteins - analysis
Title A microarray immunoassay for simultaneous detection of proteins and bacteria
URI https://www.ncbi.nlm.nih.gov/pubmed/12433105
https://www.proquest.com/docview/72689725
Volume 74
WOSCitedRecordID wos000179028300039&url=https%3A%2F%2Fcvtisr.summon.serialssolutions.com%2F%23%21%2Fsearch%3Fho%3Df%26include.ft.matches%3Dt%26l%3Dnull%26q%3D
hasFullText
inHoldings 1
isFullTextHit
isPrint
link http://cvtisr.summon.serialssolutions.com/2.0.0/link/0/eLvHCXMwpV1LS8NAEB6qFdSDj_qqzz14Dc1zHyBIKRYPtfSg0lvYV6CgSW2q4L93NmnQi3jwEnIJ7E5md7_Zmfk-gGsulYwFN57wtfIQ3waeyFw3mmGK-9oGuiL1eR6x8ZhPp2LSgpumF8aVVTZ7YrVRm0K7O_IeCykXLExu52-e04xyudWVgMYatCMEMm5Zsul3DsHFpY1enkuvNrxCYdCT2h31UfDyO66szpfh7v9Gtgc7K1xJ-rUj7EPL5h3YHDRybh3Y_sE8eACjPnl1pXhysZCfZOaaRAqE0fiOIJaUM1dnKHNbvJfE2GVVrpWTIiMVrcMsL4nMDVE107M8hKfh3ePg3lsJK3gyifylZ5KM-oJLxGKxchAl1pxyXzGmrYwsiyW1FKNXHagMf1jCMIzNaGwwNqGBNjY8gvW8yO0JEIx2KM-oNUlkYm6EkDJUVPpRIn2FXtqFq8ZoKU7YZSPq0aeN2bpwXNs9ndf8GilCjghRZ3L657dnsFWrs7grkXNoZ7hk7QVs6I_lrFxcVv6Az_Hk4QtML8Eg
linkProvider ProQuest
openUrl ctx_ver=Z39.88-2004&ctx_enc=info%3Aofi%2Fenc%3AUTF-8&rfr_id=info%3Asid%2Fsummon.serialssolutions.com&rft_val_fmt=info%3Aofi%2Ffmt%3Akev%3Amtx%3Ajournal&rft.genre=article&rft.atitle=A+microarray+immunoassay+for+simultaneous+detection+of+proteins+and+bacteria&rft.jtitle=Analytical+chemistry+%28Washington%29&rft.au=Delehanty%2C+James+B&rft.au=Ligler%2C+Frances+S&rft.date=2002-11-01&rft.issn=0003-2700&rft.volume=74&rft.issue=21&rft.spage=5681&rft_id=info:doi/10.1021%2Fac025631l&rft.externalDBID=NO_FULL_TEXT
thumbnail_l http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/lc.gif&issn=0003-2700&client=summon
thumbnail_m http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/mc.gif&issn=0003-2700&client=summon
thumbnail_s http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/sc.gif&issn=0003-2700&client=summon