Suchergebnisse - "Towrie, Michael"
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The effect of powder oxidation on defect formation in laser additive manufacturing
ISSN: 1359-6454, 1873-2453Veröffentlicht: Elsevier Ltd 01.03.2019Veröffentlicht in Acta materialia (01.03.2019)“… Understanding defect formation during laser additive manufacturing (LAM) of virgin, stored, and reused powders is crucial for the production of high quality …”
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In situ X-ray imaging of defect and molten pool dynamics in laser additive manufacturing
ISSN: 2041-1723, 2041-1723Veröffentlicht: London Nature Publishing Group UK 10.04.2018Veröffentlicht in Nature communications (10.04.2018)“… The laser–matter interaction and solidification phenomena associated with laser additive manufacturing (LAM) remain unclear, slowing its process development …”
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Toward control of electron transfer in donor-acceptor molecules by bond-specific infrared excitation
ISSN: 1095-9203, 1095-9203Veröffentlicht: United States 19.12.2014Veröffentlicht in Science (American Association for the Advancement of Science) (19.12.2014)“… Electron transfer (ET) from donor to acceptor is often mediated by nuclear-electronic (vibronic) interactions in molecular bridges. Using an ultrafast …”
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Direct observation of ultrafast long-range charge separation at polymer–fullerene heterojunctions
ISSN: 2041-1723, 2041-1723Veröffentlicht: London Nature Publishing Group UK 01.07.2014Veröffentlicht in Nature communications (01.07.2014)“… In polymeric semiconductors, charge carriers are polarons, which means that the excess charge deforms the molecular structure of the polymer chain that hosts …”
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Direct Observation of the Microscopic Reverse of the Ubiquitous Concerted Metalation Deprotonation Step in C-H Bond Activation Catalysis
ISSN: 1520-5126, 1520-5126Veröffentlicht: United States 27.01.2021Veröffentlicht in Journal of the American Chemical Society (27.01.2021)“… The ability of carboxylate groups to promote the direct functionalization of C-H bonds in organic compounds is unquestionably one of the most important …”
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Directing the path of light-induced electron transfer at a molecular fork using vibrational excitation
ISSN: 1755-4330, 1755-4349, 1755-4349Veröffentlicht: London Nature Publishing Group UK 01.11.2017Veröffentlicht in Nature chemistry (01.11.2017)“… Ultrafast electron transfer in condensed-phase molecular systems is often strongly coupled to intramolecular vibrations that can promote, suppress and direct …”
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Direct observation of two-channel photodissociation of carbon monoxide from the hemoglobin subunits
ISSN: 2041-1723, 2041-1723Veröffentlicht: London Nature Publishing Group UK 20.08.2025Veröffentlicht in Nature communications (20.08.2025)“… Determining dynamics of bond breaking between carbon monoxide (CO) and heme proteins is essential to understand the interplay between protein function and …”
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On the mechanism of vibrational control of light-induced charge transfer in donor–bridge–acceptor assemblies
ISSN: 1755-4330, 1755-4349, 1755-4349Veröffentlicht: London Nature Publishing Group UK 01.09.2015Veröffentlicht in Nature chemistry (01.09.2015)“… Nuclear–electronic (vibronic) coupling is increasingly recognized as a mechanism of major importance in controlling the light-induced function of molecular …”
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A versatile high-average-power ultrafast infrared driver tailored for high-harmonic generation and vibrational spectroscopy
ISSN: 2045-2322, 2045-2322Veröffentlicht: London Nature Publishing Group UK 01.11.2023Veröffentlicht in Scientific reports (01.11.2023)“… We report on an ultrafast infrared optical parametric chirped-pulse amplifier (OPCPA), pumped by a 200-W thin-disk Yb-based regenerative amplifier at a …”
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Electron-Transfer Acceleration Investigated by Time Resolved Infrared Spectroscopy
ISSN: 0001-4842, 1520-4898, 1520-4898Veröffentlicht: United States American Chemical Society 17.03.2015Veröffentlicht in Accounts of chemical research (17.03.2015)“… Ultrafast electron transfer (ET) processes are important primary steps in natural and artificial photosynthesis, as well as in molecular electronic/photonic …”
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Ultrafast excited-state dynamics of rhenium(I) photosensitizers [Re(Cl)(CO)3(N,N)] and [Re(imidazole)(CO)3(N,N)]+: diimine effects
ISSN: 1520-510XVeröffentlicht: United States 04.04.2011Veröffentlicht in Inorganic chemistry (04.04.2011)“… Femto- to picosecond excited-state dynamics of the complexes [Re(L)(CO)(3)(N,N)](n) (N,N = bpy, phen, 4,7-dimethyl-phen (dmp); L = Cl, n = 0; L = imidazole, n …”
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Photoelectrocatalytic H2 evolution from integrated photocatalysts adsorbed on NiO
ISSN: 2041-6520, 2041-6539Veröffentlicht: Cambridge Royal Society of Chemistry 2019Veröffentlicht in Chemical science (Cambridge) (2019)“… A new approach to increasing the faradaic efficiency of dye-sensitised photocathodes for H 2 evolution from water, using integrated photocatalysts, furnished …”
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Photophysics of singlet and triplet intraligand excited states in [ReCl(CO)3(1-(2-pyridyl)-imidazo[1,5-α]pyridine)] complexes
ISSN: 1520-5126Veröffentlicht: United States 23.04.2014Veröffentlicht in Journal of the American Chemical Society (23.04.2014)“… Excited-state characters and dynamics of [ReCl(CO)3(3-R-1-(2-pyridyl)-imidazo[1,5-α]pyridine)] complexes (abbreviated ReGV-R, R = CH3, Ph, PhBu(t), PhCF3, …”
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Photoactivation of the BLUF Protein PixD Probed by the Site-Specific Incorporation of Fluorotyrosine Residues
ISSN: 1520-5126, 1520-5126Veröffentlicht: United States 18.10.2017Veröffentlicht in Journal of the American Chemical Society (18.10.2017)“… The flavin chromophore in blue-light-using FAD (BLUF) photoreceptors is surrounded by a hydrogen bond network that senses and responds to changes in the …”
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Monitoring one-electron photo-oxidation of guanine in DNA crystals using ultrafast infrared spectroscopy
ISSN: 1755-4330, 1755-4349, 1755-4349Veröffentlicht: London Nature Publishing Group UK 01.12.2015Veröffentlicht in Nature chemistry (01.12.2015)“… To understand the molecular origins of diseases caused by ultraviolet and visible light, and also to develop photodynamic therapy, it is important to resolve …”
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Proteins in Action: Femtosecond to Millisecond Structural Dynamics of a Photoactive Flavoprotein
ISSN: 0002-7863, 1520-5126, 1520-5126Veröffentlicht: United States American Chemical Society 30.10.2013Veröffentlicht in Journal of the American Chemical Society (30.10.2013)“… Living systems are fundamentally dependent on the ability of proteins to respond to external stimuli. The mechanism, the underlying structural dynamics, and …”
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Photophysics of Threaded sp-Carbon Chains: The Polyyne is a Sink for Singlet and Triplet Excitation
ISSN: 0002-7863, 1520-5126, 1520-5126Veröffentlicht: United States American Chemical Society 31.12.2014Veröffentlicht in Journal of the American Chemical Society (31.12.2014)“… We have used single-crystal X-ray diffraction and time-resolved UV–NIR–IR absorption spectroscopy to gain insights into the structures and excited-state …”
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Variation in LOV Photoreceptor Activation Dynamics Probed by Time-Resolved Infrared Spectroscopy
ISSN: 1520-4995, 1520-4995Veröffentlicht: United States 06.02.2018Veröffentlicht in Biochemistry (Easton) (06.02.2018)“… The light, oxygen, voltage (LOV) domain proteins are blue light photoreceptors that utilize a noncovalently bound flavin mononucleotide (FMN) cofactor as the …”
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Comparing molecular photofragmentation dynamics in the gas and liquid phases
ISSN: 1463-9084, 1463-9084Veröffentlicht: England 14.05.2013Veröffentlicht in Physical chemistry chemical physics : PCCP (14.05.2013)“… This article explores the extent to which insights gleaned from detailed studies of molecular photodissociations in the gas phase (i.e. under isolated molecule …”
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Steady-State and Pseudo-Steady-State Photocrystallographic Studies on Linkage Isomers of [Ni(Et4dien)(η2-O,ON)(η1-NO2)]: Identification of a New Linkage Isomer
ISSN: 0947-6539, 1521-3765Veröffentlicht: Weinheim WILEY-VCH Verlag 10.03.2014Veröffentlicht in Chemistry : a European journal (10.03.2014)“… At temperatures below 150 K, the photoactivated metastable endo‐nitrito linkage isomer [Ni(Et4dien)(η2‐O,ON)(η1‐ONO)] …”
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