Single-Atom (Iron-Based) Catalysts: Synthesis and Applications
Supported single-metal atom catalysts (SACs) are constituted of isolated active metal centers, which are heterogenized on inert supports such as graphene, porous carbon, and metal oxides. Their thermal stability, electronic properties, and catalytic activities can be controlled via interactions betw...
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| Vydané v: | Chemical reviews Ročník 121; číslo 21; s. 13620 |
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| Hlavní autori: | , , , , , , , , |
| Médium: | Journal Article |
| Jazyk: | English |
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United States
10.11.2021
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| ISSN: | 1520-6890, 1520-6890 |
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| Abstract | Supported single-metal atom catalysts (SACs) are constituted of isolated active metal centers, which are heterogenized on inert supports such as graphene, porous carbon, and metal oxides. Their thermal stability, electronic properties, and catalytic activities can be controlled via interactions between the single-metal atom center and neighboring heteroatoms such as nitrogen, oxygen, and sulfur. Due to the atomic dispersion of the active catalytic centers, the amount of metal required for catalysis can be decreased, thus offering new possibilities to control the selectivity of a given transformation as well as to improve catalyst turnover frequencies and turnover numbers. This review aims to comprehensively summarize the synthesis of Fe-SACs with a focus on anchoring single atoms (SA) on carbon/graphene supports. The characterization of these advanced materials using various spectroscopic techniques and their applications in diverse research areas are described. When applicable, mechanistic investigations conducted to understand the specific behavior of Fe-SACs-based catalysts are highlighted, including the use of theoretical models. |
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| AbstractList | Supported single-metal atom catalysts (SACs) are constituted of isolated active metal centers, which are heterogenized on inert supports such as graphene, porous carbon, and metal oxides. Their thermal stability, electronic properties, and catalytic activities can be controlled via interactions between the single-metal atom center and neighboring heteroatoms such as nitrogen, oxygen, and sulfur. Due to the atomic dispersion of the active catalytic centers, the amount of metal required for catalysis can be decreased, thus offering new possibilities to control the selectivity of a given transformation as well as to improve catalyst turnover frequencies and turnover numbers. This review aims to comprehensively summarize the synthesis of Fe-SACs with a focus on anchoring single atoms (SA) on carbon/graphene supports. The characterization of these advanced materials using various spectroscopic techniques and their applications in diverse research areas are described. When applicable, mechanistic investigations conducted to understand the specific behavior of Fe-SACs-based catalysts are highlighted, including the use of theoretical models. Supported single-metal atom catalysts (SACs) are constituted of isolated active metal centers, which are heterogenized on inert supports such as graphene, porous carbon, and metal oxides. Their thermal stability, electronic properties, and catalytic activities can be controlled via interactions between the single-metal atom center and neighboring heteroatoms such as nitrogen, oxygen, and sulfur. Due to the atomic dispersion of the active catalytic centers, the amount of metal required for catalysis can be decreased, thus offering new possibilities to control the selectivity of a given transformation as well as to improve catalyst turnover frequencies and turnover numbers. This review aims to comprehensively summarize the synthesis of Fe-SACs with a focus on anchoring single atoms (SA) on carbon/graphene supports. The characterization of these advanced materials using various spectroscopic techniques and their applications in diverse research areas are described. When applicable, mechanistic investigations conducted to understand the specific behavior of Fe-SACs-based catalysts are highlighted, including the use of theoretical models.Supported single-metal atom catalysts (SACs) are constituted of isolated active metal centers, which are heterogenized on inert supports such as graphene, porous carbon, and metal oxides. Their thermal stability, electronic properties, and catalytic activities can be controlled via interactions between the single-metal atom center and neighboring heteroatoms such as nitrogen, oxygen, and sulfur. Due to the atomic dispersion of the active catalytic centers, the amount of metal required for catalysis can be decreased, thus offering new possibilities to control the selectivity of a given transformation as well as to improve catalyst turnover frequencies and turnover numbers. This review aims to comprehensively summarize the synthesis of Fe-SACs with a focus on anchoring single atoms (SA) on carbon/graphene supports. The characterization of these advanced materials using various spectroscopic techniques and their applications in diverse research areas are described. When applicable, mechanistic investigations conducted to understand the specific behavior of Fe-SACs-based catalysts are highlighted, including the use of theoretical models. |
| Author | Beller, Matthias Zbořil, Radek Gawande, Manoj B Varma, Rajender S Kute, Arun D Fornasiero, Paolo McNeice, Peter Singh, Baljeet Jagadeesh, Rajenahally V |
| Author_xml | – sequence: 1 givenname: Baljeet orcidid: 0000-0002-8029-8577 surname: Singh fullname: Singh, Baljeet organization: CICECO-Aveiro Institute of Materials, University of Aveiro, Aveiro, 3810-193 Portugal – sequence: 2 givenname: Manoj B orcidid: 0000-0003-1575-094X surname: Gawande fullname: Gawande, Manoj B organization: Department of Industrial and Engineering Chemistry, Institute of Chemical Technology Mumbai-Marathwada Campus, Jalna 431213, Maharashtra, India – sequence: 3 givenname: Arun D surname: Kute fullname: Kute, Arun D organization: Department of Industrial and Engineering Chemistry, Institute of Chemical Technology Mumbai-Marathwada Campus, Jalna 431213, Maharashtra, India – sequence: 4 givenname: Rajender S orcidid: 0000-0001-9731-6228 surname: Varma fullname: Varma, Rajender S organization: Regional Centre of Advanced Technologies and Materials, Czech Advanced Technology and Research Institute, Palacký University, 779 00 Olomouc, Czech Republic – sequence: 5 givenname: Paolo orcidid: 0000-0003-1082-9157 surname: Fornasiero fullname: Fornasiero, Paolo organization: Department of Chemical and Pharmaceutical Sciences, Center for Energy, Environment and Transport Giacomo Ciamiciam, INSTM Trieste Research Unit and ICCOM-CNR Trieste Research Unit, University of Trieste, Via L. Giorgieri 1, 34127 Trieste, Italy – sequence: 6 givenname: Peter orcidid: 0000-0002-6597-5437 surname: McNeice fullname: McNeice, Peter organization: Leibniz-Institut für Katalyse e. V., Albert-Einstein-Straße 29a, 18059 Rostock, Germany – sequence: 7 givenname: Rajenahally V orcidid: 0000-0001-6079-0962 surname: Jagadeesh fullname: Jagadeesh, Rajenahally V organization: Department of Chemistry, REVA University, Bangalore 560064, India – sequence: 8 givenname: Matthias orcidid: 0000-0001-5709-0965 surname: Beller fullname: Beller, Matthias organization: Leibniz-Institut für Katalyse e. V., Albert-Einstein-Straße 29a, 18059 Rostock, Germany – sequence: 9 givenname: Radek orcidid: 0000-0002-3147-2196 surname: Zbořil fullname: Zbořil, Radek organization: CEET Nanotechnology Centre, VŠB-Technical University of Ostrava, 17. Listopadu 2172/15, 708 00 Ostrava-Poruba, Czech Republic |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/34644065$$D View this record in MEDLINE/PubMed |
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| Title | Single-Atom (Iron-Based) Catalysts: Synthesis and Applications |
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