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Stochastic Simulation of Mass Transport under Arbitrary Illumination Conditions: The Influence of the Nanoparticle Localized Surface Plasmon Resonance

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Titel: Stochastic Simulation of Mass Transport under Arbitrary Illumination Conditions: The Influence of the Nanoparticle Localized Surface Plasmon Resonance
Autoren: Franco Lucio Tambosco, Silvia Adriana Ledesma, María Gabriela Capeluto
Publikationsjahr: 2025
Schlagwörter: Ecology, Space Science, Environmental Sciences not elsewhere classified, Biological Sciences not elsewhere classified, Chemical Sciences not elsewhere classified, interference pattern results, driving material away, 229 – 238, 104905 ), however, surface relief grating, arbitrary illumination conditions, surface along, certain conditions, stochastic simulation, srg ), spatial distribution, several hypotheses, nanophotonics 2024, nanoparticle acting, metallic nanoparticles, mass transport, mass propeller, heuristically explain, diffraction efficiency, definitive explanation, avoiding walk, 2946 )
Beschreibung: Mass migration is induced in some azopolymers by illumination with a spatial distribution of intensity, phase, or polarization. In particular, illumination with an interference pattern results in the formation of a surface relief grating (SRG). The addition of metallic nanoparticles to the azopolymer has shown an improvement in diffraction efficiency and modulation (Opt. Mater. 2021, 115, 111015; Nanomaterials 2023, 13, 2946). Several hypotheses have been proposed to heuristically explain this phenomenon (Nanophotonics 2024, 13, 229–238; J. Chem. Phys. 2023, 158, 104905); however, none have offered a definitive explanation. In this work, we present a Monte Carlo model based on the two-dimensional (2D) Self-Avoiding Walk (SAW) method to describe the mass transport in polymer chains surrounding metallic nanoparticles. We propose that under certain conditions, the increased modulation may result from the nanoparticle acting as a mass propeller, driving material away from its surface along the direction of the incoming electric field polarization.
Publikationsart: article in journal/newspaper
Sprache: unknown
Relation: https://figshare.com/articles/journal_contribution/Stochastic_Simulation_of_Mass_Transport_under_Arbitrary_Illumination_Conditions_The_Influence_of_the_Nanoparticle_Localized_Surface_Plasmon_Resonance/29609171
DOI: 10.1021/acs.jpcc.5c02951.s001
Verfügbarkeit: https://doi.org/10.1021/acs.jpcc.5c02951.s001
https://figshare.com/articles/journal_contribution/Stochastic_Simulation_of_Mass_Transport_under_Arbitrary_Illumination_Conditions_The_Influence_of_the_Nanoparticle_Localized_Surface_Plasmon_Resonance/29609171
Rights: CC BY-NC 4.0
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  Data: Stochastic Simulation of Mass Transport under Arbitrary Illumination Conditions: The Influence of the Nanoparticle Localized Surface Plasmon Resonance
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  Data: <searchLink fieldCode="AR" term="%22Franco+Lucio+Tambosco%22">Franco Lucio Tambosco</searchLink><br /><searchLink fieldCode="AR" term="%22Silvia+Adriana+Ledesma%22">Silvia Adriana Ledesma</searchLink><br /><searchLink fieldCode="AR" term="%22María+Gabriela+Capeluto%22">María Gabriela Capeluto</searchLink>
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  Data: 2025
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  Data: <searchLink fieldCode="DE" term="%22Ecology%22">Ecology</searchLink><br /><searchLink fieldCode="DE" term="%22Space+Science%22">Space Science</searchLink><br /><searchLink fieldCode="DE" term="%22Environmental+Sciences+not+elsewhere+classified%22">Environmental Sciences not elsewhere classified</searchLink><br /><searchLink fieldCode="DE" term="%22Biological+Sciences+not+elsewhere+classified%22">Biological Sciences not elsewhere classified</searchLink><br /><searchLink fieldCode="DE" term="%22Chemical+Sciences+not+elsewhere+classified%22">Chemical Sciences not elsewhere classified</searchLink><br /><searchLink fieldCode="DE" term="%22interference+pattern+results%22">interference pattern results</searchLink><br /><searchLink fieldCode="DE" term="%22driving+material+away%22">driving material away</searchLink><br /><searchLink fieldCode="DE" term="%22229+–+238%22">229 – 238</searchLink><br /><searchLink fieldCode="DE" term="%22104905+%29%22">104905 )</searchLink><br /><searchLink fieldCode="DE" term="%22however%22">however</searchLink><br /><searchLink fieldCode="DE" term="%22surface+relief+grating%22">surface relief grating</searchLink><br /><searchLink fieldCode="DE" term="%22arbitrary+illumination+conditions%22">arbitrary illumination conditions</searchLink><br /><searchLink fieldCode="DE" term="%22surface+along%22">surface along</searchLink><br /><searchLink fieldCode="DE" term="%22certain+conditions%22">certain conditions</searchLink><br /><searchLink fieldCode="DE" term="%22stochastic+simulation%22">stochastic simulation</searchLink><br /><searchLink fieldCode="DE" term="%22srg+%29%22">srg )</searchLink><br /><searchLink fieldCode="DE" term="%22spatial+distribution%22">spatial distribution</searchLink><br /><searchLink fieldCode="DE" term="%22several+hypotheses%22">several hypotheses</searchLink><br /><searchLink fieldCode="DE" term="%22nanophotonics+2024%22">nanophotonics 2024</searchLink><br /><searchLink fieldCode="DE" term="%22nanoparticle+acting%22">nanoparticle acting</searchLink><br /><searchLink fieldCode="DE" term="%22metallic+nanoparticles%22">metallic nanoparticles</searchLink><br /><searchLink fieldCode="DE" term="%22mass+transport%22">mass transport</searchLink><br /><searchLink fieldCode="DE" term="%22mass+propeller%22">mass propeller</searchLink><br /><searchLink fieldCode="DE" term="%22heuristically+explain%22">heuristically explain</searchLink><br /><searchLink fieldCode="DE" term="%22diffraction+efficiency%22">diffraction efficiency</searchLink><br /><searchLink fieldCode="DE" term="%22definitive+explanation%22">definitive explanation</searchLink><br /><searchLink fieldCode="DE" term="%22avoiding+walk%22">avoiding walk</searchLink><br /><searchLink fieldCode="DE" term="%222946+%29%22">2946 )</searchLink>
– Name: Abstract
  Label: Description
  Group: Ab
  Data: Mass migration is induced in some azopolymers by illumination with a spatial distribution of intensity, phase, or polarization. In particular, illumination with an interference pattern results in the formation of a surface relief grating (SRG). The addition of metallic nanoparticles to the azopolymer has shown an improvement in diffraction efficiency and modulation (Opt. Mater. 2021, 115, 111015; Nanomaterials 2023, 13, 2946). Several hypotheses have been proposed to heuristically explain this phenomenon (Nanophotonics 2024, 13, 229–238; J. Chem. Phys. 2023, 158, 104905); however, none have offered a definitive explanation. In this work, we present a Monte Carlo model based on the two-dimensional (2D) Self-Avoiding Walk (SAW) method to describe the mass transport in polymer chains surrounding metallic nanoparticles. We propose that under certain conditions, the increased modulation may result from the nanoparticle acting as a mass propeller, driving material away from its surface along the direction of the incoming electric field polarization.
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  Label: Relation
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  Data: https://figshare.com/articles/journal_contribution/Stochastic_Simulation_of_Mass_Transport_under_Arbitrary_Illumination_Conditions_The_Influence_of_the_Nanoparticle_Localized_Surface_Plasmon_Resonance/29609171
– Name: DOI
  Label: DOI
  Group: ID
  Data: 10.1021/acs.jpcc.5c02951.s001
– Name: URL
  Label: Availability
  Group: URL
  Data: https://doi.org/10.1021/acs.jpcc.5c02951.s001<br />https://figshare.com/articles/journal_contribution/Stochastic_Simulation_of_Mass_Transport_under_Arbitrary_Illumination_Conditions_The_Influence_of_the_Nanoparticle_Localized_Surface_Plasmon_Resonance/29609171
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  Data: CC BY-NC 4.0
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  Data: edsbas.C491766D
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      – Type: doi
        Value: 10.1021/acs.jpcc.5c02951.s001
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      – Text: unknown
    Subjects:
      – SubjectFull: Ecology
        Type: general
      – SubjectFull: Space Science
        Type: general
      – SubjectFull: Environmental Sciences not elsewhere classified
        Type: general
      – SubjectFull: Biological Sciences not elsewhere classified
        Type: general
      – SubjectFull: Chemical Sciences not elsewhere classified
        Type: general
      – SubjectFull: interference pattern results
        Type: general
      – SubjectFull: driving material away
        Type: general
      – SubjectFull: 229 – 238
        Type: general
      – SubjectFull: 104905 )
        Type: general
      – SubjectFull: however
        Type: general
      – SubjectFull: surface relief grating
        Type: general
      – SubjectFull: arbitrary illumination conditions
        Type: general
      – SubjectFull: surface along
        Type: general
      – SubjectFull: certain conditions
        Type: general
      – SubjectFull: stochastic simulation
        Type: general
      – SubjectFull: srg )
        Type: general
      – SubjectFull: spatial distribution
        Type: general
      – SubjectFull: several hypotheses
        Type: general
      – SubjectFull: nanophotonics 2024
        Type: general
      – SubjectFull: nanoparticle acting
        Type: general
      – SubjectFull: metallic nanoparticles
        Type: general
      – SubjectFull: mass transport
        Type: general
      – SubjectFull: mass propeller
        Type: general
      – SubjectFull: heuristically explain
        Type: general
      – SubjectFull: diffraction efficiency
        Type: general
      – SubjectFull: definitive explanation
        Type: general
      – SubjectFull: avoiding walk
        Type: general
      – SubjectFull: 2946 )
        Type: general
    Titles:
      – TitleFull: Stochastic Simulation of Mass Transport under Arbitrary Illumination Conditions: The Influence of the Nanoparticle Localized Surface Plasmon Resonance
        Type: main
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            NameFull: Franco Lucio Tambosco
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            NameFull: Silvia Adriana Ledesma
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            NameFull: María Gabriela Capeluto
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              M: 01
              Type: published
              Y: 2025
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