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Review on Structure‐Performance Relationship and Optimization Methods of Catalysts for Electrocatalytic CO2 Reduction Reaction.

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Titel: Review on Structure‐Performance Relationship and Optimization Methods of Catalysts for Electrocatalytic CO2 Reduction Reaction.
Autoren: Guan, Bin, Chen, Junyan, Zhu, Lei, Zhuang, Zhongqi, Hu, Xuehan, Zhu, Chenyu, Zhao, Sikai, Shu, Kaiyou, Dang, Hongtao, Gao, Junjie, Zhang, Luyang, Zhu, Tiankui, Zeng, Wenbo, Qian, Minfan, Li, Zhangtong, Lu, Yang, Chen, Shuai, Huang, Zhen
Quelle: ChemistrySelect; 10/6/2025, Vol. 10 Issue 37, p1-32, 32p
Schlagwörter: CARBON dioxide reduction, CATALYSTS, TRANSITION metal catalysts, MATHEMATICAL optimization, CARBON-based materials, CLEAN energy, METAL catalysts
Abstract: The electrocatalytic CO2 reduction reaction (CO2RR) holds great promise for converting CO2 into value‐added fuels and mitigating global carbon emissions. Electrocatalysts play a pivotal role in enhancing reaction efficiency, reducing overpotential, and improving product selectivity, making them the core of CO2RR research. This review systematically summarizes recent advances in CO2RR electrocatalysts, focusing on the structure‐performance relationships and optimization strategies. Noble metal catalysts exhibit excellent catalytic activity and stability, but their high cost limits large‐scale applications; nanostructuring and element doping have been developed to improve their efficiency and reduce usage. Transition metal complex catalysts show great potential due to their low cost and high performance, with optimization approaches including coordination structure design, nanostructure engineering, and bimetallic alloying to regulate active sites and electron transfer. Carbon‐based materials, including modified carbon, biomass‐derived carbon, and MOF‐derived carbon, have emerged as cost‐effective alternatives, with heteroatom doping and defect engineering being key to enhancing their catalytic activity. By integrating the latest research on catalyst design, modification, and mechanism exploration, this review aims to provide comprehensive insights for developing high‐efficiency, low‐cost CO2RR electrocatalysts, promoting their practical application in carbon neutrality and sustainable energy conversion. [ABSTRACT FROM AUTHOR]
Copyright of ChemistrySelect is the property of Wiley-Blackwell and its content may not be copied or emailed to multiple sites without the copyright holder's express written permission. Additionally, content may not be used with any artificial intelligence tools or machine learning technologies. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract. (Copyright applies to all Abstracts.)
Datenbank: Complementary Index
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  Data: Review on Structure‐Performance Relationship and Optimization Methods of Catalysts for Electrocatalytic CO<subscript>2</subscript> Reduction Reaction.
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  Data: <searchLink fieldCode="AR" term="%22Guan%2C+Bin%22">Guan, Bin</searchLink><br /><searchLink fieldCode="AR" term="%22Chen%2C+Junyan%22">Chen, Junyan</searchLink><br /><searchLink fieldCode="AR" term="%22Zhu%2C+Lei%22">Zhu, Lei</searchLink><br /><searchLink fieldCode="AR" term="%22Zhuang%2C+Zhongqi%22">Zhuang, Zhongqi</searchLink><br /><searchLink fieldCode="AR" term="%22Hu%2C+Xuehan%22">Hu, Xuehan</searchLink><br /><searchLink fieldCode="AR" term="%22Zhu%2C+Chenyu%22">Zhu, Chenyu</searchLink><br /><searchLink fieldCode="AR" term="%22Zhao%2C+Sikai%22">Zhao, Sikai</searchLink><br /><searchLink fieldCode="AR" term="%22Shu%2C+Kaiyou%22">Shu, Kaiyou</searchLink><br /><searchLink fieldCode="AR" term="%22Dang%2C+Hongtao%22">Dang, Hongtao</searchLink><br /><searchLink fieldCode="AR" term="%22Gao%2C+Junjie%22">Gao, Junjie</searchLink><br /><searchLink fieldCode="AR" term="%22Zhang%2C+Luyang%22">Zhang, Luyang</searchLink><br /><searchLink fieldCode="AR" term="%22Zhu%2C+Tiankui%22">Zhu, Tiankui</searchLink><br /><searchLink fieldCode="AR" term="%22Zeng%2C+Wenbo%22">Zeng, Wenbo</searchLink><br /><searchLink fieldCode="AR" term="%22Qian%2C+Minfan%22">Qian, Minfan</searchLink><br /><searchLink fieldCode="AR" term="%22Li%2C+Zhangtong%22">Li, Zhangtong</searchLink><br /><searchLink fieldCode="AR" term="%22Lu%2C+Yang%22">Lu, Yang</searchLink><br /><searchLink fieldCode="AR" term="%22Chen%2C+Shuai%22">Chen, Shuai</searchLink><br /><searchLink fieldCode="AR" term="%22Huang%2C+Zhen%22">Huang, Zhen</searchLink>
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  Data: ChemistrySelect; 10/6/2025, Vol. 10 Issue 37, p1-32, 32p
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  Data: <searchLink fieldCode="DE" term="%22CARBON+dioxide+reduction%22">CARBON dioxide reduction</searchLink><br /><searchLink fieldCode="DE" term="%22CATALYSTS%22">CATALYSTS</searchLink><br /><searchLink fieldCode="DE" term="%22TRANSITION+metal+catalysts%22">TRANSITION metal catalysts</searchLink><br /><searchLink fieldCode="DE" term="%22MATHEMATICAL+optimization%22">MATHEMATICAL optimization</searchLink><br /><searchLink fieldCode="DE" term="%22CARBON-based+materials%22">CARBON-based materials</searchLink><br /><searchLink fieldCode="DE" term="%22CLEAN+energy%22">CLEAN energy</searchLink><br /><searchLink fieldCode="DE" term="%22METAL+catalysts%22">METAL catalysts</searchLink>
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  Label: Abstract
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  Data: The electrocatalytic CO2 reduction reaction (CO2RR) holds great promise for converting CO2 into value‐added fuels and mitigating global carbon emissions. Electrocatalysts play a pivotal role in enhancing reaction efficiency, reducing overpotential, and improving product selectivity, making them the core of CO2RR research. This review systematically summarizes recent advances in CO2RR electrocatalysts, focusing on the structure‐performance relationships and optimization strategies. Noble metal catalysts exhibit excellent catalytic activity and stability, but their high cost limits large‐scale applications; nanostructuring and element doping have been developed to improve their efficiency and reduce usage. Transition metal complex catalysts show great potential due to their low cost and high performance, with optimization approaches including coordination structure design, nanostructure engineering, and bimetallic alloying to regulate active sites and electron transfer. Carbon‐based materials, including modified carbon, biomass‐derived carbon, and MOF‐derived carbon, have emerged as cost‐effective alternatives, with heteroatom doping and defect engineering being key to enhancing their catalytic activity. By integrating the latest research on catalyst design, modification, and mechanism exploration, this review aims to provide comprehensive insights for developing high‐efficiency, low‐cost CO2RR electrocatalysts, promoting their practical application in carbon neutrality and sustainable energy conversion. [ABSTRACT FROM AUTHOR]
– Name: Abstract
  Label:
  Group: Ab
  Data: <i>Copyright of ChemistrySelect is the property of Wiley-Blackwell and its content may not be copied or emailed to multiple sites without the copyright holder's express written permission. Additionally, content may not be used with any artificial intelligence tools or machine learning technologies. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract.</i> (Copyright applies to all Abstracts.)
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        Value: 10.1002/slct.202503072
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        Text: English
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        PageCount: 32
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