Two-Dimensional Conjugated Metal–Organic Frameworks for Electrocatalysis: Opportunities and Challenges

A highly effective electrocatalyst is the central component of advanced electrochemical energy conversion. Recently, two-dimensional conjugated metal–organic frameworks (2D c-MOFs) have emerged as a class of promising electrocatalysts because of their advantages including 2D layered structure with h...

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Vydáno v:ACS nano Ročník 16; číslo 2; s. 1759 - 1780
Hlavní autoři: Zhong, Haixia, Wang, Mingchao, Chen, Guangbo, Dong, Renhao, Feng, Xinliang
Médium: Journal Article
Jazyk:angličtina
Vydáno: United States American Chemical Society 22.02.2022
Témata:
Electrochemical energy conversion
oxygen reduction/evolution
hydrogen evolution reaction
catalytic reaction mechanism
intrinsic electrical conductivity
carbon dioxide/nitrogen reduction
electrocatalysis
two-dimensional conjugated metal−organic framework
ISSN:1936-0851, 1936-086X, 1936-086X
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Abstract A highly effective electrocatalyst is the central component of advanced electrochemical energy conversion. Recently, two-dimensional conjugated metal–organic frameworks (2D c-MOFs) have emerged as a class of promising electrocatalysts because of their advantages including 2D layered structure with high in-plane conjugation, intrinsic electrical conductivity, permanent pores, large surface area, chemical stability, and structural diversity. In this Review, we summarize the recent advances of 2D c-MOF electrocatalysts for electrochemical energy conversion. First, we introduce the chemical design principles and synthetic strategies of the reported 2D c-MOFs, as well as the functional design for the electrocatalysis. Subsequently, we present the representative 2D c-MOF electrocatalysts in various electrochemical reactions, such as hydrogen/oxygen evolution, and reduction reactions of oxygen, carbon dioxide, and nitrogen. We highlight the strategies for the structural design and property tuning of 2D c-MOF electrocatalysts to boost the catalytic performance, and we offer our perspectives in regard to the challenges to be overcome.
AbstractList A highly effective electrocatalyst is the central component of advanced electrochemical energy conversion. Recently, two-dimensional conjugated metal-organic frameworks (2D c-MOFs) have emerged as a class of promising electrocatalysts because of their advantages including 2D layered structure with high in-plane conjugation, intrinsic electrical conductivity, permanent pores, large surface area, chemical stability, and structural diversity. In this Review, we summarize the recent advances of 2D c-MOF electrocatalysts for electrochemical energy conversion. First, we introduce the chemical design principles and synthetic strategies of the reported 2D c-MOFs, as well as the functional design for the electrocatalysis. Subsequently, we present the representative 2D c-MOF electrocatalysts in various electrochemical reactions, such as hydrogen/oxygen evolution, and reduction reactions of oxygen, carbon dioxide, and nitrogen. We highlight the strategies for the structural design and property tuning of 2D c-MOF electrocatalysts to boost the catalytic performance, and we offer our perspectives in regard to the challenges to be overcome.A highly effective electrocatalyst is the central component of advanced electrochemical energy conversion. Recently, two-dimensional conjugated metal-organic frameworks (2D c-MOFs) have emerged as a class of promising electrocatalysts because of their advantages including 2D layered structure with high in-plane conjugation, intrinsic electrical conductivity, permanent pores, large surface area, chemical stability, and structural diversity. In this Review, we summarize the recent advances of 2D c-MOF electrocatalysts for electrochemical energy conversion. First, we introduce the chemical design principles and synthetic strategies of the reported 2D c-MOFs, as well as the functional design for the electrocatalysis. Subsequently, we present the representative 2D c-MOF electrocatalysts in various electrochemical reactions, such as hydrogen/oxygen evolution, and reduction reactions of oxygen, carbon dioxide, and nitrogen. We highlight the strategies for the structural design and property tuning of 2D c-MOF electrocatalysts to boost the catalytic performance, and we offer our perspectives in regard to the challenges to be overcome.
A highly effective electrocatalyst is the central component of advanced electrochemical energy conversion. Recently, two-dimensional conjugated metal–organic frameworks (2D c-MOFs) have emerged as a class of promising electrocatalysts because of their advantages including 2D layered structure with high in-plane conjugation, intrinsic electrical conductivity, permanent pores, large surface area, chemical stability, and structural diversity. In this Review, we summarize the recent advances of 2D c-MOF electrocatalysts for electrochemical energy conversion. First, we introduce the chemical design principles and synthetic strategies of the reported 2D c-MOFs, as well as the functional design for the electrocatalysis. Subsequently, we present the representative 2D c-MOF electrocatalysts in various electrochemical reactions, such as hydrogen/oxygen evolution, and reduction reactions of oxygen, carbon dioxide, and nitrogen. We highlight the strategies for the structural design and property tuning of 2D c-MOF electrocatalysts to boost the catalytic performance, and we offer our perspectives in regard to the challenges to be overcome.
Author Zhong, Haixia
Chen, Guangbo
Wang, Mingchao
Feng, Xinliang
Dong, Renhao
AuthorAffiliation Center for Advancing Electronics Dresden (cfaed) and Faculty of Chemistry and Food Chemistry
Max Planck Institute of Microstructure Physics
Shandong University
Key Laboratory of Colloid and Interface Chemistry of the Ministry of Education, School of Chemistry and Chemical Engineering
AuthorAffiliation_xml – name: Key Laboratory of Colloid and Interface Chemistry of the Ministry of Education, School of Chemistry and Chemical Engineering
– name: Shandong University
– name: Max Planck Institute of Microstructure Physics
– name: Center for Advancing Electronics Dresden (cfaed) and Faculty of Chemistry and Food Chemistry
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  givenname: Haixia
  orcidid: 0000-0002-2839-0253
  surname: Zhong
  fullname: Zhong, Haixia
  organization: Center for Advancing Electronics Dresden (cfaed) and Faculty of Chemistry and Food Chemistry
– sequence: 2
  givenname: Mingchao
  surname: Wang
  fullname: Wang, Mingchao
  organization: Center for Advancing Electronics Dresden (cfaed) and Faculty of Chemistry and Food Chemistry
– sequence: 3
  givenname: Guangbo
  surname: Chen
  fullname: Chen, Guangbo
  organization: Center for Advancing Electronics Dresden (cfaed) and Faculty of Chemistry and Food Chemistry
– sequence: 4
  givenname: Renhao
  orcidid: 0000-0002-4125-9284
  surname: Dong
  fullname: Dong, Renhao
  email: renhao.dong@tu-dresden.de
  organization: Shandong University
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  surname: Feng
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  organization: Max Planck Institute of Microstructure Physics
BackLink https://www.ncbi.nlm.nih.gov/pubmed/35049290$$D View this record in MEDLINE/PubMed
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Issue 2
Keywords Electrochemical energy conversion
oxygen reduction/evolution
hydrogen evolution reaction
catalytic reaction mechanism
intrinsic electrical conductivity
carbon dioxide/nitrogen reduction
electrocatalysis
two-dimensional conjugated metal−organic framework
Language English
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Snippet A highly effective electrocatalyst is the central component of advanced electrochemical energy conversion. Recently, two-dimensional conjugated metal–organic...
A highly effective electrocatalyst is the central component of advanced electrochemical energy conversion. Recently, two-dimensional conjugated metal-organic...
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Title Two-Dimensional Conjugated Metal–Organic Frameworks for Electrocatalysis: Opportunities and Challenges
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https://www.ncbi.nlm.nih.gov/pubmed/35049290
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