Kondo Effect in a Neutral and Stable All Organic Radical Single Molecule Break Junction

Organic radicals are neutral, purely organic molecules exhibiting an intrinsic magnetic moment due to the presence of an unpaired electron in the molecule in its ground state. This property, added to the low spin–orbit coupling and weak hyperfine interactions, make neutral organic radicals good cand...

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Veröffentlicht in:	Nano letters Jg. 15; H. 5; S. 3109 - 3114
Hauptverfasser:	Frisenda, Riccardo, Gaudenzi, Rocco, Franco, Carlos, Mas-Torrent, Marta, Rovira, Concepció, Veciana, Jaume, Alcon, Isaac, Bromley, Stefan T, Burzurí, Enrique, van der Zant, Herre S. J
Format:	Journal Article
Sprache:	Englisch
Veröffentlicht:	United States American Chemical Society 13.05.2015
Schlagworte:	Anomalies Breaking Density Electron transport Electrostatics Electrònica de l'estat sòlid Espintrònica Kondo effect Magnetism Magnetisme Radicals Solid state electronics Spintronics Transport d'electrons organic radical magnetism Kondo effect electrical transport break junction Single molecule
ISSN:	1530-6984, 1530-6992
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Abstract	Organic radicals are neutral, purely organic molecules exhibiting an intrinsic magnetic moment due to the presence of an unpaired electron in the molecule in its ground state. This property, added to the low spin–orbit coupling and weak hyperfine interactions, make neutral organic radicals good candidates for molecular spintronics insofar as the radical character is stable in solid state electronic devices. Here we show that the paramagnetism of the polychlorotriphenylmethyl radical molecule in the form of a Kondo anomaly is preserved in two- and three-terminal solid-state devices, regardless of mechanical and electrostatic changes. Indeed, our results demonstrate that the Kondo anomaly is robust under electrodes displacement and changes of the electrostatic environment, pointing to a localized orbital in the radical as the source of magnetism. Strong support to this picture is provided by density functional calculations and measurements of the corresponding nonradical species. These results pave the way toward the use of all-organic neutral radical molecules in spintronics devices and open the door to further investigations into Kondo physics.
AbstractList	Organic radicals are neutral, purely organic molecules exhibiting an intrinsic magnetic moment due to the presence of an unpaired electron in the molecule in its ground state. This property, added to the low spin-orbit coupling and weak hyperfine interactions, make neutral organic radicals good candidates for molecular spintronics insofar as the radical character is stable in solid state electronic devices. Here we show that the paramagnetism of the polychlorotriphenylmethyl radical molecule in the form of a Kondo anomaly is preserved in two- and three-terminal solid-state devices, regardless of mechanical and electrostatic changes. Indeed, our results demonstrate that the Kondo anomaly is robust under electrodes displacement and changes of the electrostatic environment, pointing to a localized orbital in the radical as the source of magnetism. Strong support to this picture is provided by density functional calculations and measurements of the corresponding nonradical species. These results pave the way toward the use of all-organic neutral radical molecules in spintronics devices and open the door to further investigations into Kondo physics. Organic radicals are neutral, purely organic molecules exhibiting an intrinsic magnetic moment due to the presence of an unpaired electron in the molecule in its ground state. This property, added to the low spin-orbit coupling and weak hyperfine interactions, make neutral organic radicals good candidates for molecular spintronics insofar as the radical character is stable in solid state electronic devices. Here we show that the paramagnetism of the polychlorotriphenylmethyl radical molecule in the form of a Kondo anomaly is preserved in two- and three-terminal solid-state devices, regardless of mechanical and electrostatic changes. Indeed, our results demonstrate that the Kondo anomaly is robust under electrodes displacement and changes of the electrostatic environment, pointing to a localized orbital in the radical as the source of magnetism. Strong support to this picture is provided by density functional calculations and measurements of the corresponding nonradical species. These results pave the way toward the use of all-organic neutral radical molecules in spintronics devices and open the door to further investigations into Kondo physics. Keywords: Single molecule; break junction; electrical transport; Kondo effect; organic radical; magnetism
Author	Frisenda, Riccardo Rovira, Concepció Franco, Carlos Mas-Torrent, Marta Bromley, Stefan T Burzurí, Enrique Veciana, Jaume Alcon, Isaac van der Zant, Herre S. J Gaudenzi, Rocco
AuthorAffiliation	Departament de Química Física and Institut de Química Teórica i Computacional (IQTCUB) Universitat de Barcelona Institició Catalana de Recerca i Estudis Avançats (ICREA) Kavli Institute of Nanoscience Delft University of Technology Institut de Ciéncia de Materials de Barcelona (ICMAB-CSIC) and CIBER-BBN
AuthorAffiliation_xml	– name: Institut de Ciéncia de Materials de Barcelona (ICMAB-CSIC) and CIBER-BBN – name: Universitat de Barcelona – name: Institició Catalana de Recerca i Estudis Avançats (ICREA) – name: Kavli Institute of Nanoscience – name: Delft University of Technology – name: Departament de Química Física and Institut de Química Teórica i Computacional (IQTCUB)
Author_xml	– sequence: 1 givenname: Riccardo surname: Frisenda fullname: Frisenda, Riccardo – sequence: 2 givenname: Rocco surname: Gaudenzi fullname: Gaudenzi, Rocco – sequence: 3 givenname: Carlos surname: Franco fullname: Franco, Carlos – sequence: 4 givenname: Marta surname: Mas-Torrent fullname: Mas-Torrent, Marta – sequence: 5 givenname: Concepció surname: Rovira fullname: Rovira, Concepció – sequence: 6 givenname: Jaume surname: Veciana fullname: Veciana, Jaume – sequence: 7 givenname: Isaac surname: Alcon fullname: Alcon, Isaac – sequence: 8 givenname: Stefan T surname: Bromley fullname: Bromley, Stefan T – sequence: 9 givenname: Enrique surname: Burzurí fullname: Burzurí, Enrique email: e.burzurilinares@tudelft.nl – sequence: 10 givenname: Herre S. J surname: van der Zant fullname: van der Zant, Herre S. J
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SubjectTerms	Anomalies Breaking Density Electron transport Electrostatics Electrònica de l'estat sòlid Espintrònica Kondo effect Magnetism Magnetisme Radicals Solid state electronics Spintronics Transport d'electrons
Title	Kondo Effect in a Neutral and Stable All Organic Radical Single Molecule Break Junction
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