Trace element geochemistry of sphalerite in contrasting hydrothermal fluid systems of the Freiberg district, Germany: insights from LA-ICP-MS analysis, near-infrared light microthermometry of sphalerite-hosted fluid inclusions, and sulfur isotope geochemistry
The historic silver mining district of Freiberg (Germany) comprises hydrothermal vein-style mineralization of Permian and Cretaceous age. We compare sphalerite compositions with associated ore-forming fluids and constrain the behavior of critical metals such as In, Ge, and Ga in contrasting hydrothe...
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| Vydáno v: | Mineralium deposita Ročník 54; číslo 2; s. 237 - 262 |
|---|---|
| Hlavní autoři: | , , , , , , |
| Médium: | Journal Article |
| Jazyk: | angličtina |
| Vydáno: |
Berlin/Heidelberg
Springer Berlin Heidelberg
01.02.2019
Springer Nature B.V |
| Témata: | |
| ISSN: | 0026-4598, 1432-1866 |
| On-line přístup: | Získat plný text |
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| Abstract | The historic silver mining district of Freiberg (Germany) comprises hydrothermal vein-style mineralization of Permian and Cretaceous age. We compare sphalerite compositions with associated ore-forming fluids and constrain the behavior of critical metals such as In, Ge, and Ga in contrasting hydrothermal environments. Fluid inclusion studies reveal that the Permian veins formed due to boiling and cooling of a low-salinity (0 to 6% eq.
w
[NaCl]) magmatic-hydrothermal fluid at 350 to 230 °C. In contrast, Cretaceous veins formed by mixing of highly saline (17 to 24% eq.
w
[NaCl + CaCl
2
] and variable Na/(Na + Ca) ratios) brines at low temperatures (~ 120 °C). Sulfides of the Permian ore stage have a narrow range of
δ
34
S
VCDT
from − 2.3 to + 0.9‰, while the sulfides of the Cretaceous stage have a large scatter and significantly more negative
δ
34
S
VCDT
values (− 30.9 to − 5.5‰), supporting the different nature of the hydrothermal systems. Contrasting fluid systems and ore-forming mechanisms correspond to markedly different trace element systematics in sphalerite. Permian sphalerite is significantly enriched in In (up to 2500 μg/g In) relative to two sphalerite generations of Cretaceous veins. The latter have higher Ge (up to 2700 μg/g Ge) and Ga (up to 1000 μg/g Ga) concentrations. The observed trace element systematics of different sphalerite generations imply that In is enriched in high-temperature, low- to intermediate-salinity fluids with a significant magmatic-hydrothermal fluid component, while Ge and Ga are more concentrated in low-temperature, high-salinity crustal fluids with no obvious magmatic-hydrothermal affiliation. |
|---|---|
| AbstractList | The historic silver mining district of Freiberg (Germany) comprises hydrothermal vein-style mineralization of Permian and Cretaceous age. We compare sphalerite compositions with associated ore-forming fluids and constrain the behavior of critical metals such as In, Ge, and Ga in contrasting hydrothermal environments. Fluid inclusion studies reveal that the Permian veins formed due to boiling and cooling of a low-salinity (0 to 6% eq. w[NaCl]) magmatic-hydrothermal fluid at 350 to 230 °C. In contrast, Cretaceous veins formed by mixing of highly saline (17 to 24% eq. w[NaCl + CaCl2] and variable Na/(Na + Ca) ratios) brines at low temperatures (~ 120 °C). Sulfides of the Permian ore stage have a narrow range of δ34SVCDT from − 2.3 to + 0.9‰, while the sulfides of the Cretaceous stage have a large scatter and significantly more negative δ34SVCDT values (− 30.9 to − 5.5‰), supporting the different nature of the hydrothermal systems. Contrasting fluid systems and ore-forming mechanisms correspond to markedly different trace element systematics in sphalerite. Permian sphalerite is significantly enriched in In (up to 2500 μg/g In) relative to two sphalerite generations of Cretaceous veins. The latter have higher Ge (up to 2700 μg/g Ge) and Ga (up to 1000 μg/g Ga) concentrations. The observed trace element systematics of different sphalerite generations imply that In is enriched in high-temperature, low- to intermediate-salinity fluids with a significant magmatic-hydrothermal fluid component, while Ge and Ga are more concentrated in low-temperature, high-salinity crustal fluids with no obvious magmatic-hydrothermal affiliation. The historic silver mining district of Freiberg (Germany) comprises hydrothermal vein-style mineralization of Permian and Cretaceous age. We compare sphalerite compositions with associated ore-forming fluids and constrain the behavior of critical metals such as In, Ge, and Ga in contrasting hydrothermal environments. Fluid inclusion studies reveal that the Permian veins formed due to boiling and cooling of a low-salinity (0 to 6% eq. w [NaCl]) magmatic-hydrothermal fluid at 350 to 230 °C. In contrast, Cretaceous veins formed by mixing of highly saline (17 to 24% eq. w [NaCl + CaCl 2 ] and variable Na/(Na + Ca) ratios) brines at low temperatures (~ 120 °C). Sulfides of the Permian ore stage have a narrow range of δ 34 S VCDT from − 2.3 to + 0.9‰, while the sulfides of the Cretaceous stage have a large scatter and significantly more negative δ 34 S VCDT values (− 30.9 to − 5.5‰), supporting the different nature of the hydrothermal systems. Contrasting fluid systems and ore-forming mechanisms correspond to markedly different trace element systematics in sphalerite. Permian sphalerite is significantly enriched in In (up to 2500 μg/g In) relative to two sphalerite generations of Cretaceous veins. The latter have higher Ge (up to 2700 μg/g Ge) and Ga (up to 1000 μg/g Ga) concentrations. The observed trace element systematics of different sphalerite generations imply that In is enriched in high-temperature, low- to intermediate-salinity fluids with a significant magmatic-hydrothermal fluid component, while Ge and Ga are more concentrated in low-temperature, high-salinity crustal fluids with no obvious magmatic-hydrothermal affiliation. |
| Author | Bauer, Matthias E. Ostendorf, Jörg Krause, Joachim Gutzmer, Jens Seifert, Thomas Burisch, Mathias Frenzel, Max |
| Author_xml | – sequence: 1 givenname: Matthias E. orcidid: 0000-0002-3363-2333 surname: Bauer fullname: Bauer, Matthias E. email: matthias.bauer@mineral.tu-freiberg.de organization: Institut für Mineralogie, Technische Universität Bergakademie Freiberg – sequence: 2 givenname: Mathias surname: Burisch fullname: Burisch, Mathias email: mathias.burisch@mineral.tu-freiberg.de organization: Institut für Mineralogie, Technische Universität Bergakademie Freiberg – sequence: 3 givenname: Jörg surname: Ostendorf fullname: Ostendorf, Jörg organization: Institut für Mineralogie, Technische Universität Bergakademie Freiberg – sequence: 4 givenname: Joachim surname: Krause fullname: Krause, Joachim organization: Helmholtz-Zentrum Dresden-Rossendorf, Helmholtz Institute Freiberg for Resource Technology – sequence: 5 givenname: Max surname: Frenzel fullname: Frenzel, Max organization: Institut für Mineralogie, Technische Universität Bergakademie Freiberg, Helmholtz-Zentrum Dresden-Rossendorf, Helmholtz Institute Freiberg for Resource Technology – sequence: 6 givenname: Thomas surname: Seifert fullname: Seifert, Thomas organization: Institut für Mineralogie, Technische Universität Bergakademie Freiberg – sequence: 7 givenname: Jens surname: Gutzmer fullname: Gutzmer, Jens organization: Institut für Mineralogie, Technische Universität Bergakademie Freiberg, Helmholtz-Zentrum Dresden-Rossendorf, Helmholtz Institute Freiberg for Resource Technology |
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| Issue | 2 |
| Keywords | Sphalerite Gallium Critical metals Erzgebirge Germanium LA-ICP-MS Sulfur isotopes Indium Near-infrared light microthermometry Geothermometer EPMA Fluid inclusions |
| Language | English |
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| PublicationDate | 2019-02-01 |
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| PublicationPlace | Berlin/Heidelberg |
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| PublicationSubtitle | International Journal for Geology, Mineralogy and Geochemistry of Mineral Deposits |
| PublicationTitle | Mineralium deposita |
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| PublicationYear | 2019 |
| Publisher | Springer Berlin Heidelberg Springer Nature B.V |
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| Snippet | The historic silver mining district of Freiberg (Germany) comprises hydrothermal vein-style mineralization of Permian and Cretaceous age. We compare sphalerite... |
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| SubjectTerms | Brines Calcium chloride Concentrates (ores) Cretaceous Earth and Environmental Science Earth Sciences Fluid inclusions Fluids Gallium Geochemistry Geology Germanium Heavy metals High temperature Historical metallurgy Hydrothermal systems Infrared analysis Isotopes Low temperature Metals Mineral Resources Mineralization Mineralogy Permian Ratios Salinity Salinity effects Silver Sodium chloride Sphalerite Sulfides Sulfur Sulfur isotopes Sulphur Systematics Temperature Trace elements Trace metals Veins (geology) Zincblende |
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| Title | Trace element geochemistry of sphalerite in contrasting hydrothermal fluid systems of the Freiberg district, Germany: insights from LA-ICP-MS analysis, near-infrared light microthermometry of sphalerite-hosted fluid inclusions, and sulfur isotope geochemistry |
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