Covalent Organic Frameworks: Design, Synthesis, and Functions

Covalent organic frameworks (COFs) are a class of crystalline porous organic polymers with permanent porosity and highly ordered structures. Unlike other polymers, a significant feature of COFs is that they are structurally predesignable, synthetically controllable, and functionally manageable. In p...

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Vydané v:	Chemical reviews Ročník 120; číslo 16; s. 8814
Hlavní autori:	Geng, Keyu, He, Ting, Liu, Ruoyang, Dalapati, Sasanka, Tan, Ke Tian, Li, Zhongping, Tao, Shanshan, Gong, Yifan, Jiang, Qiuhong, Jiang, Donglin
Médium:	Journal Article
Jazyk:	English
Vydavateľské údaje:	United States 26.08.2020
ISSN:	1520-6890, 1520-6890
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Abstract	Covalent organic frameworks (COFs) are a class of crystalline porous organic polymers with permanent porosity and highly ordered structures. Unlike other polymers, a significant feature of COFs is that they are structurally predesignable, synthetically controllable, and functionally manageable. In principle, the topological design diagram offers geometric guidance for the structural tiling of extended porous polygons, and the polycondensation reactions provide synthetic ways to construct the predesigned primary and high-order structures. Progress over the past decade in the chemistry of these two aspects undoubtedly established the base of the COF field. By virtue of the availability of organic units and the diversity of topologies and linkages, COFs have emerged as a new field of organic materials that offer a powerful molecular platform for complex structural design and tailor-made functional development. Here we target a comprehensive review of the COF field, provide a historic overview of the chemistry of the COF field, survey the advances in the topology design and synthetic reactions, illustrate the structural features and diversities, scrutinize the development and potential of various functions through elucidating structure-function correlations based on interactions with photons, electrons, holes, spins, ions, and molecules, discuss the key fundamental and challenging issues that need to be addressed, and predict the future directions from chemistry, physics, and materials perspectives.
AbstractList	Covalent organic frameworks (COFs) are a class of crystalline porous organic polymers with permanent porosity and highly ordered structures. Unlike other polymers, a significant feature of COFs is that they are structurally predesignable, synthetically controllable, and functionally manageable. In principle, the topological design diagram offers geometric guidance for the structural tiling of extended porous polygons, and the polycondensation reactions provide synthetic ways to construct the predesigned primary and high-order structures. Progress over the past decade in the chemistry of these two aspects undoubtedly established the base of the COF field. By virtue of the availability of organic units and the diversity of topologies and linkages, COFs have emerged as a new field of organic materials that offer a powerful molecular platform for complex structural design and tailor-made functional development. Here we target a comprehensive review of the COF field, provide a historic overview of the chemistry of the COF field, survey the advances in the topology design and synthetic reactions, illustrate the structural features and diversities, scrutinize the development and potential of various functions through elucidating structure-function correlations based on interactions with photons, electrons, holes, spins, ions, and molecules, discuss the key fundamental and challenging issues that need to be addressed, and predict the future directions from chemistry, physics, and materials perspectives.Covalent organic frameworks (COFs) are a class of crystalline porous organic polymers with permanent porosity and highly ordered structures. Unlike other polymers, a significant feature of COFs is that they are structurally predesignable, synthetically controllable, and functionally manageable. In principle, the topological design diagram offers geometric guidance for the structural tiling of extended porous polygons, and the polycondensation reactions provide synthetic ways to construct the predesigned primary and high-order structures. Progress over the past decade in the chemistry of these two aspects undoubtedly established the base of the COF field. By virtue of the availability of organic units and the diversity of topologies and linkages, COFs have emerged as a new field of organic materials that offer a powerful molecular platform for complex structural design and tailor-made functional development. Here we target a comprehensive review of the COF field, provide a historic overview of the chemistry of the COF field, survey the advances in the topology design and synthetic reactions, illustrate the structural features and diversities, scrutinize the development and potential of various functions through elucidating structure-function correlations based on interactions with photons, electrons, holes, spins, ions, and molecules, discuss the key fundamental and challenging issues that need to be addressed, and predict the future directions from chemistry, physics, and materials perspectives. Covalent organic frameworks (COFs) are a class of crystalline porous organic polymers with permanent porosity and highly ordered structures. Unlike other polymers, a significant feature of COFs is that they are structurally predesignable, synthetically controllable, and functionally manageable. In principle, the topological design diagram offers geometric guidance for the structural tiling of extended porous polygons, and the polycondensation reactions provide synthetic ways to construct the predesigned primary and high-order structures. Progress over the past decade in the chemistry of these two aspects undoubtedly established the base of the COF field. By virtue of the availability of organic units and the diversity of topologies and linkages, COFs have emerged as a new field of organic materials that offer a powerful molecular platform for complex structural design and tailor-made functional development. Here we target a comprehensive review of the COF field, provide a historic overview of the chemistry of the COF field, survey the advances in the topology design and synthetic reactions, illustrate the structural features and diversities, scrutinize the development and potential of various functions through elucidating structure-function correlations based on interactions with photons, electrons, holes, spins, ions, and molecules, discuss the key fundamental and challenging issues that need to be addressed, and predict the future directions from chemistry, physics, and materials perspectives.
Author	Tao, Shanshan Tan, Ke Tian Jiang, Qiuhong Gong, Yifan He, Ting Li, Zhongping Dalapati, Sasanka Geng, Keyu Jiang, Donglin Liu, Ruoyang
Author_xml	– sequence: 1 givenname: Keyu surname: Geng fullname: Geng, Keyu organization: Department of Chemistry, Faulty of Science, National University of Singapore, 3 Science Drive 3, Singapore 117543, Singapore – sequence: 2 givenname: Ting surname: He fullname: He, Ting organization: Department of Chemistry, Faulty of Science, National University of Singapore, 3 Science Drive 3, Singapore 117543, Singapore – sequence: 3 givenname: Ruoyang surname: Liu fullname: Liu, Ruoyang organization: Department of Chemistry, Faulty of Science, National University of Singapore, 3 Science Drive 3, Singapore 117543, Singapore – sequence: 4 givenname: Sasanka surname: Dalapati fullname: Dalapati, Sasanka organization: Field of Environment and Energy, School of Materials Science, Japan Advanced Institute of Science and Technology, 1-1 Asahidai, Nomi 923-1292, Japan – sequence: 5 givenname: Ke Tian surname: Tan fullname: Tan, Ke Tian organization: Department of Chemistry, Faulty of Science, National University of Singapore, 3 Science Drive 3, Singapore 117543, Singapore – sequence: 6 givenname: Zhongping surname: Li fullname: Li, Zhongping organization: Department of Chemistry, Faulty of Science, National University of Singapore, 3 Science Drive 3, Singapore 117543, Singapore – sequence: 7 givenname: Shanshan surname: Tao fullname: Tao, Shanshan organization: Department of Chemistry, Faulty of Science, National University of Singapore, 3 Science Drive 3, Singapore 117543, Singapore – sequence: 8 givenname: Yifan surname: Gong fullname: Gong, Yifan organization: Department of Chemistry, Faulty of Science, National University of Singapore, 3 Science Drive 3, Singapore 117543, Singapore – sequence: 9 givenname: Qiuhong surname: Jiang fullname: Jiang, Qiuhong organization: Department of Chemistry, Faulty of Science, National University of Singapore, 3 Science Drive 3, Singapore 117543, Singapore – sequence: 10 givenname: Donglin orcidid: 0000-0002-3785-1330 surname: Jiang fullname: Jiang, Donglin organization: Joint School of National University of Singapore and Tianjin University, International Campus of Tianjin University, Binhai New City, Fuzhou 350207, P. R. China
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/31967791$$D View this record in MEDLINE/PubMed
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Snippet	Covalent organic frameworks (COFs) are a class of crystalline porous organic polymers with permanent porosity and highly ordered structures. Unlike other...
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