Twisted Nonlinear Optics in Monolayer van der Waals Crystals

In addition to a plethora of emergent phenomena, the spatial topology of optical vortices enables an array of applications in optical communications and quantum information science. Multibeam nonlinear optical processes, augmented by optical vortices, are essential in this context, providing robust...

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Vydané v:ACS nano Ročník 19; číslo 34; s. 30919 - 30929
Hlavní autori: Norden, Tenzin, Martinez, Luis M., Tarefder, Nehan, Kwock, Kevin W. C., McClintock, Luke M., Olsen, Nicholas, Holtzman, Luke N., Yeo, June Ho, Zhao, Liuyan, Zhu, Xiaoyang, Hone, James C., Yoo, Jinkyoung, Zhu, Jian-Xin, Schuck, P. James, Taylor, Antoinette J., Prasankumar, Rohit P., Kort-Kamp, Wilton J. M., Padmanabhan, Prashant
Médium: Journal Article
Jazyk:English
Vydavateľské údaje: United States American Chemical Society 02.09.2025
American Chemical Society (ACS)
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ISSN:1936-0851, 1936-086X, 1936-086X
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Abstract In addition to a plethora of emergent phenomena, the spatial topology of optical vortices enables an array of applications in optical communications and quantum information science. Multibeam nonlinear optical processes, augmented by optical vortices, are essential in this context, providing robust access to an infinitely large set of quantum states associated with the orbital angular momentum of light. Here, we push the boundaries of vortex nonlinear optics to the ultimate limits of material dimensionality. By exploiting multipulse difference frequency, sum frequency, and four-wave mixing in monolayer quantum materials, we demonstrate their ability to independently control the orbital angular momentum and radial distribution of vortex light-fields in addition to their wavelength. Due to the atomically thin nature of the host crystal, this control spans a broad spectral bandwidth in a highly integrable platform that is unconstrained by the traditional limits of bulk nonlinear optical materials. Our work heralds an innovative path for ultracompact and scalable hybrid nanophotonic technologies empowered by twisted nonlinear light–matter interactions in van der Waals nanomaterials.
AbstractList In addition to a plethora of emergent phenomena, the spatial topology of optical vortices enables an array of applications in optical communications and quantum information science. Multibeam nonlinear optical processes, augmented by optical vortices, are essential in this context, providing robust access to an infinitely large set of quantum states associated with the orbital angular momentum of light. Here, we push the boundaries of vortex nonlinear optics to the ultimate limits of material dimensionality. By exploiting multipulse difference frequency, sum frequency, and four-wave mixing in monolayer quantum materials, we demonstrate their ability to independently control the orbital angular momentum and radial distribution of vortex light-fields in addition to their wavelength. Due to the atomically thin nature of the host crystal, this control spans a broad spectral bandwidth in a highly integrable platform that is unconstrained by the traditional limits of bulk nonlinear optical materials. Our work heralds an innovative path for ultracompact and scalable hybrid nanophotonic technologies empowered by twisted nonlinear light-matter interactions in van der Waals nanomaterials.
In addition to a plethora of emergent phenomena, the spatial topology of optical vortices enables an array of applications in optical communications and quantum information science. Multibeam nonlinear optical processes, augmented by optical vortices, are essential in this context, providing robust access to an infinitely large set of quantum states associated with the orbital angular momentum of light. Here, we push the boundaries of vortex nonlinear optics to the ultimate limits of material dimensionality. By exploiting multipulse difference frequency, sum frequency, and four-wave mixing in monolayer quantum materials, we demonstrate their ability to independently control the orbital angular momentum and radial distribution of vortex light-fields in addition to their wavelength. Due to the atomically thin nature of the host crystal, this control spans a broad spectral bandwidth in a highly integrable platform that is unconstrained by the traditional limits of bulk nonlinear optical materials. Our work heralds an innovative path for ultracompact and scalable hybrid nanophotonic technologies empowered by twisted nonlinear light-matter interactions in van der Waals nanomaterials.In addition to a plethora of emergent phenomena, the spatial topology of optical vortices enables an array of applications in optical communications and quantum information science. Multibeam nonlinear optical processes, augmented by optical vortices, are essential in this context, providing robust access to an infinitely large set of quantum states associated with the orbital angular momentum of light. Here, we push the boundaries of vortex nonlinear optics to the ultimate limits of material dimensionality. By exploiting multipulse difference frequency, sum frequency, and four-wave mixing in monolayer quantum materials, we demonstrate their ability to independently control the orbital angular momentum and radial distribution of vortex light-fields in addition to their wavelength. Due to the atomically thin nature of the host crystal, this control spans a broad spectral bandwidth in a highly integrable platform that is unconstrained by the traditional limits of bulk nonlinear optical materials. Our work heralds an innovative path for ultracompact and scalable hybrid nanophotonic technologies empowered by twisted nonlinear light-matter interactions in van der Waals nanomaterials.
Author Yeo, June Ho
Taylor, Antoinette J.
Zhu, Xiaoyang
Holtzman, Luke N.
Zhu, Jian-Xin
Tarefder, Nehan
Schuck, P. James
Martinez, Luis M.
Olsen, Nicholas
Kort-Kamp, Wilton J. M.
Kwock, Kevin W. C.
Prasankumar, Rohit P.
Zhao, Liuyan
Norden, Tenzin
McClintock, Luke M.
Hone, James C.
Yoo, Jinkyoung
Padmanabhan, Prashant
AuthorAffiliation Department of Chemistry
Theoretical Division
Deep Science Fund
Department of Electrical Engineering
Center for Integrated Nanotechnologies
Department of Applied Physics and Applied Mathematics
Department of Mechanical Engineering
Department of Physics
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Issue 34
Keywords nonlinear optics
two-dimensional semiconductors
vortex beams
difference frequency generation
sum frequency generation
orbital angular momentum
four-wave mixing
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