A Highly Efficient Coordination Polymer for Selective Trapping and Sensing of Perrhenate/Pertechnetate
A porous cationic Ag(I) coordination polymer, [Ag(1,2,4,5-p4b)](SbF ) (TJNU-302) with the ligand 1,2,4,5-p4b (1,2,4,5-tetra(pyridin-4-yl)benzene), is reported that shows high sorption capacity (211 mg g ) and distribution coefficient (5.8 × 10 mL g ) as well as outstanding selectivity in 500 times e...
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| Vydané v: | ACS applied materials & interfaces Ročník 12; číslo 13; s. 15246 |
|---|---|
| Hlavní autori: | , , , , , |
| Médium: | Journal Article |
| Jazyk: | English |
| Vydavateľské údaje: |
United States
01.04.2020
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| Predmet: | |
| ISSN: | 1944-8252, 1944-8252 |
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| Abstract | A porous cationic Ag(I) coordination polymer, [Ag(1,2,4,5-p4b)](SbF
) (TJNU-302) with the ligand 1,2,4,5-p4b (1,2,4,5-tetra(pyridin-4-yl)benzene), is reported that shows high sorption capacity (211 mg g
) and distribution coefficient
(5.8 × 10
mL g
) as well as outstanding selectivity in 500 times excess of CO
or PO
anion for perrhenate removal. TJNU-302 can act as a crystalline turn-off sensor for perrhenate upon UV radiation. In this way, a test paper strip for sensing ReO
could be produced. In water solution, TJNU-302 shows an efficient fluorescence quenching response to ReO
ion, with the highest quenching percentage (86%) among all reported ReO
sensors. These results could be elucidated by the bonding properties of single-crystal structures of TJNU-302 before and after perrhenate sorption, as well as density functional theory (DFT) calculations. |
|---|---|
| AbstractList | A porous cationic Ag(I) coordination polymer, [Ag(1,2,4,5-p4b)](SbF6) (TJNU-302) with the ligand 1,2,4,5-p4b (1,2,4,5-tetra(pyridin-4-yl)benzene), is reported that shows high sorption capacity (211 mg g-1) and distribution coefficient Kd (5.8 × 105 mL g-1) as well as outstanding selectivity in 500 times excess of CO32- or PO43- anion for perrhenate removal. TJNU-302 can act as a crystalline turn-off sensor for perrhenate upon UV radiation. In this way, a test paper strip for sensing ReO4- could be produced. In water solution, TJNU-302 shows an efficient fluorescence quenching response to ReO4- ion, with the highest quenching percentage (86%) among all reported ReO4- sensors. These results could be elucidated by the bonding properties of single-crystal structures of TJNU-302 before and after perrhenate sorption, as well as density functional theory (DFT) calculations.A porous cationic Ag(I) coordination polymer, [Ag(1,2,4,5-p4b)](SbF6) (TJNU-302) with the ligand 1,2,4,5-p4b (1,2,4,5-tetra(pyridin-4-yl)benzene), is reported that shows high sorption capacity (211 mg g-1) and distribution coefficient Kd (5.8 × 105 mL g-1) as well as outstanding selectivity in 500 times excess of CO32- or PO43- anion for perrhenate removal. TJNU-302 can act as a crystalline turn-off sensor for perrhenate upon UV radiation. In this way, a test paper strip for sensing ReO4- could be produced. In water solution, TJNU-302 shows an efficient fluorescence quenching response to ReO4- ion, with the highest quenching percentage (86%) among all reported ReO4- sensors. These results could be elucidated by the bonding properties of single-crystal structures of TJNU-302 before and after perrhenate sorption, as well as density functional theory (DFT) calculations. A porous cationic Ag(I) coordination polymer, [Ag(1,2,4,5-p4b)](SbF ) (TJNU-302) with the ligand 1,2,4,5-p4b (1,2,4,5-tetra(pyridin-4-yl)benzene), is reported that shows high sorption capacity (211 mg g ) and distribution coefficient (5.8 × 10 mL g ) as well as outstanding selectivity in 500 times excess of CO or PO anion for perrhenate removal. TJNU-302 can act as a crystalline turn-off sensor for perrhenate upon UV radiation. In this way, a test paper strip for sensing ReO could be produced. In water solution, TJNU-302 shows an efficient fluorescence quenching response to ReO ion, with the highest quenching percentage (86%) among all reported ReO sensors. These results could be elucidated by the bonding properties of single-crystal structures of TJNU-302 before and after perrhenate sorption, as well as density functional theory (DFT) calculations. |
| Author | Li, Cheng-Peng Zhou, Wuzong Du, Miao Wang, Jia-Jun Zhou, Hang Chen, Jing |
| Author_xml | – sequence: 1 givenname: Cheng-Peng orcidid: 0000-0002-6798-9541 surname: Li fullname: Li, Cheng-Peng organization: School of Chemistry, University of St. Andrews, Andrews KY16 9ST, United Kingdom – sequence: 2 givenname: Hang surname: Zhou fullname: Zhou, Hang organization: Tianjin Key Laboratory of Structure and Performance for Functional Molecules, MOE Key Laboratory of Inorganic-Organic Hybrid Functional Material Chemistry, College of Chemistry, Tianjin Normal University, Tianjin 300387, P. R. China – sequence: 3 givenname: Jing surname: Chen fullname: Chen, Jing organization: Tianjin Key Laboratory of Structure and Performance for Functional Molecules, MOE Key Laboratory of Inorganic-Organic Hybrid Functional Material Chemistry, College of Chemistry, Tianjin Normal University, Tianjin 300387, P. R. China – sequence: 4 givenname: Jia-Jun surname: Wang fullname: Wang, Jia-Jun organization: Tianjin Key Laboratory of Structure and Performance for Functional Molecules, MOE Key Laboratory of Inorganic-Organic Hybrid Functional Material Chemistry, College of Chemistry, Tianjin Normal University, Tianjin 300387, P. R. China – sequence: 5 givenname: Miao orcidid: 0000-0002-1029-1820 surname: Du fullname: Du, Miao organization: Tianjin Key Laboratory of Structure and Performance for Functional Molecules, MOE Key Laboratory of Inorganic-Organic Hybrid Functional Material Chemistry, College of Chemistry, Tianjin Normal University, Tianjin 300387, P. R. China – sequence: 6 givenname: Wuzong orcidid: 0000-0001-9752-7076 surname: Zhou fullname: Zhou, Wuzong organization: School of Chemistry, University of St. Andrews, Andrews KY16 9ST, United Kingdom |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/32150370$$D View this record in MEDLINE/PubMed |
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| Keywords | coordination polymers perrhenate/pertechnetate anion exchange test paper fluorescence sensor |
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| Snippet | A porous cationic Ag(I) coordination polymer, [Ag(1,2,4,5-p4b)](SbF
) (TJNU-302) with the ligand 1,2,4,5-p4b (1,2,4,5-tetra(pyridin-4-yl)benzene), is reported... A porous cationic Ag(I) coordination polymer, [Ag(1,2,4,5-p4b)](SbF6) (TJNU-302) with the ligand 1,2,4,5-p4b (1,2,4,5-tetra(pyridin-4-yl)benzene), is reported... |
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| Title | A Highly Efficient Coordination Polymer for Selective Trapping and Sensing of Perrhenate/Pertechnetate |
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